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Composite Structures 201 (2018) 79–85

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Composite Structures
journal homepage: www.elsevier.com/locate/compstruct

Interlaminar failure behavior of GLARE laminates under double beam five- T


point-bending load

Yanyan Lina,1, Cheng Liua,1, Huaguan Lia, Kai Jinb, Jie Taoa,c,
a
College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, PR China
b
College of Mechanical and Electrical Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, PR China
c
Jiangsu Collaborative Innovation Center for Advanced Inorganic Function Composites, Nanjing 210016, PR China

A R T I C LE I N FO A B S T R A C T

Keywords: GLARE laminates were prepared in this work to characterize their interlaminar shear failure behavior by Double
DBS method Beam Shear (DBS) method. The effect of span-to-thickness ratio (L/h ratio) and lay-up configuration on the
GLARE interlaminar failure feature of the laminates was investigated respectively. The results indicated that the failure
ILSS values mode in DBS method was single interlaminar shear delamination due to the existence of pure shear stress points.
Interlaminar shear delamination
Furthermore, the apparent interlaminar shear strength (ILSS) values measured by DBS method were higher than
those of Short-beam Shear (SBS) method, which were closer to the true value. However, the two methods did not
show exclusiveness.

1. Introduction reliable method to evaluate the interlaminar shear resistance of GLARE,


the Double Beam Shear (DBS) method could be introduced. G. Zhou
GLARE, consisting of alternative layers of thin aluminum alloy et al. from Loughborough University conducted DBS method to char-
layers and glass/epoxy composites layers [1], has found its important acterize the apparent interlaminar shear properties of resin matrix
application in aeronautics industry due to excellent fatigue, impact and composites [17]. They found that the DBS method guaranteed inter-
damage tolerance. However, debonding and delamination may develop laminar shear failure between two pure shear points by promoting the
between fiber/epoxy and metal layers in the case of bending load or dominance of interlaminar shear strength (ILSS). Unlike the homo-
torsion, representing the typical failure modes of Fiber Metal Laminates geneous resin matrix composites, GLARE laminates possess multiple
(FMLs) [2–5]. Apparently, an appropriate evaluation method for in- interfaces, including the interfaces between aluminum alloy sheet and
terlaminar shear resistance plays a key role in the quality control of matrix, fiber and matrix, composite and aluminum alloy sheet [18].
FMLs [6]. Researchers mainly used Short-beam Shear (SBS) method Consequently, the fixture for evaluation of interlaminar shear behavior
(ASTM-D2344) to measure the interlaminar shear behavior of GLARE should be designed and the key parameters (L/h ratio and lay-up con-
laminates [7–9] because a standard test method to estimate the inter- figuration) should be considered.
laminar shear properties of GLARE has not been established [10–12]. In this paper, failure mode was evaluated to determine the effective
However, the span-to-thickness ratio (L/h ratio) of 4 or 5 is usually interlaminar shear failure for GLARE laminates under double beam five-
chosen according to ASTM-D2344 [13], which is inappropriate for point-bending load. The influence of the L/h ratio and the lay-up con-
GLARE laminates. The main reason is that the SBS method is only ap- figuration on the interlaminar shear failure behavior and mechanisms
plicable to the high-modulus fiber-reinforced composite materials under DBS method were investigated. Finally, the respective failure
[14,15]. Thus, we have already investigated the interlaminar failure characteristics and apparent interlaminar shear strength of GLARE la-
behavior of GLARE-3/2-0.3 laminates under short-beam three-point- minates under DBS and SBS methods were compared.
bending load, and found that specimens with L/h ratio of 8 yielded a
relatively accurate interlaminar shear strength value [16].
Theoretically speaking, the interlaminar shear strength value of
GLARE obtained by SBS method is smaller than true value due to the
unavoidable influence of bending stress. Aimed at finding a more


Corresponding author at: College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, PR China.
E-mail address: taojie@nuaa.edu.cn (J. Tao).
1
These authors contributed equally to this work.

https://doi.org/10.1016/j.compstruct.2018.06.037
Received 14 September 2017; Received in revised form 16 May 2018; Accepted 7 June 2018
Available online 15 June 2018
0263-8223/ © 2018 Elsevier Ltd. All rights reserved.
Y. Lin et al. Composite Structures 201 (2018) 79–85

