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fits the experimental data over a wide range of shear rate and coil
electric current intensity values. A main advantage of our model is
that it can be used in regular CFD codes to compute the MRF flow in
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Page 1 of 21 Journal of Intelligent Material Systems and Structures
21 intensity. It is shown that our model accurately fits the experimental data over a wide
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range of shear rate and coil electric current intensity values. A main advantage of our
24 model is that it can be used in regular CFD codes to compute the MRF flow in
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33 INTRODUCTION
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35 Magnetorheological fluids (MRF) are suspensions of particles which can be
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37 magnetized, and exhibit fast, strong and reversible changes in their rheological
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38 properties when a magnetic field is applied. Goncalves, Koo and Ahmadian (2006)
39 review the state of the art in magnetorheological technology, and examine various
40 models used to describe the MR fluid behavior. Two models have been particularly
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well documented in the literature, namely the Bingham Plastic and the Herschel-
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Bulkley models. The focus of the present paper was to develop and validate a
44 rheological model able to capture both pre- and post-yield behavior of MRF, and in
45 the same time be easy to implement in commercially available CFD codes in order to
46 simulate the flow in practical devices.
47 Li, Chen and Yeo (1999) investigate the viscoelastic properties of MR
48 suspension within the pre-yield region, since these properties are considered
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50 especially relevant for vibration damping applications. They used a German Paar
51 Physica rheometer with plate-plate configuration in strain-controlled mode, and a
52 MRF-132LD suspension produced by Lord Corporation, both the equipment and MR
53 fluid being quite similar to the ones used in the present investigations. Both strain-
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amplitude sweep (frequency 10 Hz and amplitude 10 4 K10 3 ) and frequency sweep
56 (amplitude 10 3 and frequency from 1 Hz to 100 Hz) tests were performed in order to
57 determine the storage modulus and loss modulus as functions of oscillating frequency,
58 strain amplitude, applied coil current (which is proportional to the magnetic flux
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density) and volume fraction of iron powder dispersed in silicone oil. In a further
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E-mail: dana_resiga@yahoo.com
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Journal of Intelligent Material Systems and Structures Page 2 of 21
25 consistent with the Bingham model. They derived the yield shear stress and the
26 Bingham viscosity from the pressure drop versus the volumetric flow rate in a
27 capillary rheometer at high flow velocity, arguing that such high velocities are
28 relevant for new industrial applications such as shock and vibration dampers.
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Chadhuria et al. (2005) investigate the rheological flow curves (shear stress vs. shear
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31 rate) of a nanoparticle cobalt-based magnetorhelogical fluid, and found that either
32 Bingham-plastic or Herschel-Bulkley models can be used to describe the experimental
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33 data. Bitman, Choi and Wereley (2002) replace the Bingham model by an Eyring
34 constitutive model to investigate the behaviour of electrorhelogical dampers. Because
35 the two-parameter (yield stress and postyield viscosity) Bingham model has a zero
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37 shear rate discontinuity, it has been replaced by the Eyring model which has a smooth
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38 transition through the zero shear rate condition and also has two rheological constants
39 for a constant field (magnitude of the shear stress and steepness of the shear rate
40 gradient in the preyield region). This is a more convenient alternative to the biviscous
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model, which has two distinct viscosities and governing equations within the preyield
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(low shear rate) and postyield (high shear rate) regions. In a further study, Choi et al.
44 (2005) investigate the rheological characteristics of ER/MR fluids with respect to both
45 cylinder and parallel disk rotational viscosimeters, and derive the governing equations
46 based on Bingham-plastic, biviscous, and Herschel-Bulkley constitutive models. It
47 has been found that flow curves (shear stress versus shear rate) for the rotational
48 coaxial cylinder viscosimeter are sensitive to the calculation methods since two or
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50 three distinct flow conditions occur in the gap. However, in the case of rotational
51 parallel disk viscosimeter the flow curve can be obtained directly from fundamental
52 equations without any approximation strategies. This is the viscosimeter also used for
53 the experimental investigations presented in this paper.
54 In an attempt to model the yield behavior of magnetorheological suspensions,
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Bossis et al. (2003) propose a mechanism where, except in some special cases where
57 the forces between the particles and the wall can be larger than the interparticle
58 magnetic force, the aggregates slip on the walls when the stress is increased and begin
59 to rotate before breaking. As a result, we conclude that the a fluid model in the
60 preyield region, with a smooth transition to the shear-thinning behaviour for large
shear-rate values may be valuable for developing and evaluating practical applications
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example for steady laminar flow between parallel plates. The paper conclusions are
23 summarized in the last section.
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34 ( &) = N ( & ) W1 ( & ) + HB ( & ) W2 ( & ) (1)
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36 where the Newtonian behaviour is given by
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( &) =
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40 and the shear thinning behaviour is described by the Hershel-Bulkley model,
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21 ( &) = + y
&. (5)
22 &
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blending function
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x
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43 Figure 1. Blending functions.
