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266 IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, VOL. 59, NO.

1, JANUARY/FEBRUARY 2023

Study on Failure Mechanism of Oil Paper Insulation


Under Partial Discharge of Interlayer Bubble
Junjie Zhou , Qiaogen Zhang, Rui Zhang, Zhicheng Wu , Tao Wen , and Chong Guo

Abstract—Partial discharge (PD) induced by bubble will reduce insulation, bubbles bound between paper layers are very easy
the insulation performance, lead to insulation failure and seri- to induce partial discharge (PD), which seriously threatens the
ously affect the safe operation of power transformer. Studying safe stable operation of power transformers [7].
the influence of PD in internal bubble on oil paper insulation
and understanding the insulation failure mechanism can provide The influence of bubble PD in oil paper insulation has received
guidance for engineering practice. In this paper, a bubble PD extensive attention. The existence of bubbles will reduce the
defect model is designed to obtain the mechanism of PD degrading insulation performance. Literature [8] concluded that air bubbles
insulation. The inception and breakdown voltage of PD decrease from 100 μm to 200 μm can reduce the breakdown voltage
seriously with the increase of bubble area and height. Combined of insulating oil by 34% and sulfur hexafluoride bubbles can
with the surface state of breakdown paper observed by electron
microscope, it is concluded that PD can induce the breakdown reduce it by 19%. Usually, the internal voltage on oil paper
of oil paper insulation. Then, through the comparative analysis insulation of transformer in operation is difficult to directly
of bubble area and PD parameters, a positive feedback model for cause breakdown, instead it will induce PD in bubble, which
insulation degradation is obtained, representing that bubble defects will degrade insulation performance gradually [9]. Therefore,
will deteriorate rapidly in exponential form under the effect of the detection and identification of PD characteristics have pro-
PD. Finally, combined with the electron microscope and energy
spectrum analysis, the deterioration process of insulating paper vided direction for judging the insulation state [10]. Lots of
is divided into four stages, obtaining the micro deterioration and research has been done on the characteristics of bubble PD,
failure mechanism of insulating paper. This study contributes to including insulation breakdown voltage, PD inception voltage
understanding the mechanism of insulation failure by bubble, as and evolution process [11], [12]. Some research extracted the
well as provides a reference for risk assessment of transformers. characteristic information of PD including discharge, repetition
Index Terms—Cumulative damage, induced breakdown, oil rate and PRPD pattern, then divided and optimized the phases
paper insulation, partial discharge of bubble, positive feedback. by various algorithms, which provided guidance for the identifi-
cation of insulation degradation [13]. Also, some scholars have
I. INTRODUCTION divided the degradation stage of insulating paper according to
the polymerization degree of insulating paper under PD [14].
IL paper insulation undertakes the main insulation task
O of oil-immersed power transformer [1], [2]. And with the
development of power system, the voltage level and capacity
However, some key issues remain unresolved. First, the size
of bubble defect in previous studies remains unchanged, which
makes the aggravating effect of long-term PD on bubble defects
of oil-immersed power transformer are increasing gradually, unable to be reflected. In fact, the parameters of bubble change
making the oil paper insulation bears more severe stresses. Under with the development of PD, which may lead to the inconsistency
the effect of multiple stresses such as electricity, temperature, between the experimental results and the practice. Second, the
mechanical vibration, environmental factors and material aging, existing research studied the evolution process and other char-
power transformers in long-term operation will produce bubbles acteristics of PD unilaterally, and has not linked the bubble PD
in the paper layer between insulation turns [3], [4], [5], [6]. As with the deterioration and failure process of insulating paper.
the dielectric strength of gas is much lower than that of oil paper The relationship between the evolution of bubble PD and the
deterioration of insulating paper is unclear. Third, scant attention
Manuscript received 22 March 2022; revised 1 August 2022; accepted 10 has been paid to the evolution process of micro morphology on
September 2022. Date of publication 15 September 2022; date of current version
19 January 2023. Paper 2022-PSEC-0341.R1, presented at the 2021 IEEE 2nd
insulating paper surface, and failed to obtain the micro mecha-
China International Youth Conference on Electrical Engineering, Chengdu, nism of insulation failure under long-term PD. Establishing the
China, Dec. 15–17, and approved for publication in the IEEE TRANSACTIONS relationship between the micro surface morphology of insulating
ON INDUSTRY APPLICATIONS by the Power Systems Engineering Committee
of the IEEE Industry Applications Society. This work was supported by the
paper and degree of deterioration is significant to directly judge
Science and Technology Project of State Grid Corporation of China under Grant the insulation state.
52060021002T. (Corresponding author: Qiaogen Zhang.) Therefore, from the perspective of breakdown and micro
The authors are with the State Key Laboratory of Electric Insulation and Power
Equipment, Xi’an Jiaotong University, Xi’an, Shaanxi 710049, China (e-mail:
damage on insulating paper, this paper analyzed the PD charac-
junjie_zhou_c@163.com; hvzhang@xjtu.edu.cn; zhang_rui@stu.xjtu.edu.cn; teristics of bubbles between oil paper insulation layers and their
z_c_wu@163.com; tao-wen@xjtu.edu.cn; 13946204699@163.com). influence on oil paper insulation. This research aims to reveal the
Color versions of one or more figures in this article are available at
https://doi.org/10.1109/TIA.2022.3207118.
physical mechanism of bubble discharge deteriorating oil paper
Digital Object Identifier 10.1109/TIA.2022.3207118 insulation and evaluate its harm. The contributions are structured