Table 1 33P
τ=
The fundamental performance of the Aluminum alloy (2024-T3). 64bt (1)
Thickness Elasticity Coefficient of Yield Tensile
where P represent the load in response to the occurrence of delami-
(mm) modulus thermal expansion strength strength
(GPa) (°C) (MPa) (MPa) nation, b and t denote the average measuring width and thickness of the
specimen, respectively.
0.3 73.1 22.68 × 10−6 305 455 Indeed, the Eq. (1) is based on the assumption that the interlaminar
shear failure occurs at the centreplane when the shear stress reaches the
maximum. However, the centreplane for GLARE laminates is the alu-
2. Experimental
minum layer and its shear strength is larger than that between the
aluminum sheets and GF/EP layer. We still used the formula applied for
2.1. Materials preparation
homogeneous material due to the following reasons.
Firstly, according to our experimental results below, the debonding
The Aluminum alloy plates was 0.3 mm thick layers (2024-T3)
is near the centreplane instead of the other interface between aluminum
supported by Southwest Aluminum (Group) Co., Ltd, and the funda-
sheets and GF/EP layer. The error is quite limited in this situation.
mental performance of the Aluminum alloy plates is given in Table 1.
Secondly, the values deflection of ILSS also exists in this kind of ma-
Moreover, the surface treatment of the aluminum layers was conducted
terial, including fiber composite material, because the bending stress is
to achieve a better bonding with the fiber reinforced composites. The
unavoidable. It is the reason that interlaminar shear strength obtained
phosphoric acid anodizing (H3PO4 140 g/L, 25 °C, 10 V, 20 min) was
by these methods is still called the apparent ILSS. Actually, the newly
adopted to construct a rough surface. The high strength glass fiber
developed DBS method is less affected by bending stress than the tra-
(HS4) was provided by Nanjing Glass Fiber Research Institute and the
ditional SBS method. In this way, the relatively more accurate results
high temperature epoxy resin (E302-2) was provided by Sichuan Xin-
could be obtained. Thirdly, the stacking structure of all the GLARE la-
wanxing Carbon Fiber Composites Co., Ltd, and the fundamental per-
minates analyzed in this work was 3/2 configuration. There are some
formance of the S4-glass/epoxy composites is listed in Table 2. Alu-
additional structures in GLARE, like 4/3, 5/4, etc. We intended to seek
minum alloy plates with a thickness of 0.3 mm, S4-glass/epoxy
a relatively reasonable evaluation methodology that could be widely
composites consisting of two unidirectional prepregs with a nominal
used in fiber mental laminates. For the sake of the unity of the formula,
thickness of 0.125 mm were used in constituent materials of alleged
we referred to the formula for calculating the ILSS of homogeneous
GLARE-3/2-0.3 [19]. Four kinds of laminates were prepared as follows:
material.
GLARE 2A-0/0-0.3, GLARE 3-0/90-0.3, GLARE 4A-0/90/0-0.3 and
GLARE 6- ± 45-0.3. Specimens with dimensions of 40 mm × 10 mm
were cut from the massive FMLs by using wire electrical discharge
3. Failure behavior and mechanisms
machining (WEDM) technique. Additionally, to achieve a better po-
lished surface, all specimens were processed by carbide end milling
3.1. Failure mode and mechanisms
cutter [20]. Each group contained five qualified specimens without
interfacial debonding.
Compared to the multiple failure mode of GLARE laminates in SBS
method, it is single expression of interlaminar shear delamination in
2.2. Experiment procedures DBS method. In Fig. 3, the specimens on both sides have no evident
shear failure. Near the neutral layer, between the two indenters and
Double Beam Shear method is not the standard method for inter- intermediate holder, effective interlaminar shear failure at the interface
laminar shear test of composite materials, and the corresponding fixture of aluminum alloy and composite layer occurs in four kinds of GLARE.
cannot be acquired directly. Therefore, the five-point-bending fixture The reason is that the large residual stress caused by the difference in
was designed for DBS method as shown in Fig. 1(a) and the dimensions the coefficient of expansion exists in the interface, where is prone to
of the indenter are illustrated in Fig. 1(b). The material chosen for generate failure [24]. However, the existence of pure shear stress points
fixture is Cr12MoV, which is widely utilized in the production of weakens the influence of bending stress on failure behavior, which
standard tools and gauges. Convenient to adjust the indenters and the causes the specimens to fail under the small displacement. Namely, the
holders, the rail type is designed for the precise control of L/h ratio. whole shear failure process is completed near the elastic section, and no
Fig. 2(a) shows that the double beam five-point-bending test is large local compression deformation occurs.
conducted in a beam specimen of rectangular cross section symme- As can be seen clearly from the Fig. 4, the typical failure process of
trically supported by three holders and loaded by two indenters, which GLARE-3/2 under DBS method present two-stage failure, which could
the distance (L) between the two holders is equal to the indenter span. be divided into four parts. The first part is an elastic section, and the
The five-point-bending test is named as DBS method since two short GLARE specimen shows an elastic deformation at this stage, that is,
beams are formed by three equidistant holders. It also needs to choose after unloading the applied load, the sample can be completely re-
the appropriate span-to-thickness ratio, so that the effective inter- covered without any failure. Before the peak load occurs, the yield of
laminar shear failure occurs when the specimen is subjected to a small aluminum sheets causes the sample enter the plastic deformation stage.
bending disturbance [21]. The existence of two pure shear points in the Due to the excellent interfacial bonding of the GLARE laminates, the
beam specimen can assure pure shear stress under double beam five- bonding effect between glass fiber reinforced composite layer and
point-bending load [22], as indicated in Fig. 2(b). In addition, the aluminum alloy layer continues to maintain good adhesion, and the
loading rate of the experiment is 1 mm/min. According to DBS method specimen does not show any failure. Because of the interfacial de-
theory for homogeneous material [23], the interlaminar shear strength bonding, the curve indicates a sharp decline when the applied load
is given by reaches the maximum and at this point, the calculated ILSS is the ap-
parent interlaminar shear strength. Subsequently, the applied load in-
Table 2
creases at a relatively small slope until the end of the debonding failure
The fundamental performance of the S4-glass/epoxy composites.
to further overcome the interfacial cohesion. In the last stage, the la-
Surface Density (g/cm3) Resin content (wt%) Thickness (mm) Width (mm) minates were in bending deformed state after the failure subjected to
the transverse shear stress completion.
170 ± 5 30 ± 2 0.125 ± 0.05 1000