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All the above functions vanish as x 0 and reach the asymptotic value of 1 for
46 x . However, one can control how fast the functions approach the asymptotic
47 value by stretching the abscissa with a parameter multiplying x . The role of this
48 parameter is played in our model by the characteristic shear rate & .
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50 For the present analysis we have chosen
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& &
52 W1 = 1 tanh and W2 = tanh , (6)
53 & &
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55 but similar results are obtained with the other choices mentioned above. As a result,
56 the mathematical model used for representing the mahneto-rheological behaviour of
57 the MRF-132DG samples reads as
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Figure 2. Flow curve fitted with various blending functions.
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The shear stress vanishes as & 0 , while the viscosity / & has the limit
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43 value for vanishing shear rate
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45 lim = 0 + 0
. (8)
46 & 0 &
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48 Equation (8) clearly reveals that the start-up viscosity incorporates both the
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contribution from the Newtonian behaviour, 0 , and the contribution from the yield
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51 stress of the Hershel-Bulkley model, 0 .
52 The shear stress reaches the characteristic value of
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(& )= 0
& × 0.2384 + ( 0 + 1 ) × 0.7616 (9)
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at the characteristic shear rate value, corresponding to the shift in the rheological
58 behaviour from quasi-Newtonian to shear-thinning.
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Journal of Intelligent Material Systems and Structures Page 6 of 21
21 performed amplitude sweep tests with angular frequency of 1s 1 and shear strain
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amplitude within the range A = 10 5 K10 . Since for amplitude sweep tests the shear
24 has a sinusoidal variation in time, the average shear rate value & ( 2 / $ ) % A is
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26 considered for the flow curve. The amplitude-sweep results are shown as hollow
27 circles in the figures below, as well as in Figure 2, while the regular flow curve data
28 are shown as filled squares. One can see that the results of the two tests for each
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current intensity value overlap very well, thus the whole set of points has been used to
30 find the parameters in Eq. (7). Although our model (7) has five parameters to be found
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32 by fitting the experimental data, four of them are relevant from practical point of
view: the threshold shear rate & and the corresponding shear stress , the start-up
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viscosity , and the shear-thinning exponent n . The latest was found to have
36 practically the same value, n = 0.855 ( ±3% ) for a wide range of electric current
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intensity in the magneto-rheological cell coil I = 0.1K 3 A , and it has been
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39 subsequently fixed to a value of n = 0.855 .
40 Figure 3 through Figure 10 show the flow curves (shear stress versus shear
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rate) and viscosity curves (dynamic viscosity versus shear rate) for variable intensity
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of the electric current in the magnetorheological cell coil. On the flow curve plots
44 both & and are marked with dashed lines, since these values correspond to a
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conventional quasi-yield point. In fact, the point (& , ) on the flow curve
47 conventionally marks the transition from a quasi-newtonian behavior for low shear
48 rate values to the shear thinning behavior for large shear rate. Note that this transition
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is smooth and continuous thanks to the blending functions used in (7), and the point
51 ( & , ) is only an indication of the behaviour change. On the viscosity curve plots
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53 both both & and are shown explicitly in order to emphasize the start-up viscosity
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level. For large current intensity, Figure 10, the point (& , ) on the flow curve
56 corresponds to a local maximum of the shear stress, supporting once more the
57 interpretation as a quasi-yield point. We conclude that our rheological model (7)
58 accurately fits the experimental data within a large range of shear rate
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60 & = 10 6 K103 s 1 , and it can be reliably used to further investigate various
engineering applications. Figure 11 presents a synoptic view of the magneto-
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Figure 3. Flow curve ( &) and viscosity curve ( &) for I = 0.1 A .
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( &) ( &)
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59 Figure 4. Flow curve and viscosity curve for I = 0.25 A .
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( &) ( &)
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59 Figure 5. Flow curve and viscosity curve for I = 0.5 A .
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( &) ( &)
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( &) ( &)
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( &) ( &)
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for viscous flow. The fit parameters are shown in Table 1, and the corresponding
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34 1.0 534 2.63 '103
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1.5 996 2.63 '103
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42 independent of the electric current intensity, leading to the conclusion that the
43 temperature influence can be included into Eq.(7) simply by multiplying the right-
44 hand term with an exponential factor:
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46 1 n
( & & & (
47 ( &, T ) = 0 & 1 tanh + 0 + 1 tanh
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( ! & " & & (
49 ! " T0 (11)
.
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Ea 1 1
51 × exp
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!R T T0 "
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54 where T0 is the absolute temperature at which the flow curves have been determined
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56 (e.g. room temperature). Our measurements shown in Figure 3…Figure 10 have been
57 made at 20o C ( T0 = 293 K ).
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The physical interpretation of this result is that the temperature influence on
60 the MRF viscosity, at least within the temperature range investigated in this paper
20o C K 60o C , is due to the changes in the carrier liquid viscosity. The magnetizable
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31 Figure 14. Temperature influence on the MRF viscosity for values of electric
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34 As far as the sedimentation of the MRF-132DG sample is concerned, we have
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performed both qualitative and quantitative tests. The qualitative analysis has been
37 performed on samples held in vertical glass tubes for 7 days, while for the quantitative
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38 assessment of the sedimentation properties we have used the frontal method based on
39 X-ray diffraction. The conclusion is that the MRF-132DG sample displays a very low
40 sedimentation velocity in comparison with other MRF samples produced and tested in
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our laboratory. Moreover, before each measurement a shaker was used to homogenize
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43 the sample.
