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We show a topological spin texture called “bimeronium” in magnets with in-plane magnetization. It is a topological
counterpart of skyrmionium in perpendicularly magnetized magnets and can be seen as a combination of two bimerons
with opposite topological charges. We report the static structure and spin-orbit-torque-induced dynamics of an isolated
bimeronium in a magnetic monolayer with frustrated exchange interactions. We study the anisotropy and magnetic
field dependences of a static bimeronium. We also explore the bimeronium dynamics driven by the damping-like spin-
orbit torque. We find that the bimeronium shows steady rotation when the spin polarization direction is parallel to
the easy axis. Moreover, we demonstrate the annihilation of the bimeronium when the spin polarization direction is
perpendicular to the easy axis. Our results are useful for understanding fundamental properties of bimeronium structures
and may offer an approach to build bimeronium-based spintronic devices.
Topological magnetism and spin frustration are important trated bimeronium could be used as a special building block
and hot topics in the fields of magnetism and spintronics1–13 . for spintronic applications, however, it cannot move like the
The link between topological magnetism and spin frustration frustrated bimeron36 due to its complex and non-circular sym-
lies in the fact that many topological spin textures can be sta- metric spin structure that could be annihilated by the SOT at
bilized in frustrated spin systems14–37 . For example, the mag- certain conditions.
netic skyrmion is an exemplary topological spin texture1,2 , Our simulated system is a J1 -J2 -J3 classical Heisenberg
which can be regarded as a quasi-particle and shows intriguing model on a simple monolayer square lattice12,16,21,30,36,37,57 ,
dynamics3–13 . where the nearest-neighbor (NN) exchange interaction J1 is
The magnetism and spintronics community has focused ferromagnetic (FM), while the next-NN (NNN) J2 and next-
on skyrmions stabilized by the Dzyaloshinskii-Moriya (DM) NNN (NNNN) J3 exchange interactions are antiferromag-
interaction38–44 , however, recent progress in the field re- netic (AFM). The Hamiltonian H includes the FM and AFM
vealed that skyrmions and other topological spin textures exchange interactions, in-plane easy-axis magnetic anisotropy
can be found in a different system, where topological (K), and applied magnetic field (B), given as
spin textures are stabilized by exchange frustration14–37 . X X
Typical frustrated topological spin textures include the H = − J1 mi · mj − J2 mi · mj (1)
skyrmion14–36 , the skyrmionium37,45,46 (i.e., target skyrmion47 <i,j> i,j
and 2π-skyrmion48 ), and the bimeron20,34,36 (i.e., asymmet- X X X
ric skyrmion49 and meron pair50 ). Indeed, skyrmioniums and − J3 mi · mj − K (mxi )2 − B · mi ,
≪i,j≫ i i
bimerons can also be stabilized by the DM interaction34,51–56 .
In principle, all of these particle-like topological spin textures where mi represents the normalized spin at the site i, |mi | =
can be used to carry information4,5,7–11,13 , and thus are promis- 1. hi, ji, hhi, jii, and hhhi, jiii run over all the NN, NNN,
ing for building future information storage and logic comput- and NNNN sites in the magnetic monolayer, respectively. K
ing devices4,5,7–11,13 . is the easy-axis magnetic anisotropy constant, and the easy
In this Letter, we report that the topological counterpart of axis direction is aligned along the x axis. B is the applied
skyrmioniums, which is called the bimeronium [Fig. 1(a)], can magnetic field.
be stabilized in an in-plane magnetic system with competing The spin dynamics is simulated by using the Object
exchange interactions. We study the static structure of an iso- Oriented MicroMagnetic Framework (OOMMF)58 with our
lated bimeronium with a topological charge of zero at differ- extension modules for the J1 -J2 -J3 classical Heisenberg
ent anisotropies and magnetic fields. We also investigate the model16,21,30,36,37 . We also use the OOMMF conjugate gra-
dynamics of an isolated bimeronium induced by the damping- dient minimizer for obtaining relaxed spin structures, which
like spin-orbit torque (SOT). Our results suggest that the frus- is a method that locates local minima in the energy surface
through direct minimization techniques58 . The spin dynamics
is governed by the Landau-Lifshitz-Gilbert (LLG) equation58
a) X.Z.
and J.X. contributed equally to this work.
b) Authors
to whom correspondence should be addressed: ezawa@ap.t.u- dm dm
tokyo.ac.jp and zhouyan@cuhk.edu.cn = −γ0 m × heff + α m × , (2)
dt dt
2
(b ) (c ) (d )
where |m| = 1 represents the normalized spin, heff =
δH
− µ01MS · δm is the effective field, t is the time, α is the Gilbert (a )
damping parameter, γ0 is the absolute value of the gyromag-
netic ratio, and MS is the saturation magnetization.