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Y. Lin et al. Composite Structures 201 (2018) 79–85

Fig. 1. (a) The design sketch of fixture for DBS method, (b) the dimension parameter of indenter for DBS method. Dimensions are in millimeters.

Fig. 4. Typical failure process of GLARE-3/2 under DBS method.

Fig. 2. (a) The apparatus for the double beam five-point-bending test, (b) Stress
analysis in DBS method.

Fig. 3. Typical failure mode of GLARE-3/2 under DBS method.

3.2. Influence of L/h ratio on interlaminar shear failure behavior Fig. 5. The correlation between apparent ILSS and L/h ratios for GLARE.

The correlation between apparent ILSS and L/h ratio for various lay- tends to be gentle after the L/h ratio is 6, and when the L/h ratio arrives
up configuration is proved in Fig. 5. Experimental results illustrate the at 7, there is no obvious decline in apparent ILSS values. The reason for
fact that ILSS values drop with the increase of L/h ratio. The inter- such trend in different lay-up configuration can be attributed to the
laminar shear strength obtained by DBS method is still called the ap- analogous crisscross fiber stacking, which possesses better bending
parent ILSS due to the slight influence of bending stress. Therefore, it is stress resistance. Accordingly, the large L/h ratio not only alleviate the
necessary to adjust an appropriate L/h ratio to characterize the ap- stress concentration, but also lessen the bending influence on the
parent ILSS of GLARE laminates. Owing to unidirectional fiber stacking measurement of apparent ILSS values.
in GLARE 2A, the apparent ILSS value decreases linearly with L/h ratio The specimens are subjected to bending and shear coupling effect,
increase. It can be concluded that the L/h ratio has a significant effect which is dissimilar with the change of L/h ratio. Fig. 6 depicts the load-
on the failure behavior of unidirectional laminates under the condition deflection curves of various GLARE laminates under four different L/h
of double beam loading. Besides, the apparent ILSS value of GLARE 4A ratios. Under the L/h ratio of 5, the load values of GLARE laminates are
laminates reduces quickly at first and slow down after the L/h ratio is 7. much higher than others and the failure processes are complex. Fiber
However, the decline in apparent ILSS value of GLARE 3 and GLARE 6 breakage and matrix cracking took place, as shown in Fig. 7(a) and (b).

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Y. Lin et al. Composite Structures 201 (2018) 79–85

Fig. 6. The load-deflection curves under four different L/h ratios: specimens of (a) GLARE 2A, (b) GLARE 3, (c) GLARE 4A, (d) GLARE 6.

