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Magnetization of Hard S Uperconductors
Magnetization of Hard S Uperconductors
M AGNETIZATION OF HA RD S U P E R C O N D U C T O R S
5.1 Introduction
This chapter discusses the magnetization of hard superconductors. When the
first generation of superconducting magnets was built in the mid 1960s, many of
them failed to reach their designed operating currents. These magnets quenched
at currents far below their expected values because of a then unknown or little
understood magnetic phenomenon called flux jumping. By the late 1960s, the rea-
sons for flux jumping were elucidated, and solutions to eliminate it emerged soon
afterwards. Today, well-established methods of producing superconducting wires
and cables that minimize the problems of flux jumping are available. However,
AC loss is another magnetization issue that directly affects magnet operation and
that continues to challenge the magnet designer. This chapter discusses the funda-
mental theory behind the magnetization of hard superconductors; AC losses will
then be addressed in more detail in Chapter 7. As in previous chapters, only those
problems that can be treated analytically by simple closed-form mathematical
expressions are considered.
(5.1a)
(5.1b)
(5.1c)
Note that the slope of the H s ( x ) is equal to J c , positive where J c is positive (z-
directed, out of the paper) and negative where Jc is negative. x* (and 2a – x +)
gives the extent of the field penetration in the slab; in terms of H e and J c :
(5.2)
At H e = H p Jc a, x* = x + = a and the entire slab is in the critical state; H p is
known as the penetration field.
The average magnetic induction within the slab, B s , is thus given by
(5.3b)
(5.3c)
(5.4)
(5.5)
MA G N E T I Z A T I O N OF H A R D SU P E R C O N D U C T O R S 165
The dotted lines in Fig. 5.2 represent Hs (x) at H e = H m > H p , where H m is the
maximum external field applied in this particular field sweep sequence.
As H e is reduced from H m towards 0, H s (x) changes as indicated by the solid lines
in Fig. 5.2. When H e c = H m – 2Hp , as may be inferred from Fig. 5.2, because
Hs (x) is a complete mirror image of that at H m , –M becomes – Hp /2. That is,
magnetization is now positive. It can be shown that for the return field sweep
from H m to H e c , – M(H e ) is given by:
(5.6)
Fig. 5.3 Magnetization vs field traces for a hard superconducting slab subjected to an
external field sequence of 0 → H c 2 → 0. The solid curve presents the case Jc =constant;
the dotted curve qualitatively presents the case Jc (H e ), with J c = 0 at H c 2.
Figure 5.4 shows the current distribution within the slab corresponding to the field
distribution given in Fig. 5.1. The net current per unit length in the y-direction
[A/m] flowing through the slab in the z-direction is given by:
(5.7)
(5.8a)
(5.8b)
(5.8c)
Figure 5.6 shows current distribution J( x) in the slab. By integrating J(x) across
the slab width, we can show that the net current flowing in the slab is indeed I t :
(5.9a)
(5.9b)
As expected, the net current in the slab is the current supplied by the external
source. Note that the presence of an external field , when it is applied after
It has been applied, does not fundamentally change the distributions shown in
Figs. 5.5 and 5.6; but if is applied before It , different H s (x) and J(x) would
emerge. Problems 5.1~5.3 treat the effects of transport current on magnetization
in detail.
Fig. 5.7 Detailed tracings of field distribution data across a 0.5-mm gap
between two Nb-Ti rods, each 60 mm long and 8.3 mm in diameter. Each
of the four flat field lines running across the rod represents the field dis-
tribution immediately after a flux jump [5.5]. (Courtesy of H.T. Coffey.)
M AGNETIZATION OF H A R D S UPERCONDUCTORS 169
(5.10a)
(5.10b)
The subscripts pc and sc refer to the primary and secondary search coils, respec-
tively. N is the number of turns of each search coil and A is the effective area of
each turn in the coil through which H e (t ) is coupled. is the space-averaged
field over each search coil.
The bridge output voltage Vbg (t ) is given by:
(5.11)
(5.12)
(5.13a)
(5.13b)
Although in practice the condition required by Eq. 5.13a is not always satisfied
over a wide frequency range, Eq. 5.13b is a good approximation for most cases.
Generally k is close to 0.5. Vbg (t ) is fed into an integrator and its output, V m z (t ) ,
is proportional to M. Specifically, if the test sample is at the virgin state (M = 0)
and H e (t ) is increased (H e ↑ ) from 0 (at t = 0) to H e (at t = t 1 ), then we have:
(5.14)
(5.15a)
where the factor ƒ m is the ratio of magnetic material volume to the total test
sample volume. This factor is needed because generally a test sample does not
consist entirely of magnetic material for which magnetization is measured; in the
case of a multifilamentary conductor, for example, the test sample consists not only
of superconducting filaments but also of a matrix metal and other nonmagnetic
materials, e.g. insulator. If an external field excursion is
H p , then we have:
(5.15b)
M AGNETIZATION OF H A R D S UPERCONDUCTORS 171
(5.16)
(5.17a)
(5.17b)
where ƒ1 (i) = 1 – i.