(e ) (f) (g )
For the spin dynamics driven by the SOT, we con-
sider the damping-like SOT τd expressed as4,9,11,59 τd =
u
a (m × p × m), where u = |(γ0 ~/µ0 e)| · (jθSH /2MS ) is
y + 1
m z
z
the spin torque coefficient. ~ is the reduced Planck constant, x -1
T o ta l
3 0 y
x
texture edge51 . For the bimeronium and skyrmionium, we as-
7 .0 m
E
m
z
E
0
6 .5
sume that θ rotates 2π for spins from H the texture center to the -3 0
-0 .4 2 2
1
texture edge51 . Hence, Qv = 2π C
dφ is the vorticity and η -6 0
6 .0
-0 .4 2 4
5 .5
is the helicity defined mod 2π. Note that η = 0 is identical to E T o ta l E N N E N N N E N N N N E K 0 .0 0 .5
1 .0
( π)
1 .5 2 .0 0 .0 0 .5
1 .0
( π)
1 .5 2 .0
η = 2π. ( cd ) (e ) (f) (g )
The default simulation parameters are16,21,30,36,37 : J1 = 30
meV, J2 = −0.8 (in units of J1 = 1), J3 = −0.9 (in units
of J1 = 1), K = 0.02 (in units of J1 /a3 = 1), B = 0
(in units of J1 /a3 MS = 1), α = 0.3, γ0 = 2.211 × 105 m
A−1 s−1 , θSH = 0.2, and MS = 580 kA m−1 . The lattice
constant is a = 0.4 nm (i.e., the mesh size is 0.4 × 0.4 × 0.4
FIG. 2. (a) Different energy contributions for a relaxed bimeronium
nm3 ). We have simulated the metastability diagram showing
with η = 0. The energies are given in units of J1 = 1. (b) Total
that the frustrated bimeronium can be a metastable state for energy of a relaxed bimeronium as a function of η. (c) Spin com-
a wide range of J2 and J3 (see supplemental material). The ponents of a relaxed bimeronium as functions of η. Top views of
minimum required value of J3 for stabilizing bimeroniums relaxed bimeroniums with (d) η = 0, (e) η = π/2, (f) η = π, and
decreases with increasing J2 . (g) η = 3π/2 are given. Here, J2 = −0.8, J3 = −0.9, K = 0.02,
We first study the static structures and properties of a and B = 0. The arrows represent the spin directions. The out-of-
relaxed isolated bimeronium in the magnetic monolayer plane spin component (mz ) is color coded. The displayed area is of
with competing exchange interactions and in-plane easy-axis 10 × 10 nm2 .
anisotropy, where we set J2 = −0.8, J3 = −0.9, K = 0.02
and B = 0. Figure 1 shows the top views of relaxed com-
pact bimeronium and bimeron structures. For the purpose of for a relaxed bimeronium are given in Fig. 2(a). It shows that
comparison, we also show the relaxed solutions of compact the competition among the FM NN, AFM NNN, and AFM
skyrmionium and skyrmion obtained with the same param- NNNN exchange interactions is considerable. The magnetic
eters but an easy-axis aligned along the z axis. The given anisotropy energy is positive, which means larger anisotropy
skyrmionium with Q = 0 [Fig. 1(e)] consists of an inner constant could raise the total energy of a bimeronium and may
skyrmion with Q = −1 [Fig. 1(f)] and an outer skyrmion with reduce its stability. A controllable degree of freedom of topo-
Q = +1 [Fig. 1(g)]. Similarly, the corresponding bimero- logical spin textures in frustrated magnetic systems is the he-
nium with Q = 0 [Fig. 1(b)] exists as a combination of an licity η 15,16,21,30,36,37 . It is found that the energy [Fig. 2(b)]
inner bimeron with Q = −1 [Fig. 1(c)] and an outer bimeron and spin components [Fig. 2(c)] of the bimeronium are inde-
with Q = +1 [Fig. 1(d)]. Namely, the bimeronium in in-plane pendent of its helicity. We note that although the bimeronium
magnetized magnets can be seen as a topological counterpart helicity can freely vary between 0 and 2π, the orientation of
of the skyrmionium in out-of-plane magnetized magnets. the background spins outside the bimeronium is aligned with
The total energy as well as different energy contributions the easy axis orientation, i.e., the x direction in this work.
