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Published_Shcherbanev
Conference Paper
Author(s):
Shcherbanev, Sergey; Dharmaputra, Bayu; Solana Pérez, Roberto ; Noiray, Nicolas
Publication date:
2022-01
Permanent link:
https://doi.org/10.3929/ethz-b-000527565
Rights / license:
In Copyright - Non-Commercial Use Permitted
Funding acknowledgement:
820091 - ThermoacOustic instabilities contRol in sequential Combustion cHambers (EC)
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AIAA SciTech Forum 10.2514/6.2022-2254
January 3-7, 2022, San Diego, CA & Virtual
AIAA SCITECH 2022 Forum
This paper describes the experimental results of the flame dynamics stabilized by nanosec-
ond repetitively pulsed discharge (NRPD) in a sequential combustor configuration. In such
configuration of the combustor, two flame regions are organized sequentially: (i) first stage
flame and (ii) second-stage sequential flame placed downstream of the first one. The sequential
flame is located downstream of the injection of the dilution air and the second stage fuel into the
hot vitiated products of the first stage flame. Several operation conditions of the second stage
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
flame were considered in the present paper. The parameters of the first stage flame and amount
of the dilution air were fixed while the second stage fuel injection was composed of natural
gas/H2 mixture with different fractions of hydrogen. It is shown that the flame anchoring and
combustion dynamics is significantly affected by the amount of hydrogen and mean power of the
NRPD. Thermal effect of the plasma was studied with optical emission spectroscopy. Namely,
the temperature increase due to the fast gas heating was measured during applied high-voltage
pulses. It was shown that, for a mean vitiated flow temperature of 1000K, the temperature
increase due to nanosecond pulse discharge can reach up to 2100K. The coupling of the gas
flow with NRPD was identified for different frequencies and amplitudes of applied pulses. It
was found that for high pulse repetition frequency (PRF>40 kHz) the discharge propagation
and the parameter of the plasma have a cumulative effect. Spatially resolved electron density
and mean gas temperature in the plasma region were measured in order to characterize the
flow-discharge coupling in the flow direction. High speed OH∗ chemiluminescence is used for
quantitative analysis of the ignition and stabilization of the second stage flame.
I. Introduction
sequential combustor architecture is a key concept for the improvement of ground based heavy-duty gas turbines
S efficiency [1, 2]. This concept is attractive because it allows increasing operational and fuel flexibility at lower
emissions and higher combined cycle efficiency. This architecture of the combustion chamber is associated with a
substantially increased system complexity in terms of: (i) operating concept; (ii) 1st and 2nd stage flames are acoustically
coupled with each others; (iii) of combustion dynamics related to ignition, anchoring and blow-off physics. In such
sequential combustors, dilution air/fuel are injected downstream of the first stage lean premixed flame. The resulting
temperature in the mixing section of the sequential burner is low enough to allo high quality mixing before spontaneous
ignition, and therefore allows for ultra low NOx emissions, which is a case in this concept [3].
Sequential combustion chambers are thus of particular interest for clean combustion of sustainable fuels in gas
turbine applications. However, changes of fuel reactivity through variations of H2 fraction, can perturb the sequential
flame anchoring and dynamics. One of the possible ways to stabilize this sequential flame is to initiate a non-equilibrium
discharge in the mixing section where the vitiated flow from the first stage and dilution air are mixed with the second
stage fuel. It is known fact that NRPD is an efficient tool for the enhancement of the lean stability and blow-off limits [4].
Initiation of non-equilibrium plasma can serve as an additional flame holder that may prevent unwanted combustion
dynamics and strengthen the flame anchoring while changing the operation conditions.
This study is oriented on characterization of the discharge properties in the vitiated hot environment in a generic
sequential burner. The NRPD was initiated in pin-to-pin configuration in the mixing channel of the generic sequential
combustor. Two regimes of the discharge were identified: glow and spark. Electron number density and gas temperature
are measured for different discharge power. The effect of plasma initiation on flame ignition and anchoring on the
second stage of sequential combustor is studied. It is shown that the coupling between the flow and the plasma is
significantly affects the ignition dynamics of the sequential flame.
Copyright © 2022 by Sergey Shcherbanev, Nicolas Noiray. Published by the American Institute of Aeronautics and Astronautics, Inc., with permission.
