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http://dx.doi.org/10.1680/jstbu.16.00153
Fuzzy logic for estimating chloride Paper 1600153
diffusion in concrete Received 07/08/2016 Accepted 26/09/2017
Keywords: concrete structures/materials technology/
Mazer, Lima and Medeiros-Junior mathematical modelling
1 2 3
Chlorides are the agents responsible for starting the process of corrosion of steel reinforcement, thus reducing the
service life of concrete structures, especially in marine environments. The penetration of chloride ions depends on
several factors linked to the nature of the concrete cover and the exposure environment. The diffusion coefficient
may establish the depth of chloride penetration in concrete in a given time and therefore this coefficient is related
directly to the service life of reinforced concrete structures. This paper presents a methodology for determining the
chloride diffusion coefficient using a mathematical model based on fuzzy logic. The following parameters were
considered in the modelling: water/cement ratio, concrete compressive strength and the temperature during mixing
of the concrete. The results show the feasibility of using fuzzy logic for the development of models to estimate the
chloride diffusion coefficient in concrete.
Castellote et al. (2001) pointed out the existence of two types In addition to Fick’s laws, other methods can be used to deter-
of chloride diffusion coefficients – the effective diffusion coeffi- mine the diffusivity of chlorides in concrete. One of these
cient (Def ), determined through steady-state experiments and methods is use of the Nernst–Einstein equations (Lu, 1997),
considering only ionic transportation, and the apparent diffu- which can also be used to evaluate concrete permeability.
sion coefficient (Da), which is determined in non-stationary In addition, the Nernst–Planck and Poisson–Boltzmann
flow experiments and considers the performance of total equations, which describe ionic transportation, may also be
chloride ions. Therefore, the use of Da in prediction models for used (Bourbatache et al., 2012; Friedmann et al., 2004, 2008).
the initiation of the corrosion process in reinforcement is Narsilio et al. (2007) achieved good estimates of the chloride
highly recommended (Andrade, 1993; Castellote et al., 2001; diffusion coefficient using the Nernst–Planck equations and
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
simplified methods, when compared with results from Fuzzy systems have the characteristic of allowing the analysis
migration tests. of often vague and imprecise linguistic terms. Fuzzy set theory
was enunciated in 1965 by Lofti Zadeh (Zadeh, 1965) and has
Choi et al. (2017) presented a model for determining chloride since been applied by researchers to several fields, including
diffusivity in concrete based on capillary porosity. Migration biomedicine and energy (Liu, 2015; Yordanova, 2014). A fuzzy
tests on samples with three different water/binder (w/b) ratios set A in x is characterised by a membership (characteristic)
were used to validate the model. To do this, four ages of con- function fA(x), which associates each point in x to a real
crete were studied and the numerical results were found to be number in the interval [0, 1]. The value of fA(x) represents the
similar to the test data. Pradelle et al. (2017) conducted a sen- ‘grade of membership’ of x in A. Thus, the nearer the value of
sitivity probabilistic analysis of four different chlorides ingress fA(x) to unity, the higher the grade of membership of x in A
models and, as a result, noted the importance of the concrete (Zadeh, 1965).
cover in predicting the service life of structures.
Fuzzy set theory uses concepts similar to ordinary sets, such as
Silva et al. (2017) developed a model for predicting the chlor- empty set, complement set, union and intersection and so on
ide diffusion coefficient based on statistical analysis of 493 (Zadeh, 1965). Zadeh (1968) noted that a fuzzy set may be
case study samples from 43 publications. They concluded that used to solve problems related to information processing,
the main factors affecting the chloride diffusion coefficient control, pattern recognition, system identification, artificial
were mineral additions, the w/b ratio and the cement content intelligence and, more generally, decision processes involving
(Silva et al., 2017). Using factors such as temperature, relative incomplete or uncertain data. A fuzzy set is formally defined
humidity, w/b ratio, cracks and porosity of concrete, Zhang as (Zadeh, 1965)
et al. (2016) developed a model coupling diffusion and convec-
1: Ã ¼ fðx; μA ðxÞÞjx [ X g
tion for the transport of chlorides in unsaturated concrete. The
model produced results that were in accordance with data from
the literature. where X represents the universe of discourse in which the
elements x are defined and μA(x) is the membership function
In search of a better model of the chloride penetration profile, of x in Ã. A universe of discourse represents all elements per-
some researchers have used deterministic or probabilistic taining to the fuzzy set; elements that have a degree of mem-
models to describe the transport mechanism of chlorides in bership greater than zero create the support set (Jantzen,
concrete (Andrade et al., 2013; Bastidas-Arteaga et al., 2011; 1998).
Val and Trapper, 2008). In this context, chaos theory seems to
be a good option for the development of concrete technology The membership function μA(x) defines the degree of member-
models. Another way to model the diffusion process is through ship of a variable within the universe of discourse, and has a
the use of fractals. The flexibility of fuzzy logic is also a good value in the range of [0, 1] (Jantzen, 1998) when the set is con-
feature for working with subjective and qualitative parameters, sidered normal or standardised. Membership functions can
however the physical and chemical parameters of the material take many forms, but trapezoidal and triangular shapes are
still dominate its behaviour. commonly used due to their simplicity.