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ZHOU et al.: STUDY ON FAILURE MECHANISM OF OIL PAPER INSULATION UNDER PARTIAL DISCHARGE OF INTERLAYER BUBBLE 267

Fig. 2. Bubble partial discharge model structure and setting process:


(a) schematic flow of bubble height and area control method; (b-1)∼(b-3):
Fig. 1. PD measuring circuit. actual images of test sample (c) side view schematic diagram of test sample;
(d) simulation results of electric field distribution of test sample.

as follows. Section Ⅱ details the experimental setup and method.


Section Ⅲ reports the experimental result of bubble PD. Section For micro measurement part, Zeiss field emission electron
Ⅳ carries out the discussion on two failure mechanisms. Section microscope (GeminiSEM 500) is used to observe the surface
Ⅴ summarizes the main contributions. topography of different samples. At the same time, the surface
elements of insulating paper at different damage stages are
obtained by energy spectrum analysis, and the PD characteristics
II. EXPERIMENTAL SETUP AND PROCEDURE
in bubbles can be analyzed from the perspective of element
In order to obtain the failure mechanism of bubble PD on content and distribution.
oil paper insulation through repeated tests, the following points
need to be specially considered in the design of the experimental B. Test Cell
system:
1) The area and height of bubble in paper layers can be ad- Before sample construction, the insulating paper and oil need
justed conveniently before the experiment, and the bubble to be dried to remove moisture according to IEC 60641. The
height can be kept unchanged during the experiment. insulating paper and insulating oil are dried in vacuum box at
2) The high-voltage circuit needs to be disconnected imme- 105 °C and 80 °C respectively for 24 h. Then the insulating paper
diately within milliseconds after insulation breakdown to is immersed in the oil and vacuum dried at 80 °C for another
reduce the impact of arc discharge on the surface morphol- 24 h. Finally, stop heating and continue to maintain the vacuum
ogy of insulating paper. for 24 h, to make the temperature gradually decrease from 80°C
The details are as follows. to room temperature. After drying, the construction method and
results of the test sample are shown in Fig. 2.
Fig. 2(a) shows the setting method of interlayer bubbles:
A. Experimental Circuit 1) The ground electrode is tightly wrapped by multi-layer
The test circuit is shown in Fig. 1. It consists of three parts: Weidmann paper (relative permittivity is 4.4) whose thick-
high voltage generating circuit, testing circuit and measuring ness is 70 μm and width is 40 mm to simulate the oil-paper
circuit. The electric voltage regulator is used to realize the insulation structure between turns of transformer.
flexible regulation of input 50 Hz voltage, which can easily 2) A PVC film with a specific thickness and a through hole
control the rising rate and voltage stage. After the regula- in the middle is placed between the paper layers to control
tor, the voltage is boosted by 50 kV non-PD test transformer the distance between insulating papers.
(25 kVA) and applying on the sample after a protective resistance 3) A certain volume of gas is injected into the through hole
(R) of 100 kΩ. And a circuit breaker is set between the voltage by microinjector.
regulator and test transformer. When the sample breaks down, 4) The size of unit pixel is calculated according to the 40 mm
the breaker can disconnect the power supply within several width of insulating paper and the number of image pixels,
milliseconds, which ensures that the surface morphology of and then the area of bubble is obtained according to the
insulating paper will not be affected by the breakdown. The number of pixels of bubble.
high voltage is measured by 10000:1 resistance voltage divider 5) Multiply the calculated area by the thickness of PVC and
(R1 and R2 ) and displayed by oscilloscope (DPO3014200 MHz, compare it with the injection volume. If the difference
2.5 Gs/s). According to IEC60270, the PD signal of bubble is between the two is less than 5%, it can be considered
obtained by pulse current method. By coupling capacitance and that the area and height of bubbles have been accurately
impedance detection (Cp and ZM ), the system can record the controlled. Otherwise, the sample structure needs to be
apparent charge, discharge repetition rate and PRPD patterns in adjusted.
time, which is sent to the HAEFELY DDX91221b PD detector Based on the above sample preparation method, Fig. 2(b-1) to
for measurement and processing [15]. Fig. 2(b-3) are the images of sample with no bubble, small bubble

