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We propose a device where Electronic Quantum Optics (EQO) is combined with a BCS supercon-
ductor – a reservoir of Cooper pairs. With spin polarized wave guides, this version of the Cooper
pair beam splitter is driven by an AC drive, and observables such as period-averaged noise are com-
puted using a Keldysh-Nambu-Floquet formalism. When the (low frequency) voltage applied to the
superconductor consists of a train of periodic Lorentzian pulses and the Andreev regime is specified
(large gap limit), this allows to propose an on-demand source of non-local energy-entangled states
arXiv:2302.10744v1 [cond-mat.supr-con] 21 Feb 2023
(which we characterise with perturbation theory) operating in the AC regime. We study realistic
experimental parameters for our device in order to examine its feasibility.
ized) normal metal/superconducting junction subject to order to show the limitations of the relevance of minimal
a periodic voltage bias drive [21] using a Keldysh-Nambu- noise (the latter can become negative). A side result of
Floquet approach: it was possible to get analytical results this work – yet of great relevance for the present work –
for both current and noise in the small and the large gap was the proposal for an on-demand Cooper pair source
regime, but also for drive frequencies which are compara- operating in an AC regime, whose parameters (trans-
ble to the gap (the latter numerically). As we shall see, parency, Leviton charge, temperature, frequency) where
this work can be exploited in the present context of an optimized with respect to ∆ in order to generate with ac-
on-demand source of non-local energy-entangled states, curacy one Cooper pair per period in the superconductor
provided a multi-lead generalization of the results is op- for the regime ∆ Ω. In the present paper, we build on
erated. The scope of this paper is as follows: in Sec. II we this previous result and detail the theoretical proposal of
describe how the device operates, in Sec. III the Hamil- an optimized source of energy-entangled states based on
tonian, the Green’s function formalism and analytical re- Levitons.
sults are presented, in Sec. IV, the optimal parameters Separation of the two electronic excitations. As the two
of the source are specified. We discuss our results and constituent electrons of a Cooper pair have opposite
potential extensions in Sec. V. spins, a natural choice is to connect the superconductor
to two distinct electron wave guides with opposite spin
polarization. This can be achieved by using two half
II. DEVICE CHARACTERISTICS
metals, whose separation needs to be smaller than the
superconducting coherence length (see Ref. [28]): in the
Energy entanglement. As mentioned in the introduction, Andreev regime the tunneling between normal and super-
the fact that we are transferring electron excitations in conducting regions is expected to be dominated by CAR.
two spin-polarized leads does not allow us to generate Here, we choose specifically to connect the superconduc-
spin entangled delocalized electron pairs. In order to il- tor to a Quantum Spin Hall (QSH) bar, as presented in
lustrate the dual nature – spin v.s. energy – of entangle- Fig. 1. This has two advantages: first, QSH bars are
ment originating from a BCS superconductor, we extract two dimensional topological insulators which (thanks to
the ±~k component of the BCS wave function: spin-momentum locking) bear on their edges two spin
channels which propagate in opposite chiralities; second,
(±~
|ΨBCS i ∼ uk vk (c~† c† ~ − c~† c† ~ )|0i ,
k)
(1) direct Andreev reflection (rather than CAR) splits the
k↑ −k↓ k↓ −k↑
two constituent electrons of the Cooper pairs. The two
where uk (vk ) are the usual parameters of the BCS wave spin dependent excitations which are generated are thus
function [24]. Strickly speaking, in the device of Fig. naturally delocalized.
1, energy – rather than momentum – entanglement can Generation of non-local energy-entangled states. Before
be preserved for electrons tunneling to spin polarized presenting our results on the transport properties of the
leads [1], because of the lack of translational symme- system, we motivate our proposal by a perturbative cal-
try. This non-local energy entanglement was justified culation of the final quantum state propagating in the
by a Bell-Clauser Horne inequality [25] violation test in QSH channels when we apply a single Lorentzian volt-
Ref. [23]. age pulse to both of the spin-polarized channels of the
Controlled two electron emission. Recently in Ref. [21] QSH lead. In the Andreev regime, where the gap ∆
we studied a hybrid normal metal/superconductor de- is the largest relevant energy, charge exchange between
vice where a DC and AC voltage drive was applied on the QSH lead and the superconductor can only occur
the normal lead, with the goal to study minimal noise: through Andreev reflection, where only Cooper pairs can
under which conditions can electron wave packets be be transferred to the superconductor. This implies that
sent impinging on the superconductor without unwanted the charge of the output state is twice the charge excited
electron-hole pairs ? There, two limits served as bench- by the voltage pulse. In order to obtain a final state with
marks (where analytical expressions for the current and a charge 2e, corresponding to the emission of a single
noise could be obtained): the small superconducting gap Cooper pair, we thus excite a charge e/2 on each spin-
limit ∆ Ω (Ω is the frequency of the drive) where the polarized lead. This is obtained by using the pulse:
transport process is dominated by quasiparticle transfer
above the gap and behaves like a normal junction, and 1 1
eV (t) = − (2)
the large gap limit ∆ Ω where Andreev reflection op- 2πW 1 + t2 /W 2
erates in majority. In the former case it was proved that
integer Levitons (Lorentzian voltage pulses) lead to min- with a width W ∆−1 in order to be in the Andreev
imal excess noise (the difference between the period av- regime.