3
( a ) 0 .0
m
(b ) 1 6 (c ) 8
fect in a heavy-metal substrate layer underneath the magnetic
T o ta l
x 1 2 6
-0 .3
monolayer4,5,7–9,11,60 . We first consider that the direction of
x
K
m
E
m
y
8 4
E
-0 .6 m z
-0 .9
4 2 spin polarization is aligned along the easy-axis direction, i.e.,
0 .0 0 0 .0 2 0 .0 4
K
0 .0 6 0 .0 8 0 .1 0 0 .0 0 0 .0 2 0 .0 4
K
0 .0 6 0 .0 8 0 .1 0 0 .0 0 0 .0 2 0 .0 4
K
0 .0 6 0 .0 8 0 .1 0
p = +x̂. A recent report36 numerically demonstrates that
(d ) 1 0 8 (e ) (f) -3 6
1 0 4 -5 2 a frustrated bimeron shows SOT-induced self rotation when
N N N N
N N N
N N
-4 0
1 0 0
the spin polarization direction is parallel to the easy-axis di-
E
-5 6
E
9 6 -4 4
9 2
-6 0 rection. Similarly, we find that the bimeronium also shows
0 .0 0 0 .0 2 0 .0 4 0 .0 6 0 .0 8 0 .1 0 0 .0 0 0 .0 2 0 .0 4 0 .0 6 0 .0 8 0 .1 0 0 .0 0 0 .0 2 0 .0 4 0 .0 6 0 .0 8 0 .1 0
K K K steady self rotation induced by the damping-like SOT when
( cg ) K = 0 . 0 1 (h ) K = 0 .0 2 ( i) K = 0 .0 4 ( j) K = 0 .0 8
p = +x̂, which can be described by a theoretical approach
(see supplemental material). The rotation period decreases
with increasing driving current density [Fig. 4(a)] and the ro-
tation frequency is proportional to the driving current density
[Fig. 4(b)]. At a given current density, the inner and outer
consisting bimerons of the bimeronium rotate in an identical
FIG. 3. (a) Spin components as functions of K. A bimeronium with manner, and the rotation frequency of the whole structure de-
η = 0 is relaxed at the center of a monolayer with J2 = −0.8, creases with increasing damping parameter α. For the rotat-
J3 = −0.9, and B = 0. (b) Total energy ETotal as a function of K. ing bimeronium, its total energy [Fig. 4(c)] and spin compo-
The energies are given in units of J1 = 1. (c) Anisotropy energy EK nents [Fig. 4(d)] are independent of time when the steady ro-
as a function of K. (d) NN exchange energy ENN as a function of tation state is reached. Note that the rotating bimeronium is
K. (e) NNN exchange energy ENNN as a function of K. (f) NNNN a dynamic stable object, which will not be annihilated even
exchange energy ENNNN as a function of K. Top views of relaxed at a high speed rotation as the the inner and outer consisting
bimeroniums with η = 0 at (g) K = 0.01, (h) K = 0.02, (i) K =
bimerons rotate in an identical frequency and direction. On
0.04, and (j) K = 0.08 are given. The arrows represent the spin
directions. The out-of-plane spin component (mz ) is color coded.
the other hand, due to the non-circular symmetric out-of-plane
The displayed area is of 12.4 × 12.4 nm2 . spin structure of the bimerionium, its rotation can be observed
by imaging the out-of-plane cores, while the self rotation of
skyrmions and skyrmioniums can only be observed by imag-
As the magnetic anisotropy can be adjusted experimentally, ing their in-plane spin components. Thus, we point out that it
we study the bimeronium structure for different anisotropy is possible to observe rotating bimeroniums by using the Kerr
constants K, as shown in Fig. 3. By increasing K from 0 to microscope system.
