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ChEnggSc FullPaper
ChEnggSc FullPaper
www.elsevier.com/locate/ces
Received 5 April 2004; received in revised form 9 June 2004; accepted 12 June 2004
Available online 24 August 2004
Abstract
An arbitrary flow of a viscous, incompressible fluid past a porous sphere of radius ‘a’ with an impermeable core of radius ‘b’, using
Brinkman’s equation in the porous region is discussed. At the interface of the clear fluid and porous region, stress jump boundary condition
for the tangential stresses along with the continuity of normal stresses and the velocity components are used. On the surface of the
impermeable core no slip condition is used. The corresponding Faxen’s laws are derived to compute the drag and torque acting on the
surface r = a. It is found that the drag and torque not only change with the change of the permeability, but also a significant effect of
the stress jump co-efficient is observed. The variation of drag and torque with permeability for different thickness (a − b) of the porous
region as well as for different values of stress jump coefficient is discussed when the basic flow is due to uniform flow, two dimensional
irrotational flow, doublet in a uniform flow, stokeslet, rotlet. In case of uniform flow the flow field has been plotted. In all the cases, a
significant effect of the stress jump coefficient has been realized.
䉷 2004 Elsevier Ltd. All rights reserved.
Keywords: Stokes flow; Brinkman equation; Impermeable core; Stress jump co-efficient
Z qI = 0. (16)
3. Solution method
X
Recently, Raja Sekhar et al. (1997) have shown the com-
C pleteness of a representation of the Brinkman’s equation. In
fact this representation has been used by Padmavathi et al.
(1993). For the flow inside the porous region we use this
representation given by
VI = CurlCurl(rAI ) + Curl(rB I ), (17)
Y
*
p I = p0 + [r(∇ 2 − 2 )AI ], (18)
Fig. 2. Model of the problem considered. *r
4484 A. Bhattacharyya, G.P. Raja Sekhar / Chemical Engineering Science 59 (2004) 4481 – 4492
where 2 = k1 , p0 is a constant and AI , B I are the scalars that n , n , n , Anm , Bnm , Cnm and Dnm are known constants.
satisfy ∇ 2 (∇ 2 − 2 )AI = 0 and (∇ 2 − 2 )B I = 0 and r is the Also A0 and B0 satisfy ∇ 4 A0 = 0 and ∇ 2 B0 = 0. Now due
position vector. In fact Manas-Zloczower et al. (2001) have to the presence of the porous body the modified flow in the
used this representation while discussing the stress distribu- liquid region r > a is represented by
tion inside a partially infiltrated porous sphere of uniform ∞
permeability k, in various linear flow fields (simple shear, AI I = {n r n + n r (n+2) + n r −(n+1)
planar elongation and uniaxial extension). n=1
For the velocity and pressure outside the porous sphere, +n r −(n−1) }Sn (, ), (25)
which are due to Stokes flow, we use the following repre-
sentation: ∞
BI I = {n r n + n r −(n+1) }Tn (, ), (26)
II II II
V = CurlCurl(rA ) + Curl(rB ), (19) n=1
The boundary conditions given in Eqs. (14)–(16) on the −pv(3 + a ) + f s(3 + a ) − a (qv + gs)
T=4a 2
impermeable boundary r = b can be written in terms of {s(f − g) − v(p + q)}
scalars AI and B I as follows: ×[∇ × Q0 ]0 (43)
AI (b, , ) = 0, (35) where Q0 is the velocity corresponding to the basic flow and
[ ]0 is the evaluation at the origin r = 0. p, q, v, s, f , g are
*AI defined in the Appendix. If the basic flow is irrotational then
(b, , ) = 0, (36)
*r the torque vanishes, which agrees with example (ii) given
in Section 5. Now if we take the limit k → 0 and a = b the
B I (b, , ) = 0. (37) expressions for drag and torque for the ‘porous core’ given
in Eqs. (42) and (43) reduce to
Now using these boundary conditions, we have to deter-
mine the unknown co-efficients in expressions (25)–(28). D = 6a[Q0 ]0 + a 3 [∇ 2 Q0 ]0 ,
While doing this we get a system of nine equations in nine
unknowns. We have solved the system using Mathematica T = 4a 3 [∇ × Q0 ]0
version 4.2. Solving them gives a cumbersome expressions
of these unknown coefficients in terms of the known co- which are the corresponding ones for an arbitrary Stokes
efficients n , n and n . Since our immediate concern here flow past a solid sphere.
is to discuss examples for particular flows and to derive
the corresponding Faxen’s laws (1924) which give drag and
torque acting on the porous core, we have given the unknown 5. Examples
coefficients wherever it is necessary.