eraged noise and the equivalent DC noise) [21, 26], while As the tunneling Hamiltonian exchanges one electron
in the latter, Levitons with half-integer charge lead to between the polarized leads and the superconductor (see
minimal noise [21, 27]. Moreover, in Ref. [21] we were Sec.III), two tunneling events are required in the An-
able to describe the intermediate regime ∆ ∼ Ω using dreev regime to inject excitations in the edge states. For
numerics (for a junction with arbitrary transparency) in this reason, a perturbative calculation to second order in
3
the tunneling between the QSH lead and the supercon- that, in the absence of a time dependent bias, both spin-
ductor is required. Using second order time-dependent polarized channels have their Fermi energy equal to the
perturbation theory, with the Hamiltonian model speci- chemical potential of the superconductor, the resulting
fied in Sec.III, we computed the quantum state generated state at the output for large times is found to be:
at large times by the application of V (t) [29]. Assuming
∞ ε
λ2
Z Z
|Fi = i dε ϕT (2ε) dEc†k(ε+E),↑ c†k(ε−E),↓ |F↑ i ⊗ |F↓ i ⊗ |ΨBCS i . (3)
4π 2 −∞ −ε
where λ is the tunneling amplitude between leads while The different leads are described in equilibrium by the
|F↑ i and |F↓ i are the Fermi seas for the spin-polarized following Hamiltonians
channels. For convenience, we set the density of states
ν0 of the superconducting lead at its chemical potential HN = H0,↑ + H0,↓
such that πν0 = 1. We also introduced X
HS = H0,↑ + H0,↓ + ∆ c†i,S,↓ c†i,S,↑ + ci,S,↓ ci,S,↑ ,
ϕT (ε) = δ(ε) + 2W e−W ε H(ε) , (4) i
(5)
as the Fourier transform of exp [−2iφ(t)], where the phase where H0,σ is the kinetic part of the Hamiltonian for the
Rt spin-σ polarized lead, i labels the various sites of these
reads φ(t) = e −∞ dτ V (τ ), and H() is the Heaviside
leads, ∆ is the superconducting gap and the chemical
distribution.
potential is set to zero in all electrodes. Here ci,j,σ is
We stress that this state is energy-entangled, i.e., one
the electron annihilation operator at site i on the j lead
cannot factorize it into a product of two states acting
(j = S for the superconductor), with spin σ. The tunnel
separately on the Fermi seas of the leads. Moreover, this
Hamiltonian is defined as
final state is purely electronic, i.e. devoid of additional
hole-like excitations or electron-hole pairs. This can be
λj,j 0 eiφj,j0 (t)/2 c†ejj0 ,j,σ cej0 ,j ,j 0 ,σ + H.c. , (6)
X
HT (t) =
achieved only by pulses with Lorentzian shape carrying
j,j 0 ,σ
a half-integer charge (or an integer multiple of it), and
cannot be generalized to other types of signals. An ex- where λj,j 0 is the tunneling amplitude from lead j to
tension of this single pulse perturbative treatment to a lead j 0 , ei,j denotes the site of lead i from which tun-
periodic train of Lorentzian pulses will be presented else- Rt
where. [29] neling to lead j occurs, and φjj 0 (t) = e −∞ dt0 Vjj 0 (t0 )
It seems reasonable to speculate that, in the An- is the time-dependent phase difference between the leads
dreev regime, our results can be extended to the which accounts for the drive-induced voltage difference
non-perturbative regime by the replacement λ2 → Vjj 0 (t) between lead j 0 and lead j. One can introduce
λ2 / 1 + λ4 . This conjecture is based on the fact that
the tunnel matrix in lead space Wjj 0 = λjj 0 σz eσz iφjj0 (t)/2
the vanishing of excess-noise for quantized Lorentzian for leads carrying both spin orientation. For the device of
pulse is indeed obtained in the non-perturbative regime Fig. 1, the superconducting lead is connected to the spin-