0.095, while keeping the easy-axis orientation aligned along The bimeronium rotation depends on both the internal
the x direction, the size of relaxed bimeronium decreases ob- structure of the bimeronium as well as the spin polarization
viously. The spin component mx reduces with increasing K, direction. As shown in Fig. 4(e), when the bimeronium con-
while my and mz do not depend on K [Fig. 3(a)]. The total sists of an inner bimeron with Q = −1 and an outer bimeron
energy [Fig. 3(b)], anisotropy energy [Fig. 3(c)], AFM NNN with Q = +1, it shows counterclockwise rotation driven by
exchange energy [Fig. 3(e)], and AFM NNNN exchange en- the damping-like SOT with p = +x̂. If the initial bimeronium
ergy [Fig. 3(f)] increase with K, while the FM NN exchange structure consists of an inner bimeron with Q = +1 and an
energy [Fig. 3(d)] decreases with increasing K. When K outer bimeron with Q = −1, it may show clockwise rotation
is larger than certain threshold (i.e., 0.1 in this work), the driven by the damping-like SOT with p = −x̂ (see supple-
bimeronium structure becomes unstable and cannot exist in mental material).
the system. As reported in Ref. 36, a frustrated bimeron could show
We also study the effect of an external in-plane magnetic SOT-induced translational motion when the spin polarization
field on the bimeronium structure (see supplemental material). direction is perpendicular to the easy-axis direction. How-
As the bimeronium size is related to its spin component along ever, we find that the frustrated bimeronium cannot be driven
the easy-axis orientation, which is mx in this work [Fig. 3(a)], into steady motion when the spin polarization direction is per-
we apply a magnetic field along the x direction with a strength pendicular to the easy-axis direction, i.e., p = ±ŷ. Instead,
of Bx . Within a reasonable range of Bx that does not destroy the damping-like SOT leads to the deformation and annihi-
the bimeronium (i.e., in this work Bx /1000 = −0.2 ∼ 0.8 lation of the bimeronium structure, as shown in Fig. 5. To
in units of J1 /a3 MS = 1), it is found that the bimeronium be more specific, the damping-like SOT leads to different ro-
size is insensitive to Bx . The spin component mx increases tation behaviors of the inner and outer consisting bimerons
with Bx , while my and mz are independent of Bx . The to- of the bimeronium, and the bimeronium structure is twisted
tal energy, anisotropy energy, and FM NN exchange energy upon the application of the SOT. When the out-of-plane cores
are proportional to Bx , while the AFM NNN and NNNN ex- of the inner and outer consisting bimerons merge together,
change energies are inversely proportional to Bx . Note that a the bimeronium is thus destroyed and annihilated. The to-
larger external magnetic field may lead to the deformation and tal energy [Fig. 5(a)] and spin component mx [Fig. 5(b)] de-
annihilation of the bimeronium texture. crease significantly during the SOT-induced annihilation of
As shown in Fig. 4, we continue by investigating the dy- the bimeronium. The spin components my and mz also show
namics of an isolated bimeronium driven by the damping-like certain fluctuations during the annihilation process. Note that
SOT τd . We assume that τd is generated by the spin Hall ef- the initial bimeronium structure in Fig. 5 consists of an inner
4
1 .4 (a ) 8 (b )
(a ) p = + x (b ) 1 2
= 0 .1 = 0 .1 7 p = + y -0 .9
1 .2
x
= 0 .3 1 0 = 0 .3 6 = 0 . 1
m
1 .0 -1 .0
= 0 .5 = 0 .5 5 j = 5 ×1 0 1 0
A m -2
8 0 .0 5
f (G H z )
0 .8
T (n s )
to ta l
0 .0 0
y
0 .6 6
3
m
E
-0 .0 5
0 .4 4 2
0 .0 5
1
0 .2 2 0 .0 0
z
0
m
0 .0 0 -0 .0 5
6 8 1 0 1 2 1 4 6 8 1 0 1 2 1 4 -1
1 0 -2 1 0 -2 0 .0 0 .1 0 .2 0 .3 0 .4 0 .5 0 .0 0 .1 0 .2 0 .3 0 .4 0 .5
j (1 0 A m ) j (1 0 A m ) t (n s ) t (n s )
-0 .8 3
(c ) (d ) (c )
6 .9 9 x
-0 .8 4
m
2
t (n s ) 0 0 .0 6 0 .0 8 0 .0 9 0 .1 1 0 .1 7 0 .2 4
)
1
-1 1
to ta l
6 .9 8
(1 0
0
E
A m
-1 1
= 0 . 1
6 .9 7
time during its annihilation induced by the SOT. (c) Top views of
z
-1
m
No. 2019A1515110713). M.E. acknowledges the support 28 T. Kurumaji, T. Nakajima, M. Hirschberger, A. Kikkawa, Y. Yamasaki, H.