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268 IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, VOL. 59, NO. 1, JANUARY/FEBRUARY 2023

and large bubble respectively, which shows that bubbles are


bound between the insulating paper layers, forming multilayer
structure of insulating paper, oil and bubble. Fig. 2(c) is the
diagram of side view, which further shows the structure of the test
sample, that is, bubble is added between the wrapped multilayer
insulating paper. Finally, a two-dimensional axisymmetric simu-
lation model of the electrode system is established by COMSOL
simulation software, and the electric field distribution in the
sample is obtained, as shown in Fig. 2(d). where R is the radius
of the disk bubble, H is the height of the bubble, D is the gap Fig. 3. Withstand characteristics: (a) influence of bubble area on PDIV and
distance, and the applied voltage in the model is 10 kV. Taking BV. (b) Effect of bubble height on BE at two voltage raising rates.
bubble with radius of 10 mm, height of 0.4 mm and height of 0.8
mm as example, the distribution of electric field in the sample
of the area. The highest breakdown voltage in a small area
and the electric field non-uniformity coefficient corresponding
decreases from above 15 kV to about 4 kV in a large area. And
to different height and radius are obtained through electrostatic
the larger the area, the closer the PDIV is to the BV. As the bubble
field simulation.
height increases, BE also decreases rapidly from 14 kV/mm to 7
kV/mm. There is little difference in BE under different voltage
III. EXPERIMENTAL RESULT rising rates, and the maximum difference on BE is less than
A. Breakdown Characteristics of Oil-paper Insulation 6.56%.
This is explained as follows: PD in bubbles induces oil-paper
The existence of bubbles will affect the voltage withstand
insulation breakdown. For the bubble area, charges will accumu-
capacity of oil paper insulation. Studies on the influence of
late on the surfaces at both ends of the bubble, which enhances
bubble size on breakdown characteristics of oil paper insulation
the space electric field in the oil gap [18], [19]. And with the
and quantitatively obtaining the variation laws of breakdown
increase of area, the repetition rate of PD also increases, which
voltage of oil paper insulation with different bubble area and
is equivalent to increasing the number of inductions. Therefore,
height are significant in understanding the threat of bubbles [16],
it’s more likely to cause streamer discharge in the oil gap, which
[17]. Therefore, this paper studied the short-time breakdown
lead to the whole insulation breakdown. In a word, when the
characteristics of oil paper insulation by step-up method, and the
area increases to a certain extent, PD can induce breakdown
voltage withstand characteristics of oil paper insulation under
once it starts. For the bubble height, the higher the height,
bubble defects with different area and height are obtained.
the stronger the electric field in the bubble, and the inception
First, it’s necessary to obtain and eliminate the influence of
probability of PD is greater. After the bubble PD occurs, all
PVC film. In pre-experiments, the voltage is increased at the rate
voltage is on the remaining oil paper insulation. Therefore, the
of 1 kV/s without bubble and only adding PVC film. The results
higher the bubble, the greater the voltage borne by the remain-
show that there is no PD inception under the voltage of 25 kV.
ing oil paper insulation, which are easier to cause breakdown.
What’s more, no PD incepts and the insulation performance is
For the interpretation of the voltage rising rate, PD has been
intact under 25 kV for 30 min. The applied voltage is much
generated at different rising rates before breakdown, which can
higher than that of formal experiments. Therefore, it can be
provide enough initial electrons for the breakdown of the whole
concluded that within the range of experimental voltage, PVC
insulation. The breakdown delay of the whole insulation does
film has no effect on the results and PD only occurs in the bubble
not consider the initial electron generation time delay, and the
defects.
breakdown delay decreases, which can reduce the difference of
Then in the formal experiment, the geometric parameters of
breakdown voltage under different rising rates. Therefore, the
bubbles and voltage rising rate in the experiment are changed.
rising rate has little effect on the breakdown electric field.
Under bubble height of 0.5 mm, electrode distance of 2 mm and
Based on the influence of area and height on the breakdown,
volage rising rate of 0.5 kV/2 min, the variation of breakdown
it can be found that the breakdown of oil-paper insulation is
voltage (BV) and partial discharge inception voltage (PDIV)
induced by PD in the bubble in the process of voltage rise. The
with different bubble area is obtained. Then, in order to obtain
larger the area and the higher the height, the easier the PD is to
the short-time breakdown characteristics of oil-paper insulation
induce the breakdown of the overall insulation at a lower voltage
under the influence of bubble height, the variation curve of oil-
and the harm of PD to the insulation is more significant.
paper insulation breakdown electric field (BE) is obtained by
changing the bubble height under the two voltage rising rates of
0.5 kV/10 s and 0.5 kV/2 min, keeping the area of 40 mm2 and the B. Positive Feedback Mechanism of Oil-paper Insulation
gap distance of 2 mm unchanged. where BE can be obtained by Failure.
multiplying the BV measured by experiments by the electric field 1) Basic Phenomenon of PD: Bubble defects in transformers
non-uniformity coefficient calculated by COMSOL simulation. may withstand constant voltage for a long time. Under constant
The experimental results are shown in Fig. 3. voltage, the process of bubble PD is accompanied by the change
Results show that in the experimental area range, the break- of energy. The main characterization parameters for PD are
down voltage of the bubble decreases sharply with the increase discharge per second (Q) and discharge repetition rate per second