Although the interlaminar shear stress accounts for a sizeable propor- desirable. In addition, there are perforative cracks along 90°-fiber layer
tion, it is easy to form stress concentration. Owing to the low fracture in Fig. 7(b) and (d). This is caused by the relatively weak adhesion
toughness of resin matrix and glass fibers, the failure was not domi- between resin matrix and glass fibers under the DBS loading condition.
nated by the interlaminar shear delamination, the L/h ratio of 5 was not When L/h ratio is 8, the load-deflection curves of four GLARE

Fig. 7. The failure microgram of GLARE specimens: (a) and (b) for L/h ratio of 5, (c) and (d) for L/h ratio of 8.

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Y. Lin et al. Composite Structures 201 (2018) 79–85

Fig. 8. The load-deflection curves of four different lay-up GLARE specimens: (a) for L/h ratio of 5, (b) for L/h ratio of 8.

variants are of typical two sections, representing the occurrence stable and shear coupling, which is similar to that of SBS method [28]. The
failure of interlaminar shear delamination, as presented in Fig. 7(c) and difference is that the pure shear points exist between intermediate
(d). The first peak is initial debonding formed by the effect of inter- holder and two indenters under double beam five-point-bending load,
laminar shear stress, and the formation of second peak is delamination the effect of interlaminar shear force is stronger than that of bending
between pure shear points. In practice, the results demonstrate that force, the shear failure is not difficult to happen under interlaminar
effective interlaminar shear failure occurs at the first peak, and the shear stress in that region, ensuring the reliability of the test results.
corresponding load values could be used to calculate the apparent ILSS When the influence of bending stress is reduced, the apparent inter-
values of GLARE laminates. laminar shear strength values obtained by DBS method are relatively
larger.
3.3. Influence of lay-up configuration on interlaminar shear failure The mechanical behaviors of four GLARE variants between SBS and
behavior DBS method are compared in Fig. 9. It can be pointed out that the load
value of SBS method is lower than that of DBS method when the L/h
The mechanical behavior of GLARE laminates is mostly influenced ratio is 5 or 8. Although the values in GLARE 2A with two methods are
by the lay-up configuration under the DBS method. Fig. 8 (a) presents considerably different, the failure deflections are close to each other, as
the load-deflection curves of GLARE variants at L/h ratio of 5. Effective presented in Fig. 9(a). This is caused by the fiber direction of uni-
interlaminar shear failure occurs at the first peak. Subsequently, owing directional layers, which is identical with the direction of normal stress
to its low L/h ratio, GLARE laminates are easy to be compressed and and interlaminar shear stress, and the 0°-fiber layers are the main
buckled lacking stability, displaying irregular fluctuation of the load- bearing part.
deflection curves [25]. It is worthy of noting that the mechanical be- Fig. 9(b) shows the load-deflection curves of GLARE 3 under two
havior of all kinds of specimens with different lay-up configurations methods. The failure deflections are almost same when L/h ratio of 5 or
under L/h ratio of 5 is complex. The specimens are subjected to a 8 under double beam five-point-bending load. After the external load
variety of stresses, mainly controlled by interlaminar shear stress, hitting the ultimate bearing of matrix, crack initiated between 90°-fiber
bending stress and shear stress which parallel to the loading direction. layer and aluminum alloy layer, causing interlaminar delamination and
It is shown in Fig. 8(b) that the load-deflection curves of all GLARE matrix cracking phenomenon in 90°-fiber layers. Under two L/h ratios
variants at L/h ratio of 8 are regular. The interlaminar shear failure manner of SBS method, the failure deflections are inconsistent. It in-
occurred at the first peak of the curve, presenting the debonding be- dicates that the stress concentration at L/h ratio of 5 is more profound,
tween the middle aluminum alloy layer and the composite layer. leading to the earlier failure. In addition, the curve presents a fluc-
However, fiber layers are the primary bearing part in GLARE laminates, tuation state at L/h ratio of 5 and a stable expression of two sections at
and the fiber orientation varies in different lay-up configurations, L/h ratio of 8.
which determine the difference in the interlaminar failure feature of The configuration of fiber layer in GLARE 4A is 0°/90°/0°, and the
laminates. Based on the analysis of four GLARE variants, GLARE 4A has two unidirectional fiber layers are the main bearing part in the loading
the largest load value and shortest failure deflection. This is due to the process, leading to excellent interlaminar shear resistance. It can be
highest thickness of GLARE 4A among four GLARE variants, which is concluded in Fig. 9(c) that the load and the deflection values of GLARE
sensitive to the small bending disturbance [26]. Notably, GLARE 2A has 4A are largest than other GLARE variants at equal level. Under double
the largest failure deflection since the unidirectional fiber layers. 0°- beam five-point-bending load, the failure deflections are almost the
Fiber layers play a bridging role in the failure process and effectively same at different L/h ratios. It can be confirmed that the unidirectional
transfer the load [27]. In addition, the failure deflection of GALRE 3 is fiber layers are the principal bearing part during the loading process.
relatively small due to the inclusion of 90°-fiber layers, since they are Obvious damage does not occur in 90°-fiber layers until the ILSS values
not bearing part in the loading process and easy to crack under stress of GLARE 4A reach the shear stress limit.
condition. Moreover, the load and deflection values of GLARE 6 are Fig. 9(d) contains the load-deflection curves of GLARE 6 under SBS
among four of them. ± 45° oblique crossing fiber layers possess better and DBS methods. Among the consequences, the failure deflection at L/
stress distribution, where delamination between inner aluminum alloy h ratio of 8 is higher than that of 5. The debonding between the ± 45°
layer and composite layer happens. oblique crossing fiber layers and the matrix could be alleviated, and the
effect of shear stress would be delayed. However, interlaminar shear
4. Comparison between SBS and DBS methods failure occurs earlier in DBS method due to the dominant position of
interlaminar shear stress.
4.1. Failure characteristics in SBS and DBS methods

