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Article history: This work presents a theoretical law to predict the mean Nusselt number for a laminar pipe flow of a
Received 26 January 2018 magnetic fluid subjected to an uniform magnetic field. The intensity of the field, the magnetic suscep-
Revised 14 May 2018
tibility of the fluid and the orientation angle formed between the magnet and the direction of the flow
Accepted 16 May 2018
appear explicitly in the final expression obtained in this work. The theory developed here considers the
Available online 17 May 2018
superparamagnetism hypothesis, so it can not be applied for magneto-rheological suspensions of large
Keywords: (micrometric) particles. However, it could be used for the vast majority of commercial ferrofluids in con-
Magnetic fluid ceptual designs of more efficient heat exchangers, specially in microfluidic applications. The limitations
Pipe flow of our theory are also discussed. We provide a curve with combinations of operational parameters for
Heat transfer increase which the Nusselt number of the flow may be intentionally controlled in order to increase or decrease
Microfluidic devices the convective heat transfer rates inside the pipe. The breakthroughs and limitations of our theory are
Ferrohydrodynamics.
also discussed in details as well as some suggestions for future works.
© 2018 Elsevier Ltd. All rights reserved.
https://doi.org/10.1016/j.mechrescom.2018.05.005
0093-6413/© 2018 Elsevier Ltd. All rights reserved.
28 R.G. Gontijo / Mechanics Research Communications 91 (2018) 27–32
NuD
θ = 5π/4
conditions T to be finite in the center of the tube and Ts in the wall 10 +
(keeping in mind that if qs is constant at the wall, then Ts = Ts (z )), θ = 3π/2
we have 8
2vm r02 dTm r2 r4 3
T (r, z ) = Ts (z ) + − −
α dz 4r02 16r04 16 6
4 v m μ0 ( 1 + χ ) H02
+ r 3 − r03 sin θ cos θ . (14) 4
+++++++++++++++++++++++++++++++++++++++++++++++++++
9kr02
Eq. (14) can be used to determine the mean temperature Tm , de-
2
fined for a circular tube as 0 0.2 0.4 0.6 0.8 1
Tm =
2
r0
vz (r )T (r, z )rdr, (15)
λm
vm r02 0
Fig. 2. NuD as a function of the magnetic parameter λm for several values of θ . The
replacing Eq. (14) in (15), we obtain legend of the symbols used in the plot are shown in the trigonometric circle in the
11 v dT top left of the figure.
m m
Tm (z ) = Ts (z ) − r02
48 α dz
108μ0 vm (1 + χ )H02
−r0 sin θ cos θ . (16) in the values of the Nusselt number. This condition occurs for
315k
θ = [0, π /2, π , 3π /2]. It is important to mention that our theory,
Through a simple energy balance it is possible to show that up to now, does not consider any effects regarding a non-uniform
dTm q P magnetic field. It has been pointed out that a magnetic field gra-
= s , with P = π D and m˙ = ρvm π r02 , (17) dient in a Poiseuille flow modifies the velocity distribution inside
dz m˙ C p
the pipe [20]. We may speculate that a magnetic field gradient
where P denotes the perimeter of the tube cross section and m˙ could increase or decrease the mean values of the Nusselt number,
represents the mass flow rate through the tube. Using Eq. (17) and even when the field is perpendicular or parallel to the direction
Newton’s cooling law in Eq. (16) we have of the flow. However, for sufficiently strong magnetic fields acting
qs 11qs D 108μ0 vm (1 + χ )H02 on small tubes (when the hypothesis of uniform field may apply)
= + r0 sin θ cos θ . (18) our theory indicates that the average values of the convective heat
h 48αρC p 315k
transfer coefficients are not altered for these angles.
Multiplying Eq. (18) by k/qs D it is straighfoward to show that the It is also noticeable that depending on the orientation between
mean Nusselt number (NuD = hD k
) is given by: the magnet and the flow direction we may increase or decrease
11 −1 the mean value of the Nusselt number. For θ = π /4 and θ = 5π /4
108
NuD = + λm f (θ ) . (19) we observe a decrease on the mean Nusselt number values, while
48 315 for θ = 3π /4 and θ = 7π /4 a meaningful increase is observed.
Where λm and f(θ ) are given by This behavior suggests an operational condition for which the heat
transfer rates inside the pipe may be controlled.