(S1.1a)
(S1.1b)
(S1.1c)
( S1.2 a)
c (S1.2b)
(S1.2c)
(S1.3b)
(S1.3c)
( S1.4 a)
(S1.4b)
(S1.4c)
Fig. 5.12 Field profile with transport current (solid) for computation of magnetization.
M AGNETIZATION OF HA R D S UPERCONDUCTORS 175
(S1.5a)
(S1.5b)
(S1.6a)
(S1.6b)
(S1.7a)
(S1.7b)
(S1.8a)
(S1.8b)
(S1.9)
(5.17a)
(5.17 b)
(5.18a)
(5.18b)
c) To determine the magnetization in the slab, we must first find x* (Fig. 5.14),
which can be determined from Hs 1 (x) and Hs 2 (x).
(S2.3a)
(S2.3b)
(S2.4a)
(S2.4b)
We can now compute the shaded area, which is the sum of AI and AII (Fig. 5.14).
(S2.6a)
(S2.6b)
(S2.7a)
(S2.7b)
(S2.8)
(5.18 a )
(5.18b)
(5.19a)
(5.19b)
where f 3 ( i ) = (1 – i )².
(S3.3b)
(S3.4a)
(S3.4b)
(S3.5a)
(S3.5b)
(S3.6)
(S3.7)
(5.19 a)
(5.19 b)
where f 3 (i) = (1 – i)².
Insulation none — —
(5.20)
Fig. 5.21 V m z vs B e plot with the test sample at 4.2K and oriented with
respect to B e as in Fig. 5.20a. B e was swept at a |rate| of 0.05T/s.
MAGNETIZATION OF H A R D S UPERCONDUCTORS 187
(5.13b)
(5.16)
(S5.1)
where for Nb-Ti, B0 ~ 0.3T. J 0 is the zero-field critical current density, which is
usually difficult to measure. Thus from the Jc value at 5T and B 0 = 0.3T, we
can first solve for J 0 B0 :
(S5.2)
(S5.3)
188 C HAPTER 5
c) The –M vs B plot shown in Fig. 5.21 suggests, as remarked above, that the
search coils are well balanced. Thus:
(S5.4)
(S5.5a)
(S5.5b)
(S5.6)
MAGNETIZATION OF H ARD S UPERCONDUCTORS 189
(5.21)
Note that the entire slab is in the critical state with field at its surface (± a)
exposed to external field of
b) Derive Eq. 5.21 by computing the Poynting energy flow into the slab at
x = a and equating it with change in magnetic energy storage and dissipation
energy ε ø in the positive half of the slab.
c) To relate ∆ Jc , to an equivalent temperature rise in the conductor, we may
assume a linear temperature dependence for Jc (T):
(5.22)
(5.23)
(5.24)
190 C HAPTER 5
Because there is a change in magnetic field within the slab, an electric field is
generated, which from Faraday’s law of induction, is given by:
(S6.2)
(S6.3)
(S6.4)
Dissipation power density, p(x), is given by E z (x)J c and total energy density
dissipated in the slab, ε ø [W/m²], per unit slab surface area in the y-z plane is
given by:
(S6.5)
(5.21)
MAGNETIZATION OF HA R D S UPERCONDUCTORS 191
(S6.6)
(S6.7)
Thus:
(S6.8)
As expected, (a) points in the –x-direction or energy flux indeed flows into the
slab. Thus:
(S 6.9)
(S6.10)
(S6.11)
(S6.12)
(S6.13)
Replacing J c with J co in Eq. 5.21 and combining it with Eq. S6.14, we obtain:
( S 6.15)
Note that e ø is not only proportional to ∆ T but more importantly varies with
a 2 . Under adiabatic conditions, the dissipation energy density eø increases the
superconductor’s temperature by ∆ T s , given by:
( S6.16)
where C s is the superconductor’s heat capacity [J/m3 K]. Combining Eqs. S6.15
and S6.16 and requiring ∆ Ts < ∆ T for thermal stability, we have:
( S6.17)
For a given superconducting material and operating temperature, the only param-
eter that can be varied by the magnet designer to satisfy Eq. S6.17 is a. That
is, thermal stability can only be satisfied if the slab half width a is less than the
critical size a c , given by:
(5.24)
( S6.18)
Fig. 5.23 Magnetization vs ambient field trace for a 0.5-mm dia. Nb-Zr monofilament.