44 The magneto-rheological model presented and validated in this paper is a
45 steady one. It does not incorporate the MRF response to the dynamics of the time-
46 dependent electric current variation, as investigated by Laun and Gabriel (2007) with
47 switching times of a few milliseconds. However, for preliminary design of magneto-
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rheological devices and analysis of their performance using regular CFD codes, our
50 model (11) offers a good starting point.
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52 NUMERICAL EXAMPLE
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We use the rheological model (7) to compute the steady laminar flow between two
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56 plane plates 2 mm apart. Because of the problem symmetry, we consider only half the
57 channel width. The shear stress decreases linearly from the maximum value at the
58 wall to zero at the middle of the channel, as shown in Figure 15. Inserting this shear
stress behaviour in (7) leads to a non-linear equation for & ( y ) , where y denotes the
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distance from the wall.
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mass flow rate 1.E−6 kg/s
22 3e+03
ma
3e−07
shear stress [Pa]
23 ss
flo velocity [m/s]
w
24 ra
te
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0e+00 0
31 0e+00 2e−04 4e−04 6e−04 8e−04 1e−03 0e+00 2e−04 4e−04 6e−04 8e−04 1e−03
y [m] y[m]
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33 Figure 15. Shear stress profile for Figure 16. Velocity profiles for Poiseuille
34 Poiseuille flow. flow of a MRF.
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36 As a numerical example, we consider the Poiseuille flow of the MRF-132DG subject
37 to a magnetic field corresponding to a 0.75 A current intensity. Two cases are
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39 considered, for mass flow rate (per unit span) of 10 7 kg / s and 10 6 kg / s , respectively.
40 The corresponding velocity profiles are shown in Figure 16. The solid lines show the
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results obtained with the quasi-analytical approach outlined above, while the circles
42 correspond to the numerical solution obtained with the commercial code FLUENT 6.3
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44 (2006). For the numerical solution, we have implemented the rheological model
45 ( & ) = ( & ) / & through an User Defined Function. One can see that both quasi-
46 analytical and numerical approaches lead to the same results, showing that regular
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commercial CFD codes can be employed to analyze various magneto-rheological
49 applications.
50 If pure Bingham plastic or Herschel-Bulkley models, with yield stress, would
51 be employed, then the CFD code needs to account for solid regions within the flow
52 domain. Moreover, from Figure 6 one can see that without the start-up region
53 included in the present model the MRF is not supposed to flow if the shear stress is
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55 lower than = 2617 Pa . However, the present model predicts flows with small mass
56 flow rate (e.g. 10 7 kg / s ) even when the shear stress is smaller than the conventional
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58 yield value, Figure 15. The same is true for larger mass flow rate ( 10 6 kg / s ), where
59 the MRF is supposed to flow only close to the wall (where > ) while behaving like
60 a solid in the middle of the channel where the velocity should be constant. Within the
present model, the velocity profile for mass flow rate of 10 6 kg / s , Figure 15, has a
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physical model of Bossis et al. (2003) where in the start-up phase the aggregates slip
23 on the walls and then begin to rotate before breaking is consistent with our rheological
24 model. The influence of temperature is shown to be independent from the electric
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25 current intensity. As a result, the variation in the MRF viscosity with temperature is
26 due to the changes in the carrier liquid viscosity with temperature.
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The new MRF rheological model is validated against measurements for the
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29 MRF132-DG suspension. The fitted flow curves are in very good agreement with
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30 experimental data within a wide range of shear stress values & = 10 6 K103 s 1 as well
31 as current intensity in magnetorheological cell coil I = 0.25K 3 A . An example is
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presented for numerical implementation in the FLUENT 6.3 code, and the computed
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34 velocity profile for laminar flow between parallel plates is validated with a quasi-
35 analytical solution.
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ACKNOWLEDGEMENTS
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40 The present research was supported by the Swiss National Science Foundation under
41 the SCOPES Joint Research Project IB7320-110942/1, and by the Romanian National
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21 Acta, 46:665-676.
22 Li, W.H., Chen, G. and Yeo, S.H. 1999. „Viscoelastic properties of MR fluids,” Smart
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Materials and Structures, 8:460-468.
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25 Li, W.H., Du, H., Chen, G. and Yeo, S.H. 2002. „Experimental investigation of creep
26 and recovery behaviors of magnetorheological fluids,” Materials Science and
27 Engineering, A333:368-376.
28 Macosko, C.W. 1994. Rheology. Principles, Measurements, and Applications, Wiley-
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VCH.
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31 Papanastasiou, T.C. 1987. „Flow of Materials with Yield”, Journal of Rheology,
32 31(5):385-404.
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33 *** 2006. FLUENT 6.3 User’s Guide, Fluent Inc., Lebanon, NH, U.S.A.
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