μ0 vm (1 + χ )H02
λm = and f (θ ) = sin θ cos θ . (20) In order to provide a more realistic information regading the
2qs practical use of this heat transfer control technique we present
Note that in the limit λm → 0 we have NuD = 4.36, which is the Table 1. For this table we have considered typical values of r0 =
classical solution for fully developed laminar pipe flow subjected 2.5 mm, χ = 1, qs = 10 0 0 W/m2 and vm = 0.01 m/s. The table was
to a constant heat flux boundary condition. Eq. (19) states that it built for two fixed angles θ 1 and θ 2 that may produce an increase
is possible to control the Nusselt number inside the tube through and a decrease in the mean Nusselt number respectively. We have
the application of an external magnetic field. It also provides use- selected θ1 = 3π /4 and θ2 = π /4.
ful information regarding the orientation of the field in order to The mean velocity considered for the calculations shown in
achieve a desired increase/decrease effect on the convection heat Table 1 is compatible with a volume flow rate Q ≈ 0.05 ml/s. This
transfer coefficient inside the tube. value of Q is consistent with the context of microfluidic applica-
tions (flows in capillary tubes for example). This would be a po-
3. Results and discussions tential application of our theory. Thus, in order to check the va-
lidity of these numerical values with our assumptions, we esti-
Our first result concerns the behavior of the mean Nusselt num- mated ReD ≈ 0.25. This estimation was done based on typical val-
ber NuD with respect to the magnetic parameter λm for several ues of density and dynamic viscosities of commercial ferrofluids
combinations of the orientation angle θ . This plot is shown in (ρ ≈ 850 kg/m3 and η ≈ 80 × 10− 3 Pa s). The estimated value of
Fig. 2. ReD is much smaller than 2300, so we may consider the hypoth-
It is possible to observe that when the magnet is perpendic- esis of laminar duct flow. Moreover, for a laminar duct flow with
ular or parallel to the flow direction, there is no modification ReD ≈ 0.25, the average hydrodydynamic entrance length according
30 R.G. Gontijo / Mechanics Research Communications 91 (2018) 27–32
Table 1 is always aligned with the appplied vector field H . This assump-
Variation of λm and NuD as a function of the applied field H considering two ori-
tion is expressed by the classical constitutive law: M = χ H , where
entation angles θ 1 and θ 2 . This table was built considering r0 = 2.5 mm, qs =
10 0 0 W/m2 , vm = 0.01 m/s and χ = 1. χ is the fluid’s magnetic susceptibility. The superparamagnetism
assumption is equivalent to assume that all the magnetic parti-
μ0 H0 (T) θ1 = 3π /4 θ2 = π /4 cles dipole respond instanteneously to the magnetic torques in-
λm NuD λm NuD
duced by the applied field. Indeed, we may highlight two impor-
0 0.0 0 0 4.36 0.00 4.36 tat time scales for the magnetization dynamics here: a Néel time
0.01 0.001 4.37 0.00 4.36
scale τ N and a Brownian rotational time scale τ B . These charac-
0.02 0.003 4.37 0.00 4.35
0.03 0.007 4.39 0.01 4.34 teristic time scales are related to the time that the particle dipole
0.04 0.013 4.41 0.01 4.32 takes to respond to the action of a magnetic field (τ N ) and the
0.05 0.020 4.43 0.02 4.30 time the particle itself takes to turn around in response to Brown-
0.06 0.029 4.46 0.03 4.27
ian torques (τ B ). These scales are both related to the size of the
0.07 0.039 4.49 0.04 4.24
0.08 0.051 4.53 0.05 4.20 particles. While τ B ∼ exp (a3 ), being a the radius of the particle,
0.09 0.064 4.58 0.06 4.16 we have τ B ∼ a3 , so even in the nano realm smaller particles tend
0.10 0.080 4.64 0.08 4.12 to present an internal spin dynamics uncoupled with the body of
0.11 0.096 4.70 0.10 4.07 the particle itself. The magnetic relaxation time scale τ M is simply
0.12 0.114 4.77 0.11 4.02
the smaller of τ N or τ B when both scales are very different. The
0.13 0.134 4.85 0.13 3.97
0.14 0.156 4.93 0.16 3.91 superparamagnetic hypothesis adopted here, may be expressed in
0.15 0.179 5.03 0.18 3.85 terms of time scale relations as: τ N τ B and τ N → 0. The super-
0.16 0.204 5.14 0.20 3.79 paramagnetic hypothesis presents the following consequences: 1 –
0.17 0.230 5.26 0.23 3.73
the fluid’s stress tensor is symmetric; 2 – magnetic torques in any
0.18 0.258 5.39 0.26 3.66
0.19 0.287 5.54 0.29 3.60
continuum fluid volume are absent; 3 – the vorticity of the flow
0.20 0.318 5.71 0.32 3.53 does not alter the supension magnetization field; 4 – magnetic ori-
gin surface forces on the momentum equation within the fluid are
only present for non-uniform applied fields; 5 – the supension vor-
to Langhaar [22] would be LH ≈ 0.03 mm and the thermal entrance ticity may be altered only when a magnetic field gradient is con-
length considering Pr ≈ 300 according to Kays et al. [23] would sidered. From this short discussion it is evident that the observed
be LT ≈ 9 mm. These values indicate the possibility of using the effects on the behavior of the Nusselt number as a function of the
present theory in microfluidic applications without a major loss applied field arise exclusively from the term σ : ∇ v in the energy
of generality, specially in capillary tubes where the magnetic field equation. We may interpret these effects as an absortion or pro-
produced by a large magnet would be approximately uniform in duction of internal energy within the fluid due to magnetic effects.
the region of the capillary. These arguments and preliminary cal-
culations suggest that the physical reality of the problem is more
likely to fit into the restrictive assumptions made during the de- 3.2. λm × θ neutral line
duction process of the present theory for microfluidic applications.