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ZHOU et al.: STUDY ON FAILURE MECHANISM OF OIL PAPER INSULATION UNDER PARTIAL DISCHARGE OF INTERLAYER BUBBLE 269

Fig. 6. Evolution of bubble area: decreases first due to oxygen consumption,


Fig. 4. Evolution of discharge Q and repetition rate N under constant voltage. and then increases due to PD gas production.

The results show that there has large Q in the reverse phase of
the voltage at initial stage, while the Q in other phase is basically
stable, forming the form shown in Fig. 5(a). During the transition
stage, the Q gradually increases and the number of PD with low
Q value is reduced, as shown in Fig. 5(b). Fig. 5(c) shows that
when PD just entered the stable period, the Q decreased and the
N increased sharply. The PD becomes dense in low discharge
area. Fig. 5(d) shows the PRPD pattern after entering the stable
period for a period of time. A high-density band of PD appears
in the middle of the PRPD pattern. Then the shape of PRPD
pattern will not change until the insulation breakdown.
Subsequent studies will mainly focus on the long-term cu-
mulative degradation effect of insulating paper when PD is
Fig. 5. Evolution of PRPD pattern. (a) initial stage. (b) transition stage.
in stable stage, to obtain the mechanism of insulation failure
(c) beginning of stable stage. (d) later stage of stable stage. caused by long-term bubble PD. In the experiment, keeping the
bubble height unchanged, the bubble area can change with gas
consumption or generation under bubble PD. The bubble area is
(N). The Q is the average value of apparent charge per unit time, used to characterize the degree of defect deterioration, and the
and the N is the number of PDs per unit time. Combined with discharge Q is used to characterize the severity of PD. Combined
the literature and the experimental research in this paper, it is with bubble area and Q, a positive feedback mechanism of the
found that the development process of bubble PD can be divided interaction between defect deterioration and PD intensification
into three stages: initial stage, transition stage and stable stage under long-term PD can be obtained.
[20], [21], [22]. Typical evolution of PD characteristic in the 2) Gas Production Rate: During the evolution of PD in stable
experiment is shown in Fig. 4. stage, a common phenomenon has been found, which is that a
Results show that Q increases gradually at first, drops sud- large amount of gas is generated in the process of bubble PD,
denly after several minutes, and then increases slowly with time and the gas accumulates between the oil-paper insulation layers,
after entering the stable discharge stage. The N tends to a large affecting the bubble area. This may be one of the reasons for the
value in the initial stage and gradually decreases in the transition intensification of PD. In the experiments, the height of bubble
stage. After a few minutes of transition, it rises suddenly and is 0.2 mm, the gap distance is 2 mm, and the applied voltage
finally rises steadily. In a word, the Q and N changed suddenly is 9 kV. The bubble area is recorded at regular intervals in the
in different stages, and the repeated experiments showed the experiment. Fig. 6 shows the change curve of bubble area.
same trend. Results show that the area of bubbles decreases at first. This
PRPD pattern is also a critical method containing lots of can be explained as follows: the gas used in the experiment is
characteristic information of PD. Corresponding to the four air, and the proportion of bubble area decrease is 22.45%, which
positions: (a), (b), (c) and (d) in Fig. 4, take 1 min PD data to build is exactly the proportion of oxygen in air. Therefore, the reason
PRPD pattern. The results are shown in Fig. 5. Where the vertical of bubble area decrease is that when PD transits from the initial
axis represents the discharge Q, the horizontal axis represents stage to stable stage, oxygen will be consumed continuously,
the voltage phase, and the legend represents the density of and the oxygen consumption rate is greater than gas generation
discharges. rate, causing the bubble area decreasing continuously [17].

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270 IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, VOL. 59, NO. 1, JANUARY/FEBRUARY 2023

Fig. 8. Verification of linear relationship between bubble area and discharge


Q. (a) discharge. (b) relationship.