Here we discuss few examples. Generally, a simple phys-
ical model is when the basic flow is due to uniform flow.
4. Faxen’s laws for a porous core In case of electromagnetic field theory application, etc., the
simplest situation is when the basic field is potential. There-
Faxen’s laws (1924) provide us expressions for computing fore by considering irrotational flow as basic flow one can
drag and torque. For a spherical surface r = a, the force drag study some applications related to electromagnetic theory.
D exerted on the surface r = a by the fluid and the torque Then the complex situations would be when the flow is gen-
T are given by erated by a source or a sink or a combination of them. Hence,
2
keeping this in view we discuss the following examples. The
examples are discussed with a configuration such that the
D= [Trr êr + Tr ê + Tr ê ]r=a
0 0 origin of the ‘porous core’ is located at (0,0,0).
×a 2 sin d d, (38) (i) Uniform flow along OX. Consider uniform flow U
along x-direction.
2
The basic flow is given by (A0 , B0 ) where
T= [rT r ê − rT r ê ]r=a a 2 sin d d, (39)
0 0 U
A0 = r cos , (44)
We now derive the corresponding Faxen’s laws which pro- 2
vide expressions for the drag and torque acting on the porous
B0 = 0 (45)
body in an unbounded arbitrary Stokes flow. TrrI , TrI and
TrI are computed using the expression given in Eqs. (5)–(7) for which
and are used in Eqs. (38), (39) to get the following expres- U
sions for drag and torque as 1 = ,
2
D = −8(A11 î + B11 jˆ + A10 k̂)1 , (40) 1 = 0.
T = −8(C11 î + D11 jˆ + C10 k̂)1 . (41) Hence using Eqs. (40) and (41), drag and torque are given by
Here L U
D = −8 î, (46)
L M De 2
1 = 1 + and 1 = −K 1 ,
De De 1 T = 0. (47)
where L , M, De and K are given in the Appendix. The variation of drag with permeability for different values
Therefore, the drag and torque reduces to the following of the stress jump coefficient has been plotted. As per
form: Ochoa-Tapia and Whitaker, the values of ranges from −0.9
L 2 M 2 to 0.9. Therefore, we have plotted for some negative values
D = −4 [Q0 ]0 − [∇ Q0 ]0 , (42) and some positive values within the range −0.9 to 0.9.
De 5 De
4486 A. Bhattacharyya, G.P. Raja Sekhar / Chemical Engineering Science 59 (2004) 4481 – 4492
400
120
100 300
80 (iii)
200
60
(ii) (i)
100
40 Drag
Drag (iii)
(ii)
20
10 20 30 40 50
-100
10 20 30 40 (i) 50
Permeability k
Permeability k
Fig. 5. Variation of drag with permeability for uniform flow when thickness
Fig. 3. Variation of drag with permeability for uniform flow when a = 4, of the porous region (i) a = 4, (a − b) = 3, (ii) a = 6, (a − b) = 5, (iii)
(i) = −0.9, (ii) = −0.5, (iii) = −0.3. a = 11, (a − b) = 10.
11.5 6 13.1 6
9.51 10.1
7.51 8.03
4 6.03 4
80 4.51
3.51 4.03
2.51
1.51
0.50
2 2.05
1.05 2
0
Y
0
Y
60
-2 -2
-4 -4
40 (iii) -6 -6
(ii) (i) -6 -4 -2 0 2 4 6 -6 -4 -2 0 2 4 6
(i) X (ii) X
Drag
20 6
12.8
10.8
8.8
6.8
4.8
4
2.8
1.8 2
0.8
10 20 30 40 50
Y
Permeability k 0
-2
Fig. 4. Variation of drag with permeability for uniform flow when a = 4,
(i) = 0.3, (ii) = 0.5, (iii) = 0.9. -4
-6
-6 -4 -2 0 2 4 6
(iii) X
Here drag decreases as the permeability increases and
it is observed from Figs. 3 and 4 that as the stress jump Fig. 6. Streamlines for uniform flow with k = 10, a = 5, (a − b) = 4, (i)
coefficient increases from −0.9 to 0.9 the rate at which = −0.5, (ii) = 0, (iii) = 0.5.
the drag is decreasing has been reduced. Also, if we see
closely, for negative values of , the magnitude of the drag
is smaller than that of the positive values of . Also the of the porous body are related as follows:
variation of drag with permeability for different thickness
18.32 Q∞ = −0.9,
d = (a − b) of the porous region has been plotted. If we see
Fig. 5, in general as permeability increases the magnitude
19.02 Q∞ = −0.5,
of drag decreases. But the variation of drag also depends on
Q0 = 20.2 Q∞ = 0, (48)
the thickness of the porous region. As the thickness of the
porous region increases the rate at which drag is decreasing
21.6 Q∞ = 0.5,
has been reduced.