Models with applications to concrete technology based on a A fuzzy inference system is elaborated, for the most part, from
mathematical approach using fuzzy logic, chaos theory or frac- knowledge built by an expert and it consists of determining
tals are few and quite recent (Altmann et al., 2012; Anoop and which rules will be activated and combined in the system
Raghuprasad, 2012; Anoop et al., 2002) and therefore the (Jantzen, 1998).
development of new models is of interest. To this end, a meth-
odology for the determination of the chloride diffusion coeffi- Shaw and Simões (1999) highlighted the existence of two basic
cient using a mathematical model based on fuzzy logic is types of fuzzy rules – the modus ponens rule (affirmative mode)
presented in this paper. and the modus tollens rule (negative mode). The modus ponens
rule is used in engineering problems, since it keeps the cause–
effect relationship.
2. Basic concepts of fuzzy logic
The expression ‘intelligent systems’ (previously known as Fuzzy sets are applied when it is necessary to evaluate sets
‘artificial intelligence’) is used in a large number of compu- whose elements are not numeric. In such cases, the variables
tational systems. The adjective ‘intelligent’ is used as these are called linguistic variables. For example, in a temperature
systems are created based on human behaviour. However, set, the variables may assume values of low, medium or high,
such a system does not itself present reasoning. Intelligent and each value that a variable can take is represented by a
systems include neural networks, genetic algorithms and fuzzy membership function. The linguistic variables should systema-
systems. tically characterise complex phenomena, badly defined
2
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
phenomena or subjective phenomena (Huang and Ruan, 2.3 Mean of maximum method
2000). Thus, a linguistic variable normally expresses a qualitat- This method consists of using the output. Its value has the
ive value, while the membership functions represent a value greatest pertinence value, as indicated by Equation 4.
quantitatively.
X
N
ui
In order to apply fuzzy set theory, it is first necessary to trans- 4: u ¼
i¼1
N
form the values of the working variables into fuzzy values.
This process, called fuzzification, consists of attributing mem-
bership degrees to each one of the input variables of the
system using the membership functions (Jantzen, 1998). Shaw and Simões (1999) present orientations on how to
choose the best method of defuzzification to be used, accord-
The decision-making process of a fuzzy system involves two ing its purpose of use. For quantitative decision support, the
aspects: (a) the rule base that has all knowledge associated authors recommend the centre of maximum method.
with the application domain, as well as the linguistic rules that
will lead to the decision making; (b) the inference that relates 3. Mathematical modelling
the fuzzy sets of the input and output of the system, using The mathematical model proposed in this paper aims to esti-
information from the rule base (Jantzen, 1998). mate the chloride diffusion coefficient using fuzzy logic, con-
sidering parameters of the concrete (w/c ratio, compressive
After the decision-making process, the obtained fuzzy values strength and concrete pouring temperature). A fuzzification
have to be transformed into real values so that those can be process is used to define the degree of membership of each one
used. In other words, it is necessary to turn a linguistic vari- of these parameters. The relevant membership functions of the
able into a discrete value. This process is called defuzzification output variable are defined based on fuzzy rules in order to
(Jantzen, 1998). perform the defuzzification process. From this step, the chlor-
ide diffusion coefficient (Da) is defined. The fuzzy rules base
Therefore, when designing a system of fuzzy inference it is of the system and the chloride diffusion coefficient values
important to consider that the input data are non-fuzzy or should be set on a number of relevant data, with statistical
precise, as in the case of most practical applications, it then significance, considering the cement type and mineral admix-
being necessary to transform those data into fuzzy sets (fuzzifi- ture used.
cation). After processing the inference system, an answer in a
fuzzy set is obtained and it is then necessary to interpret this 3.1 w/c ratio
result, transforming it into a non-fuzzy or precise value (defuz- An increase in w/c ratio leads to increased concrete porosity,
zification) (Huang and Ruan, 2000). The main defuzzification which affects mass transport properties, including permeability
methods are centre of area, centre of maximum and mean of and diffusivity (Medeiros-Junior and Lima, 2016). To define
maximum methods (Shaw and Simões, 1999). the membership functions and the range of w/c ratios, the
Brazilian standard NBR 6118 (ABNT, 2014) was used. This
2.1 Centre of area method
standard is the most frequently used for concrete design in
This method calculates the centroid of the composed area
Brazil and it sets maximum values of the w/c ratio as a func-
according to Equation 2. This equation represents the fuzzy
tion of the environmental aggression class (EAC) to which the
output term, composed of the union of all rule contributions.