area. Therefore, it can be considered that the increase of Q is


closely related to the change of bubble area.
Fig. 7. Variation of PD apparent charge Q with time.
In order to verify the linear relationship between bubble area
and discharge Q, further experiments are carried out in this
paper. Three typical bubble areas, 20 mm2 , 40 mm2 and 70
After all oxygen is consumed, the experimental result shows mm2 respectively, are selected to carry out the constant voltage
that the increase of area conforms to the exponential curve. long-term PD experiment under the voltage of 7 kV. The results
The abscissa of the experimental point is substituted into of the change of Q with time are shown in Fig. 8(a). Select four
the fitting curve to obtain the corresponding fitting value and time points in the initial stage and stable stage of PD process,
the Pearson correlation coefficient between the fitting value and including 2 min, 45 min, 90 min and 135 min, and calculate the
the experimental value is 0.9969. Compared with the correlation average value of 200 data points nearby as the value of Q at that
coefficient of linear fitting of 0.9888, it can be concluded that time. The results are plotted in Fig. 8(b) and fitted linearly.
exponential fitting is the best fitting method. Equation (1) is The results further prove that the linear relationship between
obtained by exponential fitting curve. Q and bubble area is significant. The correlation coefficient
between them is 0.9934 in the initial stage and 0.8990 in the
A = 65.66e0.00702t (1) stable stage. Therefore, it can be concluded that the apparent
charge Q of PD in interlayer bubble has a linear relationship with
where t is the time, in minutes, A is the area, in mm2 . The gas
the bubble area, which means that the bubble area determines
production rate is positively correlated with the area of existing
the severity of PD.
gas. And the coefficient of t indicates that 7.02 μL of gas will
The above studies have shown the positive feedback interac-
be produced per milliliter of gas in one minute.
tion between gas area and PD. Bubble PD will continuously
3) Positive Feedback Mechanism: Combined with the evolu-
produce gas and increase the bubble area, and the increase
tion process of bubble PD, this paper mainly studies the change
of bubble area will further promote the development of PD.
process of PD parameters in the stable stage, and takes the Q
The mathematical model of positive feedback mechanism is as
as the main research object. The discharge Q represents the
follows. In the model, it is assumed that the growth rate of bubble
energy released by each PD, and its increase can fully reflect
area is directly proportional to the area, and the proportional
the continuous deterioration of insulation. In a large number of
coefficient is set to k. The differential equation shown in (4) can
experiments, it is found that under the condition of long-term
be obtained. The variation function of area with time shown in
constant voltage, the apparent charge of PD will continue to rise
(5) can be obtained by solving the differential equation, where
with time, and presents an upward trend similar to exponent,
c is the undetermined coefficient. From the linear relationship
which is the same as the change trend of bubble area. The
between discharge Q and area, the function of Q with time can
discharge corresponding to the area change in Fig. 6 is fitted
be obtained, where C is the product of the linear coefficient of
exponentially and the results are shown in Fig. 7 and (2).
Q and area and the coefficient of (5). Finally, the insulation de-
Q = 0.177e0.00652t (2) terioration mode characterized by discharge Q can be expressed
as (6).
±Q = πε0 b2 [1 + εr (K (a/b) − 1)] ΔE (3)
dA
where Q is the apparent charge, in nC, t is the time, in min. = kA (4)
dt
The b represents the bubble diameter, a is the height, K(a/b) is
a constant related to a and b. A = cekt
By comparing (1) and (2), it can be seen that both are in Q = Cekt (5)
good agreement with the exponential fitting trend, and their
exponential coefficients are very close, less than 7.13%. And The established model indicates the deterioration of insulation
the calculation formula of charge is given in the literature [24], through the increase of Q. The change trend of the function is
as shown in (3). The Q has a linear relationship with the bubble consistent with the experimental results, which indicates that