23.2 Q∞ = 0.9
Here streamlines are plotted in case of uniform flow. If
we observe Fig. 6(i)–(v) for a fixed thickness of the porous which means that as increases there is an increase in the
region d = (a − b) = 4 cm, when the permeability is as large volume flow coming inside porous body.
as k = 10 cm2 , the volume flow coming inside the porous In Fig. 7(i)–(v), the streamlines are plotted for k = 10 cm2
region Q0 and Q∞ that flows into the same region in absence and for small thickness d = (a − b) = 1cm. Here Q0 and
A. Bhattacharyya, G.P. Raja Sekhar / Chemical Engineering Science 59 (2004) 4481 – 4492 4487
9.26
6 9.35 6 8.07 6 6
7.26 7.35 7.07 8.12
6.07 7.12
5.26 5.35 5.07 6.12
3.26
4 4.35 4 4.07 4 5.12
4.12 4
2.35 2.07 3.12
2.26
2.12
1.26 2 1.35
2 1.07
2 1.12 2
0.35
0.07 0.12
Y
0
Y
0 0
Y
0
Y
-2 -2 -2 -2
-4 -4 -4 -4
-6 -6 -6 -6
-6 -4 -2 0 2 4 6 -6 -4 -2 0 2 4 6 -6 -4 -2 0 2 4 6 -6 -4 -2 0 2 4 6
(i) X (ii) X (i) X (ii) X
6 6
8.46 8.26
7.46 7.26
5.46 6.26
4.46
3.46
4 4.26 4
2.46
2.26
1.46
0.46
2 1.26
2
0.26
0 Y 0
Y
-2 -2
-4 -4
-6 -6
-6 -4 -2 0 2 4 6 -6 -4 -2 0 2 4 6
(iii) X (iii) X
Fig. 7. Streamlines for uniform flow with k = 10, a = 5, (a − b) = 1, (i) Fig. 8. Streamlines for uniform flow with k = 0.02, a = 5, (a − b) = 4,
= −0.5, (ii) = 0, (iii) = 0.5. (i) = −0.5, (ii) = 0, (iii) = 0.5.
Y
15.10 Q∞ = 0.9.
Even when the thickness of the shell is small the volume -2
flow coming inside increases as the value of increases.
But, since the thickness of the porous region is small, the
-4
streamlines experience the effect of the rigid core much early
and would be deviated, which results in a smaller volume
flow compared to the larger thickness. -6
-6 -4 -2 0 2 4 6
In Fig. 8(i)–(v), the streamlines are plotted for very small X
permeability k = 0.02 cm2 and for the larger thickness (a −
b)=4 cm. Here also as in the earlier cases there is an increase Fig. 9. Streamlines for uniform flow with k = 0.02, a = 2, (a − b) = 0.5.
in the volume flow Q0 coming inside the porous region
which can be seen from
d = (a − b) =
,
< 1, with small permeability k = 0.02
14.10 Q∞ = −0.9, the entire body is almost like a solid sphere and hence the
streamlines deviate much early.
14.14 Q∞ = −0.5,
(ii) Two dimensional irrotational flow. Let the flow at
Q0 = 14.24 Q∞ = 0, (50) infinity be given by the following cartesian components of
velocity:
14.52 Q∞ = 0.5,
16.52 Q∞ = 0.9. u = x, (51)
In terms of A0 and B0 the basic flow is given by direction of the x-axis. The corresponding expressions for
2 2 A0 and B0 in terms of spherical harmonics are
A0 = r P2 ( ) cos 2, (54) ∞
18 F1
A0 =
B0 = 0 (55) 8
n=1
for which r (n+2) (n − 2)r n
× −
(n + 1)(2n + 3)c (n+2) n(n + 1)(2n − 1)cn
1 = 0, (56)
×Pn1 ( ) cos , (68)
1 = 0, (57)
∞
F1 rn
2 = , B0 = Pn1 ( ) sin . (69)
18
(58) 8 n(n + 1)c(n+1)
n=1
2 4
1.75
3
1.5
2 (iii)
1.25 (iii)
Torque
Drag 1 (ii)
10 20 30 40 50
0.75 (ii)
(i) 10 20 30 40 50
0.5 (i)
Permeability k Permeability k
Fig. 10. Variation of drag with permeability for stokeslet when thickness Fig. 13. Variation of torque for stokeslet with permeability when thickness
of the porous region (i) a = 4, c = 5, (a − b) = 3, (ii) a = 6, c = 7, of the porous region (i) a=4, c=5, (a−b)=3, (ii) a=6, c=7, (a−b)=5,
(a − b) = 5, (iii) a = 11, c = 12, (a − b) = 10. (iii) a = 11, c = 12, (a − b) = 10.