of tunneling. polarized chiral edge states of the QSH bar, so that j can
be identified with the spin index to describe the QSH part
of the device. This allows us to replace the σz prefactor
III. HAMILTONIAN AND NOISE in WSj 0 by (σz ±σ0 )/2 (for j 0 =↑, ↓). Also, the direct tun-
CALCULATION nel coupling between the two counter-propagating edge
states vanishes λ↑↓ = 0, and we mostly focus on the
We focus on the device represented in Fig. 1 corre- symmetric situation where λS↑ = λS↓ = λ (as implicitly
sponding to a junction between a BCS superconduc- assumed in Eq. (3)). P
tor and a QSH edge state. Using the properties of Writing the Hamiltonian as H = j Hj + HTun , the
spin-momentum locking of the QSH, the latter lead can current operator from lead j is given by
be viewed, from a formal point of view, as two de-
iψj† (t)σz Wjj 0 (t)ψj 0 (t) + H.c.
X
coupled spin-polarized reservoirs so that we are dealing Ij (t) = (7)
with an effective three-terminal device. The formalism j0
of Ref. [21] is thus naturally extended to a multi-lead
setup, with an arbitrary number of (spin polarized) nor- The real time irreducible noise correlator between lead j
mal leads. Note that, strictly speaking, a similar for- and l is defined as
malism could very well be used to describe a junction h i
involving half-metals instead. Sjl (t, t0 ) = hIj (t + t0 ) Il (t)i−hIj (t + t0 )i hIl (t)i , (8)
4
where we introduced the standard Nambu spinor nota- Keldysh contour. We look at Sjl (t), the zero frequency
tion ψj for the electron operators. It can be computed in component of the noise with respect to time difference t0 .
the framework of Keldysh theory [30] D with the KeldyshE Because the Hamiltonian is quadratic one can safely use
Green’s function G±∓ 0 ± † ∓ 0
Wick’ theorem to cast the noise as a product of single
jj 0 (t, t ) = −i TK ψj (t )ψj 0 (t ) ,
particle Green’s functions:
where TK denotes Keldysh ordering, and ± superscripts
have been added to t and t0 to specify the branch of the
e2 X
Z
dt0 TrN σz Wjj 0 (t)G−+ 0 0 +− 0 −+ 0 0 +− 0
Sjl (t) = − j 0 l (t, t )σz Wll (t )Gl0 j (t , t) + σz Wj j (t)Gjl0 (t, t )σz Wl l (t )Glj 0 (t , t)
0 0 0
~ 00 (9)
j l
−+ 0 0 +− 0 −+ 0 0 +− 0
−σz Wj 0 j (t)Gjl (t, t )σz Wll0 (t )Gl0 j 0 (t , t) − σz Wjj 0 (t)Gj 0 l0 (t, t )σz Wl0 l (t )Glj (t , t) .
0 0.5 1
ism which has been used profusely in Refs. [21, 31, 32]
and we refer the reader to these works. Fundamen- 0.25
b) θ = 0.001
tally, it amounts to recast the two-time Green’ func-
0.2
tions using two frequencies then use the periodicity in the
drive frequency Ω to our advantage in order to express
0.15
the correlation functions in terms of a single frequency
and two harmonic indices so that the Green’s function 0.1
G(ω + nΩ, ω + mΩ) is converted into a matrix function
Gnm (ω). 0.05
Defining the advanced/retarded self-energy entering
the Dyson equation as the matrix in Nambu-lead- 0
harmonics space Σ(t, t0 ) = δ(t − t0 )W (t) it can be shown 0 0.5 1
that its lead-harmonics components yield q
pjj 0 ,n−m 0
Σjj ,mn (ω) = λjj
0 0 . (10) Figure 2. Excess noise for the device driven by a cosine, a
0 −p∗jj 0 ,m−n
periodic square and a periodic Lorentzian drive (with relative
width η = 0.15) as a function of the injected charge q in the
The time-averaged noise can then be written as the Andreev regime Ω = 10−2 ∆. a) experimentally realistic tem-
energy integral of a Nambu-harmonics trace, allowing to perature (see below), θ = 5 × 10−4 ∆ and b) very low reduced
obtain the zero-frequency period averaged noise (PAN) temperature θ = 10−5 ∆. These plots are independent of the
R T /2
hSjl i ≡ −T /2 dt
T hSjl (t) + Slj (t)i.
tunnel coupling (for this figure λ = 0.5).