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ZHOU et al.: STUDY ON FAILURE MECHANISM OF OIL PAPER INSULATION UNDER PARTIAL DISCHARGE OF INTERLAYER BUBBLE 271

Fig. 9. SEM image of non-damaged paper.

Fig. 10. SEM image of induced breakdown paper: breakdown point.

the model is correct, that is, the gas production rate of PD is


positively correlated with the bubble area. Therefore, it can be
seen that as long as bubbles appear in the oil-paper insulation,
the internal PD will continue to intensify exponentially, and the
insulation will eventually fail through the mechanism of positive
feedback.

C. Microscopic Study on the Effect of Partial Discharge on Oil


Paper Insulation
1) SEM Analysis: Cellulose is the main component of insu-
lating paper and will be modified under the effect of electric, Fig. 11. SEM images of paper surface under PD effect: four stages.
heat and other stress, which will seriously reduce the insulation
capacity. The macroscopic characteristics of oil paper insula-
tion failure have been studied in previous sections. Next, the failure of the insulating paper when the insulation performance
damage of bubble PD to insulating paper is analyzed from the is not degraded much, which is consistent with Section A.
microscopic point of view, in order to obtain the mechanism of While the PD effects on the insulating paper for a long
insulation failure. time without breakdown, the insulating paper will deteriorate
First, the surface of insulating paper without PD is observed, continuously in the long-term discharge. According to the dam-
and the images with magnification of 200 times and 5000 times age degree of insulating paper, the continuous deterioration of
are obtained, as shown in Fig. 9. It can be seen that without the insulating paper can be divided into four stages as shown in
effect of PD, the surface of insulating paper is relatively flat, the Fig. 11.
fibers are dense and the structure of the whole fiber is compact Fig. 11 shows the typical surface morphology of insulating
without defects. And there are lots of fiber filaments on the paper in four damage stages under different magnification.
surface of fiber that can be observed at the large magnification. Fig. 11(a) to Fig. 11(c) include SEM images magnified by 1000
As shown in Fig. 10, for the insulating paper after bubble PD times and 5000 times respectively and Fig. 11(d) shows images
induced breakdown, the surface structure of the insulating paper magnified by 200 times and 1000 times respectively. In the
was observed at 100 times and 2500 times magnification. It can first stage of Fig. 11(a), the fine fibers in the insulating paper
be seen that the main fiber is completely broken, and there is a have disappeared, leaving only the coarser fiber, and the surface
breakdown hole in the middle, with a diameter of about hundreds of the coarser fiber has become flatter, which shows that the
of microns, while the surrounding insulating paper basically energy of PD is low and only destroys fine fibers at first. The
undamaged. This further proves that the induced breakdown may main sign of the second stage is surface roughing as shown in
be caused by the streamer discharge in the oil gap, resulting in the Fig. 11(b). the surface of the insulating paper and the thicker

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272 IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, VOL. 59, NO. 1, JANUARY/FEBRUARY 2023

Fig. 12. Proportion of elements on the surface of insulating paper.