0.4
0.25
0.3
(iii) 0.2
0.2 (ii)
0.15
0.1
Drag 0.1
10 20 30 40 50 Torque
Fig. 11. Variation of drag with permeability for stokeslet when a = 4, Permeability k
c = 5 (i) = −0.9, (ii) = −0.5, (iii) = 0.3.
Fig. 14. Variation of torque for stokeslet with permeability when a = 4,
c = 5 (i) = −0.9, (ii) = −0.5, (iii) = −0.3.
0.35
∞
Torque for stokeslet. Here the variation of torque with per- F2 rn
meability for different thickness of the porous region has A0 = − Pn1 ( ) sin , (75)
8 n(n + 1)c(n+1)
been plotted. It is observed from Fig. 13 that torque de- n=1
4490 A. Bhattacharyya, G.P. Raja Sekhar / Chemical Engineering Science 59 (2004) 4481 – 4492
0.1
10 20 30 40 50
(i)
10 20 30 40 50
-0.1
(i) (ii)
(ii)
(iii) -0.1
-0.2 (iii)
Torque
-0.2
Torque
-0.3
-0.3
Permeability k
-0.4
Permeability k
Fig. 16. Variation of torque for rotlet with permeability when thickness of
Fig. 15. Variation of torque for stokeslet with permeability when a = 4, the porous region (i) a =4, c=5, (a −b)=3, (ii) a =6, c=7, (a −b)=5,
c = 5 (i) = 0.3, (ii) = 0.5, (iii) = 0.9. (iii) a = 11, c = 12, (a − b) = 10.
∞
F2 rn
B0 = − Pn1 ( ) sin . (76)
8 (n + 1)c(n+2) 10 20 30 40 50
n=1
-0.01 (ii) (iii)
Comparing these form of A0 and B0 with Eqs. (18) and (19) (i)
we get n , n and n as follows: -0.02
F2 1 -0.03
n = − , (77)
8 n(n + 1)c(n+1)
Torque -0.04
n = 0, (78)
-0.05
F2 1
n = − . (79) -0.06
8 (n + 1)c(n+2) Permeability k
Similarly, in this case also from the expressions n , n and Fig. 17. Variation of torque for rotlet with permeability when a = 4, c = 5
n we can get the values of 1 , 1 and 1 and compute 1 (i) = −0.9, (ii) = −0.5, (iii) = −0.3.
and 1 . Hence the drag and torque in this case are as follows:
F 2 L 0.1
D= î, (80)
3c2 De
F2 0.08
T=
2c3
−pr(3 + a ) + f s(3 + a ) − a (qr + gs) ˆ 0.06
× j,
{s(f − g) − r(p + q)}
(81) 0.04
(iii)
Torque
where L , De, p, q, r, s, f and g are given in the Appendix.
(ii) (i)
Then for positive values of torque first increases and then tion of drag on the porous surface gives useful information
decreases in magnitude along positive x-axis as increases in several chemical engineering processes like chemical ag-
from 0 to 0.9. Here the value of critical permeability de- glomerations, gas–solid reaction system(Levenspiel, 1972),
creases as increases. etc. In chemical agglomeration this drag force can initiate
the agglomeration and as the porous particles agglomerate
more, the filtration will be good. In gas–solid reaction for
6. Discussion and conclusion the case of a cylinder type reactor when gas and porous par-
ticles enter into the tube from the same direction dead zone
In this paper we have discussed an arbitrary viscous flow is expected inside the tube where gas is unable to reach the
past a porous sphere of radius ‘a’ with an impermeable core solid surface to initiate the reaction. Then manipulating the
of radius ‘b’ by considering Brinkman equation in the porous drag force, one can avoid the dead zone and get a well-mixed
region and Stokes equation in the liquid region . At the condition in the reactor so that reaction is uniform. Also the
porous–liquid interface stress jump boundary condition for above finding may have potential applications in colloid sci-
tangential stresses, continuity for normal stresses and con- ence. Hence the present study has useful implications in the
tinuity of velocity components have been used. The effect above mentioned chemical engineering processes.