by the Grants-in-Aid for Scientific Research from JSPS Sagayama, H. Nakao, Y. Taguchi, T.-h. Arima, and Y. Tokura, Science 365,
KAKENHI (Grant Nos. JP18H03676 and JP17K05490) and 914 (2019).
29 L. Desplat, J. V. Kim, and R. L. Stamps, Phys. Rev. B 99, 174409 (2019).
the support by CREST, JST (Grant Nos. JPMJCR20T2 30 J. Xia, X. Zhang, M. Ezawa, Z. Hou, W. Wang, X. Liu, and Y. Zhou, Phys.
and JPMJCR16F1). O.A.T. acknowledges the support by Rev. Applied 11, 044046 (2019).
31 R. Zarzuela, H. Ochoa, and Y. Tserkovnyak, Phys. Rev. B 100, 054426
the Australian Research Council (Grant No. DP200101027),
the Cooperative Research Project Program at the Re- (2019).
32 V. Lohani, C. Hickey, J. Masell, and A. Rosch, Phys. Rev. X 9, 041063
search Institute of Electrical Communication, Tohoku Uni- (2019).
versity (Japan), and by the NCMAS grant. G.Z. ac- 33 I. F. Sharafullin, M. Kh. Kharrasov, and H. T. Diep, Phys. Rev. B 99, 214420
knowledges the support by the National Natural Science (2019).
34 B. Göbel, A. Mook, J. Henk, I. Mertig, and O. A. Tretiakov, Phys. Rev. B
Foundation of China (Grant Nos. 51772004, 51771127,
and 51571126). X.L. acknowledges the support by the 99, 060407(R) (2019).
35 I. F. Sharafullin and H. T. Diep, Symmetry 12, 26 (2020).
Grants-in-Aid for Scientific Research from JSPS KAK- 36 X. Zhang, J. Xia, L. Shen, M. Ezawa, O. A. Tretiakov, G. Zhao, X. Liu, and
ENHI (Grant Nos. JP20F20363). Y.Z. acknowledges the Y. Zhou, Phys. Rev. B 101, 144435 (2020).
support by the Guangdong Special Support Project (Grant 37 J. Xia, X. Zhang, M. Ezawa, O. A. Tretiakov, Z. Hou, W. Wang, G. Zhao,
No. 2019BT02X030), Shenzhen Peacock Group Plan (Grant X. Liu, H. T. Diep, and Y. Zhou, Appl. Phys. Lett. 117, 012403 (2020).
38 S. Mühlbauer, B. Binz, F. Jonietz, C. Pfleiderer, A. Rosch, A. Neubauer, R.
No. KQTD20180413181702403), Pearl River Recruitment
Georgii, and P. Böni, Science 323, 915 (2009).
Program of Talents (Grant No. 2017GC010293), and National 39 X. Z. Yu, Y. Onose, N. Kanazawa, J. H. Park, J. H. Han, Y. Matsui, N.
Natural Science Foundation of China (Grant Nos. 11974298 Nagaosa, and Y. Tokura, Nature 465, 901 (2010).
and 61961136006). 40 S. Woo, K. Litzius, B. Kruger, M.-Y. Im, L. Caretta, K. Richter, M.