TABLE I
ELEMENT PROPORTION
Fig. 13. Element line distribution image: (a) undamaged paper. (b) paper under
PD effect.

connecting fibers began to crystallize and the main fibers and


the thicker connecting fibers between the main fibers appeared
spherical protrusions as shown in the yellow coil, which means
that the long-term cumulative damage effect of PD begins to
appear. In Fig. 11(c) for the third stage, the surface of the
insulating fiber is further roughened. The coarser fibers have also
broken and the fracture is spherical crystal. The fiber damage
of insulating paper is further aggravated In Fig. 11(d) for the
fourth stage, the surface of insulating paper began to become flat
with the intensification of crystallization, the pores and the fiber
structure have basically disappeared. And the crack channels
have appeared on the surface of insulating paper.
2) EDS Analysis: In order to further analyze the causes and Fig. 14. Element plane distribution image: (a) undamaged insulating paper.
(b) paper under PD effect. where different colored points represent different
components of crystallization and study the physical and chem- elements and distributions.
ical changes on the surface of insulating paper, the distribution
of elements on the surface of insulating paper were studied by
energy spectrum analysis. The line distribution of element on Result in Fig. 13 shows that the distribution of carbon and
the surface of insulating paper is shown in Fig. 12 and Table Ⅰ oxygen on both undamaged and damaged paper is uniform.
shows the proportion of carbon and oxygen. Comparing the element content and distribution of insulating
The peaks in the Fig. 12 show the contents of carbon and paper before and after PD, it can be concluded that the insulating
oxygen respectively. Platinum is an impurity element introduced paper is carbonized continuously with the development of PD.
due to the need for gold spraying during observation, which can The insulation capacity of carbonized insulating paper decreases
be ignored. According to the results in Fig. 12 and Table I, it seriously due to the looseness of the structure and the reduction
shows that under the effect of PD for a long time, the proportion of strength, which can lead to breakdown of oil paper insulation.
of carbon and oxygen in insulating paper has changed greatly: Finally, the surface distribution of carbon and oxygen ele-
the proportion of carbon has increased by 11.53%, while the ments on the surface of insulating paper before and after damage
proportion of oxygen has decreased by about 11.53%. is further analyzed by EDS analysis. The results are shown in Fig
Ten different positions of the damaged paper are randomly 14, in which Fig. 14(a) shows the sampling area and distribution
selected for EDS analysis in line to obtain surface elements results of carbon and oxygen on undamaged insulating paper,
distribution of insulating paper under effect of bubble PD and and Fig. 14(b) shows the corresponding results of damaged
Fig. 13 is representative. Fig. 13(a) represents undamaged paper insulating paper. From the element plane distribution, it can be
while Fig. 13(b) is the damaged. seen that the surface elements of insulating paper before and

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ZHOU et al.: STUDY ON FAILURE MECHANISM OF OIL PAPER INSULATION UNDER PARTIAL DISCHARGE OF INTERLAYER BUBBLE 273

Fig. 16. Cumulative damage process of insulating paper.