of the stress jump coefficient on various flow quantities like
volume flow, drag, torque has been observed for different
flows viz. uniform flow, two dimensional irrotational flow, Appendix A
doublet in a uniform flow, stokeslet and rotlet. In particu-
lar when the basic flow is uniform flow we have analyzed L = − a 2 [3b2 (−3pv + 3f s + bf u + bpt)
the flow field with varying permeability as well as varying − 9ab2 2 (pv − f s + qv + gs) + 3ab3 3
thickness of the porous region and studied the effect of the (pt + qt + f u − g u) + 2a 4 {32 (p + q)t
stress jump coefficient . It is observed that there is a signif-
icant effect of on the volume-flow. It is noticed that as + 32 f u − 3g 2 u} + 6a 3 2 (pt + f u)],
increases the volume flow coming inside the porous region
M= − a 2 [10a 5 2 (2qt − 2gu + f u + pt)
Q0 is increased compared to Q∞ which is the volume flow
coming inside the same region in absence of the ‘porous + 10a 6 3 (pt + f u + qt − gu) + 5a 2 b2 {−6qv
core’. But, when the thickness is small, eventhough Q0 in- − 6gs + 2bq t + 6st − 2bgu + 6vu
creases as increases, when compared to the case of large + (−3pv + 3f s + bpt + bf u)}
thickness it is small. As far as the behavior of the drag is con-
+ ab2 {60(qv + gs − st − vu) − 20b(qt − gu)}
cerned, when the basic flow is uniform flow or two dimen-
sional irrotational flow, drag decreases with the increasing + 2a 4 {10t (3p + q) − 30f (q − u) − 10g(3p + u)}
permeability, but as the thickness of the porous region in- + a 3 {5b2 2 (p + q)(bt − 3v) + 60pt
creases the rate of decrease is reduced. When the basic flow − 5g (12p + 3b2 2 s + b3 3 u) + f (5b2 2 (3s + bu)
is due to a stokeslet or a rotlet,with the increase of perme-
+ 60(u − q))}],
ability drag first decreases and then increases in magnitude.
If we define the permeability where drag changes its behav- De=2[2a 4 2 (gu − qt + f u − pt) + 2a 5 3 (pt + f uqt
ior as ‘critical permeability’, it is noticed that the value of the
critical permeability is decreasing as increasing. In case − g u) + b2 (3qv + 3gs − bqt
of torque, when the basic flow is due to a stokeslet, torque − 3st + bg u − 3vu)
decreases and then increases in magnitude and as is in- + ab2 (3qv + 3gs − bqt − 3st + bg u − 3vu
creasing the value of critical permeability is decreasing. But + (−3pv + 3f s + bpt + bf u)}
when the basic flow is due to a rotlet torque first increases
+ a 3 {−3f q + 3pt + qt + 3f u − g(3p + u)}
and then decreases. Here as increases the value of critical
permeability decreases. Hence, it is felt that there is a sig- + a 2 {−3b2 2 pv − 3b2 2 qv + b3 3 pt + 3pt
nificant effect of the stress jump coefficient on the flow + b3 3 qt − g (3p + b2 2 (3s + bu))
quantities discussed above like volume flow, drag and torque
+ f (−3(q − u) + b2 2 (3s + bu))}]
when the basic flow is due to some particular flows given in
examples. Therefore while studying viscous flow problems and
involving Brinkman equation in porous media and Stokes −pv(3 + a ) + f s(3 + a ) − a (qv + gs)
equation in clear fluid region, one has to take the stress jump 1 = − a 2 1
{s(f − g) − v(p + q)}
in the tangential stress components into consideration, which
has a significant impact on the physical problem. Also, this with
helps us to estimate the flow quantities more accurately and f = f1 (a), g = f0 (a), p = g1 (a), q = g0 (a),
to realize the dependency of the physical problem on the
boundary conditions. In particular the findings on the varia- v = f1 (b), s = g1 (b), t = f0 (b), and u = g0 (b).
4492 A. Bhattacharyya, G.P. Raja Sekhar / Chemical Engineering Science 59 (2004) 4481 – 4492
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