The input variable for controlling the convective heat trans- Eq. (19) indicates that there is a combination of parameters λm
fer coefficient inside the tube is the applied field μ0 H0 , which in and θ that may lead to an increase or decrease in the mean Nusselt
Table 1 is presented in [T]. Note that we would need a high mag- number value for a fully developed laminar pipe flow. The neces-
netic field in order to produce a substantial increase in the mean sary condition for an increase in the Nusselt number is expressed
Nusselt number for these conditions. For a field of approximately by the following inequality
0.2T = 20 0 0G we could achieve an increase of 31% considering av- 11
erage values of thermophysical properties of typical magnetic flu- − < 0.34λm sin θ cos θ < 0 (21)
48
ids. This result seems promising, but it is important to highlight
that this theoretical prediction is highly conceptual. In terms of Eq. (21) states that for positive values of the trigonometric function
a real experiment we could hardly attend all the hypothesis con- sin (θ )cos (θ ) the necessary condition for an increase in the Nusselt
sidered in this theoretical analysis. A main concern would be the number is that λm < 0. This condition would be satisfied only for
generation of an uniform, controllable magnetic field. However, in negative values of χ (which applies only for diamagnetic materials,
a recent numerical study, performed by Mousavi et al. [21], con- not the case of real ferrofluids). In the second and fourth quad-
sidering a sinusoidal double pipe heat exchanger, the authors have rant of the trigonometric circle (π /2 < θ < π and 3π /2 < θ < 2π )
claimed to observe an increse of 40% in the Nusselt number for any positive value of λ will lead to an increase in the Nusselt num-
the totally developed region, using magnetic fluids and an applied ber. However, the values of λm must be bounded by the restriction
field. This increase was observed from the surface Kelvin forces
that appear in the equations of motion when a magnetic field gra- 11
dient is considered. In this paper [21] the authors did not con- − < 0.34λm sin θ cos θ , (22)
48
sider the effect of the term σ : ∇ v in the energy equation, which
is the source of the effects explored by our theory. However, this so we don’t have physically inconsistent negative values of NuD .
work provides a support towards the possibility of heat transfer This restriction leads to λm < −0.67/(sin θ cos θ ) for the second
enhancement using magnetic fluids under the presence of an ex- and fourth quadrants. In Fig. 3 we plot the crictical condition in
ternal field. which this inequality is satisfied. Any value of λm above the curve
will lead to a physically inconsistent value on the prediction of the
3.1. A brief discussion regarding stress asymmetry effects mean Nusselt number for that orientation angle θ . The values bel-
low the curve and above the dashed line (gray area) will lead to an
At this point is important to provide a short discussion regard- increase in the mean Nusselt number according to our theory. This
ing the non-symmetric effects on the stresses within the fluid. curve may be used to calculate the intensity of the applied field
In our formulation we have considered the superparamagnetism for a typical orientation of the magnet that will lead to a desired
hypothesis. This hypothesis states that the fluid magnetization M increase in the convective heat transfer coefficient inside the pipe.
R.G. Gontijo / Mechanics Research Communications 91 (2018) 27–32 31
Acknowledgments
Supplementary material
[23] W.M. Kays, M.E. Crawford, B. Weigand, Convective Heat and Mass Transfer, [27] S. Odenbach, H.W. Muller, Stationary off-equilibrium magnetization in ferroflu-
fourth ed., Boston: McGraw-Hill Higher Education, 2005. 2005. ids under rotational and elongational flow, Phys. Rev. Lett. 89 (3) (2002).
[24] M. Osaci, C. Abrudean, A. Berdie, Relaxation times in magnetic nanoparticles [28] S. Odenbach, H.W. Muller, On the microscopic interpretation of the coupling
system and memory effects, Acta Phys. Pol. A 112 (6) (2007). of the symmetric velocity gradient to the magnetization relaxation, J. Magn.
[25] M.I. Shiliomis, Comment on magnetoviscosity and relaxation in ferrofluids, Magn. Mater. 289 (2005) 242–245.
Physical Review E 64 (2001) 063501(R).
[26] M.I. Shiliomis, Ferrohydrodynamics: testing a third magnetization equation,
Phys. Rev. E 64 (2001) 060501(R).