damaged. Therefore, the first stage of insulating paper dam-


age is that the fiber filaments scattered in insulating paper are
Fig. 15. Induced breakdown process. ablated and disappeared. With the increase of time, the elec-
trons produced by PD begin to destroy the internal structure of
cellulose, making most sugar ring begin to break. Therefore,
after damage of PD are also evenly distributed, which further the fiber surface in insulating paper began to be damaged and
strengthens the conclusion that PD in bubble causes uniform roughened, which can be considered as the second stage. In third
damage to the surface of insulating paper. stage, the damage of insulation paper caused by PD reaches
a certain degree, destroyed the polymer structure of cellulose.
Therefore, crystalline substances begin to appear on the surface
IV. DISCUSSION of insulating paper. And the thicker connecting fibers will break
Above all, the short-time breakdown characteristics and pos- and form crystalline fracture. Finally, based on the destruction
itive feedback mechanism of oil paper insulation are studied, of polymer structure, PD will consume oxygen element faster,
the surface morphology and element content distribution of resulting in the continuous appearance of carbonized crystals
insulating paper under long-time PD is analyzed, and the basic on the surface of insulating paper. As a result, the surface of the
process and principle of insulating paper damage and breakdown insulating paper is completely covered with fine crystals, and
under micro are obtained. According to the above results, two the whole surface is carbonized and loose. In this process, the
physical mechanisms of oil paper insulation breakdown are insulation capacity of insulating paper continues to decline.
proposed in this paper. In conclusion, the electrons generated by PD will interact
First, bubble PD can induce the breakdown of the whole oil with insulating paper, destroy the chemical bond of cellulose
paper insulation gap. As shown in Fig. 15, the PD of bubble and consume oxygen element, resulting in the carbonization of
can accumulate charges on the surface of insulating paper [13]. insulating paper and eventually lead to insulation failure.
These accumulated charges are easy to become the initial elec-
trons causing gap breakdown, and the space electric field formed
V. CONCLUSION
by the accumulated charges enhances the electric field in the
oil gap, making the gap more likely to break through under the In this paper, the characteristics of insulation short-time
effect. When the charge accumulates to a certain extent, the weak breakdown under the influence of height and area are studied.
part in the oil gap may develop into streamer discharge, resulting Then, the relationship between gas production and development
in the breakdown of the whole gap. Generally, the induced of PD is analyzed, and the positive feedback failure mechanism
breakdown probability increases with the increase of bubble of insulation under long-time PD is obtained. Finally, the micro
defects, which is the reason for the formation of short-time morphology, element content and distribution of insulating pa-
breakdown characteristics of oil paper insulation. per under different damage states are analyzed, and the micro
Second, bubble PD accumulated damage to insulating pa- mechanism of insulation failure is studied. The summary is as
per and cause breakdown [22]. From the positive feedback follows:
mechanism, the cumulative damage will be faster and faster. 1) The short-time breakdown voltage of insulation decreases
Fig. 16 shows the whole damage process of insulating paper. significantly with the deterioration of bubble defects and
The PD electrons bombard the surface of the insulating paper gradually approaches the inception voltage of PD.
continuously at first. Due to the dense structure of insulating 2) The gas production rate of PD is directly proportional to
paper, only the exposed hydroxyl and methyl groups on the the bubble size. The increase of bubble will aggravate the
insulating paper surface will be damaged. And for some fine PD. The positive feedback between them makes the PD
fibers in voids, the ether bond on the sugar ring may also be develop exponentially, resulting in rapid insulation failure.

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274 IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, VOL. 59, NO. 1, JANUARY/FEBRUARY 2023

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ZHOU et al.: STUDY ON FAILURE MECHANISM OF OIL PAPER INSULATION UNDER PARTIAL DISCHARGE OF INTERLAYER BUBBLE 275

Zhicheng Wu was born in China. He received the Chong Guo was born in China, in 1992. He received
Ph.D. degree from Xi’an Jiaotong University, Xi’an, the B.S. and M.S. degrees in electrical engineering
China, in 2020. He is currently an Assistant Professor from the Harbin University of Science and Technol-
with Xi’an Jiaotong University. He mainly engaged ogy, Harbin, China, in 2015 and 2018, respectively.
in research on improvement of insulation reliability He is currently working toward the Ph.D. degree
of GIS/GIL equipment, preparation, and development with Xi’an Jiaotong University, Xi’an, China. His
of electrical epoxy materials. main research focuses on measurement and oil-paper
insulation of transformers.

Tao Wen was born in Shaanxi, China, in 1990. He


received the B.S. and Ph.D. degrees in electrical
engineering from Xi’an Jiaotong University, Xi’an,
China, in 2012 and 2017, respectively. His main re-
search interests include pulse power technology, gas
discharge, and its applications.

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