194 CH A P T E R 5
b) We can derive the flux jump energy density, eφ , using the Poynting energy
balance: e s = e φ + ∆ em , where e s is the Poynting energy density entering the
superconductor at x = a and ∆ e m is its change in stored magnetic energy density.
Let’s consider only 0 ≤ x ≤ a. ∆ H (x) within the slab is given by:
(S7.1)
From Eq. S7.1, we have:
(S7.2)
(S7.6)
(S7.7)
Because e φ = e s – ∆ em , we obtain:
(S7.8)
(5.25)
(5.26)
c) At a critical length l c , the net current I cp given by Eq. 5.26, becomes equal
to Jc d f , the slab’s critical current (per unit conductor depth). Show that an
expression for l c in terms of appropriate parameters is given by:
(5.27)
b) Once the E field is known, the current density Jcu in the copper slab is given
by: J cu = E 1x / ρ cu . The net current flowing in the copper from one superconduct-
ing slab to the other over half the conductor length is given by:
(5.26)
c) Equating Icp given by Eq. 5.26 with Jc d f and solving for l c , we have:
(5.27)
(S8.2)
In typical submicron strands, the twist pitch length is ~10mm! This means that
the diameter of such strands, by mechanical requirements, should be ~1 mm; ac-
tually a thermal-magnetic stability criterion, similar to the flux jump criterion,
requires it to be even smaller than 1mm. This is because the strand, to reduce
coupling losses, use Cu-Ni alloys as the matrix materials, resulting in a magnetic
diffusion time constant that is smaller than its thermal diffusion time constant.
(S8.3)
Solving for Nƒ from Eq. S8.3 with appropriate values of parameters, we obtain:
(S8.4)
(S 9.1)
(S 9.2)
= 27 mm
This value is close enough to the actual twist pitch of 10 mm. Because magneti-
zation of Conductor 1 (trace C) at a sweep rate of 320 oersted/sec is considerably
smaller than that of Conductor 2 for the same field sweep rate, we conclude that
p1 is significantly shorter than p2 .
b) Table 5.2 presents the values of a c for the temperature range 4~80 K. It
also includes values of Ic extracted from Fig. 5.26 and corresponding Jc used for
computation.
T Ic Jc Cs* ac
[K] [A] [MA/m²] [kJ/m³K] [mm]
4 228 1932 0.8 0.2
10 217 1839 7.7 0.7
20 194 1644 68.5 2.4
30 163 1381 240 5.5
40 135 1144 534 9.8
50 108 915 881 16
60 80 678 1219 25
70 53 449 1540 43
80 24 203 1825 103
The HTS tape used to compute a c is of “single-core,” meaning each tape contains
a central strip 3~5 mm wide (2a), processed with a silver matrix which occupies
60~70% of the total conductor volume. Tape 1, including its silver matrix, is
4.09 mm wide and 0.153 mm thick. Values of ac listed in Table 5.2 indicate that
even these “single- core” tapes are stable against flux jumping when they are op-
erated above ~20K. Within a few years these silver-sheathed tapes will likely be
multifilamentary, consisting of many (up to ~100) “mini strips” [5.13, 5.14]. The
need to process tapes in the multifilamentary form, however, is driven not so much
to satisfy the flux jumping criterion but to make them more strain resistant. Also
making strips thin inherently improves the critical current density of these HTS
tapes [5.15].
202 C HAPTER 5
References
[5.1] C.P. Bean, “Magnetization of hard superconductors,” Phys. Rev. Lett. 8 , 250
(1962).
[5.2] Y.B. Kim, C.F. Hempstead, and A.R. Strnad, “Magnetization and critical super-
currents,” Phys. Rev. 129 , 528 (1963).
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superconductor,” Phys. Rev. Letts. 11 , 149 (1963).
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[5.8] M. Yunus and Y. Iwasa (preliminary results, FBNML, 1994).
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[5.10] Superconducting Applications Group (Rutherford Laboratory), “Experimental
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[5.11] Y. Iwasa, “Magnetization of single-core, multi-strand, and twisted multi-strand
superconducting composite wires,” Appl. Phys. Lett. 14 , 200 (1969).
[5.12] K. Sato, T. Hikata, and Y. Iwasa, “Critical currents of superconducting BiPb-
SrCaCuO tapes in the magnetic flux density range 0 to 19.75T at 4.2, 15, and
20 K,” Appl. Phys. Lett. 5 7 , 1928 (1990).
[5.13] K. Sato, N. Shibutani, H. Maki, T. Hikata, M. Ueyama, T. Kato, and J. Fu-
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243 (1993).
[5.14] A. Otto, L.J. Masur, J. Gannon, E. Podtburg, D. Daly, G.J. Yurek, and A.P. Mal-
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[5.15] H. Ogiwara, M. Satou, Y. Yamada, T. Kitamura, T. Hasegawa, “Induced critical
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