The Dyson equation in Nambu-harmonics space were
solved in [21], and the extension to the multi-lead case is
straightforward. We define the total excess noise as have a unique transport channel hS↑↓ i = hS↓↑ i = hS↑↑ i =
hS↓↓ i, see [1]) is the total noise of the source.
In the case of a two terminal N-S device, the auto-
Sexc = hST i − hST i . (11)
DC+AC DC correlations on the normal side were obtained for arbi-
P trary ∆ and Ω in Ref. [21]. The same applies for the
where hST i ≡ σ,σ 0 =↑,↓ hSσσ0 i (note that because we present effective three-terminal geometry (see Fig. 1).
5
In the pure Andreev regime Ω ∆, the total noise of To achieve a reliable, controlled source of entangled
the source has the analytical expression: states, one needs to ensure two important properties: the
average charge transmitted through the junction per pe-
e2
riod should be quantized, corresponding to an even num-
hST iq = 4τA2 θ + 2τA (1 − τA )
π ber of electrons, and the excess noise should be vanish-
X
Ω
ingly small so as to generate primarily minimal excitation
× (2q + n)ΩPn (2q) coth (2q + n) , states.
n
2θ The average charge transmitted per period is defined
(12) as
where τA = 4λ4 /(1 + λ4 )2 .
In Fig. 2, we use the full numerical approach to com- hIiq
hQi = 2π = 4qeτA , (14)
pute the excess noise, relying on a numerical solution of Ω
the Dyson equation in Keldysh-Nambu-Floquet space al- see [21]. An ideal source of energy-entangled states would
lowing us to compute the transport properties for any thus require to operate at near perfect transmission and
set of parameters. There, we observe that with the cho- tune the bias voltage such that the injected charge q is
sen parameters, the curves match exactly with the excess half-integer, leading to the emission of exactly 2q ∈ N
noise obtained in the Andreev regime using Eq. (12). Cooper pairs per period into the leads. Surprisingly, this
This excess noise is plotted both at finite (top) and zero turns out to be independent of the type of AC drive
(bottom) temperature, and minimal noise is achieved for considered. However, the second property of such an
half-integer and integer q at zero temperature, and for ideal source, the minimization of excess noise, can only
slightly higher values of q when the temperature is finite. be achieved by a Leviton voltage drive, as we will show
Periodic trains of Levitons always lead to minimal noise below.
when compared to cosine, or square voltages, as defined Following our numerical results at low temperature
in Ref. [21]: which are displayed in Fig. 2, we can argue that the quan-
tized periodic Lorentzian drive shows the lowest excess
Vcos (t) = VDC (1 − cos Ωt) noise. In the limit of zero temperature, this is demon-
Vsqu (t) = VDC [1 + sgn (cos Ωt)] strated by considering the expression for the excess noise
! (13) in the Andreev regime, obtained from Eq. (12),
1X η
Vlor (t) = VDC .
π η + (t/T − k)2
2 X
k Sexc (q) ∝ Pn |2q + n| [1 − Sgn (2q + n)] . (15)
n
1 are centered around λ ' 0.78, i.e., τA ' 0.79) for which
9 the excess noise is close to the minimum allowed for this
0.8 choice of temperature and drive frequency. We remark
7 that this corresponds to a value of q ∗ ' 0.65, in this
0.6 regime the Lorentzian drive displays the minimal noise,
5 as can be seen in Fig. 2. While one understands that a
q∗
s
channels is quantized. The model here employed to de- is the required high transparency, which may be difficult
scribe the QSH bar is relevant as long as electronic inter- to achieve in experiments. If this assumption is relaxed
action between the two spin channels can be neglected, our device would rather become a stochastic [36] source
and the inclusion of electronic correlations would further of non-local energy-entangled states which (for a period
require a Luttinger liquid picture in order to account for interval of the drive), generates a random time sequence
fractionalization phenomena [35]. Finally, a strong as- of either states of the type F or vacuum states.
sumption for the ideal operation of the device of Fig. 1