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
Fig. 1 Axially staged combustor consisting of a lean premixed first stage with a 4×4 array of turbulent flames
and a secondary jet flame in vitiated cross flow. The combustor has a constant cross section and is composed of
several modules equipped with quartz windows.
Table 1 Operational conditions of the sequential combustor. First stage conditions are NG1 =0.7 g/s, air1 =15 g/s.
Dilution air was fixed to 18 g/s for all OPs.
For direct discharge visualization the Pi-Max4 ICCD camera is used. The camera is equipped with 337 nm narrow
band filter in order to capture the morphology of the N∗2 . Optical emission spectroscopy techniques is used for the
analysis of the heat release in the discharge region. The temperature is measured from the emission spectra of the second
positive system of molecular nitrogen. The electron density was measured with the Stark broadening of the H 𝛼 line. For
spatially resolved measurements of the discharge temperature and electron density the discharge region was projected to
2
the entrance slit of the PI IsoPlane-320 spectrometer equipped with Pi-Max4 camera (are not shown in the figure).
The effect of the discharge initiation on the combustion of the second stage flame was characterized for different
operational points (OP). All considered experimental conditions are listed in a test matrix presented in table 1. The
parameters of the first stage flame as well as the amount of dilution air were fixed for all OPs. The equivalence ratio of
the first stage flame is set to 0.8 by injecting 0.7 g/s of the natural gas and 15 g/s of the air. These parameters result to
the 35 kW of thermal power of the first stage flame. The thermal power of the second stage flame was nearly equal to
37 kW for all OPs. Mixtures of natural gas/hydrogen with different fractions of hydrogen is used as fuel on the second
stage of the combustor.
discharges the conditions with low fraction of hydrogen were selected. The second stage flame without initiation
of NRPD was not igniting for operation points OP1 and OP2 shown in table 1. For other conditions the flame was
autoignited. With increase of the hydrogen fraction in the fuel mixture the flame becomes more stable and shifts toward
the wake of the combustion chamber. A backward facing step configuration (from 25x38mm2 to 62x62mm2 ), enables
strong anchoring of the sequential flame due to strong recirculation regions. In order to shift the flame downstream of
the combustion chamber a temperature and equivalence ratio of the gas mixture on the second stage, 18 g/s of dilution
air were injected that resulted in mean flow temperature about 950 K and equivalence ratio 0.57-0.6.
Figure 2 shows the high speed chemiluminescence images of the flame while initiation of the NRPD. The relative
position of the electrode system, fuel injector are shown the combustion chamber is shown in the figure. First column
demonstrated the dynamics of the ignition kernels and the initiation of the flame for the OP2 conditions. It can be seen
that there is no flame in the combustion chamber when the NRPD is turned off. While the discharge is switched on the
first distinct ignition kernels take place in the combustion chamber that further expand and the well developed flame is
stabilized in the downstream part of the chamber. The discharge was initiated during 0.1 s at 50 kHz pulse repetition
frequency (PRF) and 13.5 kV of applied voltage.
The second column in figure 2 corresponds to the OP5 conditions. Even without plasma the flame is autoignited and
stabilized in the combustion chamber. The flame has asymmetrical structure. This can be caused by a non-symmetric
injector geometry. In the case where the discharge is switched off, the flame is distributed along the entire length of the
combustion chamber. During the discharge initiation the distinct spontaneous ignition kernels can be partially observed
at the outlet of the mixing channel. These kernels propagate downstream, merge with the flame and stabilize the flame
on both (upper and lower) parts of the combustion chamber wake. The flame becomes anchored and more symmetrical
with respect to the axis of the combustor. The overall length of the flame is reduced and for a particular case of OP5
occupies only a half of the volume of the combustion chamber.
On the averaged OH∗ chemiluminescence the mean flame profiles can be seen. For the OP2 the flame was initiated
and stabilized with NRPD. Once the discharge is turned off some remaining flame can be still observed in the chamber
during the following 0.02-0.05 s. At later time the flame is blown out. For the OP5 the flame profile has rather symmetric
structure and well anchored to the outlet of the mixing channel. When the plasma is off the flame is detached and
stabilized downstream of the chamber wake.