The stress state of DBS method attributes to the effect of bending

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Fig. 9. The mechanical behavior comparison between SBS and DBS method: specimens of (a) GLARE 2A, (b) GLARE 3, (c) GLARE 4A, (d) GLARE 6.

4.2. Apparent interlaminar shear strength with SBS and DBS methods ILSS values [29]. SBS method is just simple and convenient in terms of
testing set-up to provide information of quality control and material
The comparison of apparent interlaminar shear strength at L/h ratio screening. In fact, based on the study of GLARE-3/2-0.3 in interlaminar
of 8 with two methods is showed in Fig. 10. It illustrates that the ap- failure behavior, the ILSS values obtained from DBS method are closer
parent ILSS values measured by DBS method are much larger than those to the true values since the smaller influence of unavoidable bending
obtained from SBS method. Particularly, for GLARE 6, the average stress. Besides, the materials involved in DBS methods (specimens with
apparent ILSS value obtained for DBS method is 50.2% greater. In ad- dimensions of 40 mm × 10 mm) are larger than those in SBS methods
dition, it demonstrates that the stability of the consequences in DBS (20 mm × 10 mm). When it comes to evaluating the interlaminar
method is better according to the relatively smaller dispersion degree. failure behavior of GLARE laminates, appropriate test methods could be
This is attributed to the existence of pure shear points in DBS method, selected according to the actual service conditions of samples.
which effectively alleviates the influence of the bending stress on test
results. 5. Conclusions
However, although pure shear failure could happen among the
modified SBS method specimens with well stability at L/h ratio of 8, it (1) Effective interlaminar shear delamination was the single failure
is still severely subjected to bending stress. Thereby, the fiber rupture or mode in this study. The L/h ratio of 8 under DBS method that leads
matrix cracking caused by the bending stress will affect the measured to stable results for the load-deflection curves of four GLARE var-
iants, and the corresponding load values could be used to calculate
the apparent ILSS values of laminates.
(2) The apparent ILSS values measured by DBS method were higher
and more stable than those used in SBS method. The ILSS values
obtained from DBS method were closer to the true values since the
smaller influence of unavoidable bending stress. Appropriate test
methods could be selected according to the actual service condi-
tions of samples.

Acknowledgments

The authors gratefully acknowledge the support from the


Postgraduate Research & Practice Innovation Program of Jiangsu
Province (KYCX17-0259), the financial support of the National Natural
Science Foundation of China (51705235), the Jiangsu Province Natural
Science Foundation (BK20170762), the Fund of China Postdoctoral
Science Foundation funded project (2017M611758), the Key Project of
Fig. 10. Apparent ILSS of SBS and DBS methods at L/h ratio of 8. Key Laboratory of Railway Vehicle Door System in Jiangsu Province

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