The time averaged profiles of the OH∗ can be seen in figure 3 for all OPs and fixed parameters of the applied HV
pulses: 𝑉 = 19.5 kHz and 𝑃𝑅𝐹 = 50 kHz. For the lowest hydrogen content in the fuel mixture (OP1), the unstable
pulsed ignition with plasma was observed. The ignition take place well downstream near the outlet of the combustion
chamber. Ignition kernels were instantly extinguished once the plasma discharge is turned off. For the voltage amplitudes
lower than 16 kV any ignition events was observed for the OP1. For the OP2 the similar behaviour to the one explained
above can be observed with the only difference that the flame is shifted upstream because the higher amplitude of the
applied voltage. For the case of OP3 the ignition kernels in the mixing channel can be observed more regularly because
of higher reactivity of the mixture.
For even higher amount of hydrogen in the gas mixture (OP4 and OP5) the flame without plasma is anchored from
the one side of the combustion chamber inlet. However, once the NRPD is on, the ignition takes place in the vicinity
of the electrode system and well developed flame can be observed at the outlet of the mixing channel. It should be
mentioned that the flame in the mixing channel is initiated from the side of the cathode electrode. The energy density in
3
Instantaneous OH chemiluminescence
100 Mixing channel Combustion chamber
X, (mm)
Injector Electrodes
50
t=1.5 ms t=1.9 ms
0
100
X, (mm)
50
t=2.1 ms t=2.7 ms
0
100
X, (mm)
50
t=2.4 ms t=2.9 ms
0
100
X, (mm)
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
50
t=2.7 ms t=3.2 ms
0
100
X, (mm)
50
t=3.3 ms t=3.7 ms
0
100
(mm)
X, (mm)
50
X,
0
t=3.9 ms t=4.1 ms
100
X, (mm)
50
t=4.5 ms t=4.8 ms
0
Z, (mm) Z, (mm)
Averaged OH chemiluminescence
Plasma ON Plasma ON
X, (mm)
Z, (mm) Z, (mm)
Fig. 2 Time-resolved OH∗ chemiluminescence images for OP2 (left column) and OP5 (right column). Discharge
parameters: PRF=50 kHz, V=13.5 kV.
the cathode region is higher than that near the anode, the further spectroscopy analysis confirmed that issue.
4
Mixing channel Combustion chamber
OP 1 Electrodes OP 2 OP 3
OP 4 OP 5
Fig. 3 Time averaged images of the OH∗ chemiluminescence. OP - stands for operational point listed in the
table. Applied voltage V=19.5 kV, PRF = 50 kHz.
Fig. 4 Dynamic of gas (left) and vibrational (right) temperature during the discharge for different applied
voltages.
within collisional quenching of N∗2 with O2 molecules leading to the dissociation of the latter and energy release as high
as several electronvolts.
This mechanism of fast gas heating is well studied in air [7]. The kinetic mechanism of the fast gas heating in more
complex gas mixtures is not known nowadays. The energy balance and transfer between different degrees of freedom
might be significantly complicated by the presence of 3- or higher atomic molecules.
Here we present the temperature dynamics in the discharge region for the plasma initiated in vitiated hot flow gas.
For further analysis the discharge was initiated at atmospheric pressure for a OP5 conditions. Figure 4 shows the
dynamics of the gas and vibrational temperature measured from the optical emission of N2 (C-B)(Δ𝜈 = 1) transition
of second positive system. The presented temperature curves are shown together with the profile of the applied HV
pulse. The emission spectra are acquired with the system described in Experimental setup section. Camera gate for the
acquisition of the optical emission spectra was set to 2 ns with 100 on-CCD accumulations. Experimental emission
spectra were fitted with the SpecAir [8] software in order to obtain rotational and vibrational temperatures in the plasma
region. Temperatures were measured for 4 different amplitudes of applied voltages: 10.5, 12.0, 22.5 and 27.5 kV. As
one can see in the left plot of figure 4, there is practically no temperature increase for 10.5 kV case. With increase of
amplitude of applied voltage heat release rate gradually increases. For 27.0 kV amplitude the temperature is increased
5
0.01
a) b)
1E-4
10 12 14 16 18 20 22 24 26 28
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
Applied voltage, kV
Fig. 5 a) Signal from back current shunt; b) deposited energy per pulse for different applied voltages.
from 1000 K to 2200 K during 14 ns which is equivalent to the increase rate of 85 K/ns. This value of the gas heating
rate exceeds the values given in the literature for measuring the temperature dynamics in the air.
Figure 4 also shows the dynamic of vibrational temperatures during the applied HV pulse. It can be clearly seen that
the vibrational temperature values start at about 4000 K and then decreases during 6-8 ns for all voltages. For the lowest
voltage, this trend continues until the end of the applied pulse. However, with increase of voltage amplitude the value
of vibrational temperature has an infimum. After this value the vibrational temperature starts increasing. The point
of minimal vibrational temperature is shifted towards the leading edge of the pulse with increase of the amplitude of
applied voltage.
6
1E16
1E14
10 12 14 16 18 20 22 24
Applied voltage, kV
7
+ HV electrode
Slit
orientation
Flow
- HV electrode a)
Slit orientation
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
Gap axis
b) d)
0.8 0.5
0.6 0.0
0.4
0.2
c) e)
0.0
Fig. 7 Space resolved measurements of the electron density and gas temperature in the plasma region in the
middle of the inter-electrode gap. (a) and (c) spatially resolved emission spectra of the H 𝛼 line and second
positive system of N2 respectively; (b) H 𝛼 line profile for different distances from the electrode axis; (d) Spatially
resolved gas temperature, electron density and ionization degree. Operational conditions: 100 kHz, V=19.5 kV,
OP5
temperature value T and atmospheric pressure as 𝑛𝑔𝑎𝑠 = 𝑁 𝐿 · (𝑇0 /𝑇), where 𝑁 𝐿 = 2.68678 · 1019 cm−3 - is Loschmidt
constant. The ionization degree gives information about the specific energy deposition. As can be seen, the highest
specific energy is correlated with the highest electron number density region.
According to the above-mentioned descriptions, 3 regions of the plasma-flow coupling can be distinguished:
• Pre-heating region, where the energy is progressively delivered and increased from pulse to pulse. In this region,
the discharge heats up the gas by several hundred degrees producing active species and metastable states. They
are convected further downstream allowing initiation of the discharge with higher ionization degree.
• The region with the highest efficiency of the energy transfer.
• Thermal maintenance region, where the balance of energy is established between the gas heating by subsequent
8
pulses and heat transfer to the surrounding flow.
IV. Conclusion
An experimental study was carried out to investigate the effects of nanosecond repetitively pulsed discharge (NRPD)
on the stabilization of the flame in a generic sequential combustor. By means of fast OH∗ chemiluminescence imaging, it
was shown that the effect of NRPD on the flame anchoring is significantly depend on the composition and the reactivity
of the gas mixture. The bursting ignition events can be observed for NRPD initiation at a low fraction of hydrogen
(OP1), but the flame was not stabilized in the combustion chamber. For a moderate amount of hydrogen (OP2), the
ignition efficiency is significantly affected by the mean power of the NRPD, which can be controlled either by voltage
or by PRF of applied pulses. For a higher content of the hydrogen in second stage fuel mixtures (OP3-5), the flame
was auto-ignited without plasma. However, the NRPD showed a significant effect on flame anchoring and stabilisation
of flickering flames on the second stage of the sequential combustor by both glow and spark NRPD regimes. The
temperature dynamics during a single pulse was measured for different deposited energies. It was shown that the fast gas
heating leads to a significant temperature increase rate of up to 85 K/ns. The analysis of the energy deposition and the
Downloaded by Sergey Shcherbanev on December 31, 2021 | http://arc.aiaa.org | DOI: 10.2514/6.2022-2254
electron density as a function of the amplitude of applied voltage demonstrated the presence of two regimes of discharge:
glow and spark. In a glow regime, no significant gas heating was observed, and the electron density did not exceed
5·1014 cm−3 at 10.5 kV. Whereas, for a spark regime, the single event of the discharge leads to the rapid heat release and
the electron number densities 1-2 orders of magnitude higher than that in the glow regime. Spatially resolved emission
spectroscopy measurements were carried out for electron number density and temperature profiles along the gas flow
direction to characterize the coupling between the plasma and hot flow. It was shown that for considered operation
points, the NRPD with pulse repetition frequencies 𝑃𝑅𝐹 ≤ 40 kHz is not coupled with the flow for the peak amplitudes
of applied voltage 𝑉 ≤ 27 kV. For spark NRPD with 𝑃𝑅𝐹 ≤ 40 kHz, the plasma parameters are significantly affected by
the preceding applied pulses and have a cumulative character of plasma properties.
Acknowledgments
This study was supported by the European Research Council under the ERC Consolidator Grant (No: 820091) TORCH
(2019-2024).
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