structure is exposed, as shown in Table 1. EAC I refers to a
PN rural or submerged environment, EAC II refers to an urban
ui μout
2: u ¼ Pi¼1
N environment, EAC III indicates a marine or chemically less
i¼1 μout
aggressive industrial environment and EAC IV refers to a
chemically more aggressive industrial environment and tidal
In Equation 2, ui is the position of the centroid of the individ- splash zones. Therefore, according to NBR 6118 (ABNT,
ual pertinence function, μout is the area of the pertinence func- 2014), a structure subjected to the action of chlorides will be
tion and u* is the result of the defuzzification. EAC III or EAC IV depending on the exposure area con-
sidered. The membership functions for w/c ratio are defined in
2.2 Centre of maximum method Equation 5, based on values established by NBR 6118 and
In this method, the discrete output is calculated as a weighted
mean of the maximum, whose weights are given by the vector
of output possibilities, as indicated by Equation 3. Table 1. w/c ratio of reinforced concrete as a function of
environmental aggression according to NBR 6118 (ABNT, 2014)
PN P
ui nk¼1 μ0;k EAC I EAC II EAC III EAC IV
3: u ¼ Pi¼1
N P n
i¼1 k¼1 μ0;k w/c ratio ≤0·65 ≤0·60 ≤0·55 ≤0·45
3
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
1·0
0·9
Grade of membership
considering the linear relationship between w/c ratio and the 3.2 Compressive strength
chloride diffusion coefficient observed by several authors The compressive strength of concrete is related to its porosity:
(Andrade et al., 2013; Sun et al., 2012). Figure 1 shows the as compressive strength increases, concrete porosity and the
membership functions for EAC III and EAC IV. chloride diffusion coefficient are reduced. NBR 6118 (ABNT,
2014) also sets minimum values of compressive strength as a
For EAC III function of the EAC (Table 2), in the same way that it estab-
lishes values for the w/c ratio.
If 045 w=c 055 ! μ ¼ 1
5a: If w=c , 045 ! μ ¼ 0 The membership functions for compressive strength (Equation 6)
If w=c . 055 ! μ ¼ 0 were defined considering the minimum values set by
NBR 6118 for EAC III and EAC IV. The functions are illus-
trated in Figure 2. The curves represent the classes of concrete
defined by NBR 6118 as a function of environmental aggres-
For EAC IV sion corresponding to the action of chlorides. Triangular func-
tions were used to represent the compressive strength since it is
If 030 w=c 045 ! μ ¼ 1 possible that a given value may be part of two distinct sets in
5b: If w=c , 030 ! μ ¼ 0 fuzzy set theory, with different membership degrees, with a
If w=c . 045 ! μ ¼ 0 smooth transition between sets, as illustrated in Figure 2.
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
1·0
0·9
0·8 C30
Grade of membership
0·7 C35
0·6 C40
0·5
0·4
0·3
0·2
0·1
0
25 30 35 40 45 50
Compressive strength: MPa
existing structures from where samples were extracted, the 3.3 Concrete pouring temperature
results of compressive strength testing. The concrete pouring temperature affects chloride ingress in
concrete at early ages. A high curing temperature accelerates
To use the proposed method, in accordance with the compres- the early hydration reactions in Portland cement, but does not
sive strength set in the design, the expressions shown in produce significant long-term effects.
Equation 6 or Figure 2 should be used to set the degree of
membership of this variable; this generates the vector A temperature of 5°C, recommended by the British Cement
B = [b1, b2, b3]. Association as the minimum temperature for concrete pouring
and also used by Peterson et al. (2013) for observing chlorides
For C30 concrete ingress, was considered as the lower limit for the concrete
temperature. Generally, it is not recommended to perform con-
If fck , 275 ! μ ¼ 0 crete pouring at low temperatures because it reduces the
fck 275 hydration rate of the cement, thus harming the concrete prop-
If 275 fck 30 ! μ ¼
6a: 30 275 erties. A temperature of 40°C, as used by Anoop et al. (2002),
fck 30
If 30 fck 35 ! μ ¼ 1 was set as the upper limit because in most research studies con-
35 30
crete moulded in situ is submitted to curing at ambient temp-
If fck . 35 ! μ ¼ 0
erature. The values adopted also cover the variation of normal
temperatures in Brazil.
For C35 concrete The membership functions adopted try to represent a con-
dition where temperatures are considered as low or high, with
If fck , 325 ! μ ¼ 0 a smooth transition between them, adopting a temperature
fck 325 considered as medium for that and using the condition of
If 325 fck 35 ! μ ¼
6b: 35 325 fuzzy sets that allows a value to be part of two distinct sets.
fck 35
If 35 fck 40 ! μ ¼ 1 The membership functions used for variable placement con-
40 35 crete temperature, T, are presented in Figure 3 and defined by
If fck . 40 ! μ ¼ 0
Equation 7.
For T = low
For C40 concrete
If fck , 375 ! μ ¼ 0 If T , 5 ! μ ¼ 0
fck 375 If 5 T 10 ! μ ¼ 1
If 375 fck 40 ! μ ¼
6c: 40 375 7a:
fck 40 T 10
If 40 fck 45 ! μ ¼ 1 If 10 T 20 ! μ ¼ 1
45 40 20 10
If fck . 45 ! μ ¼ 0 If T . 20 ! μ ¼ 0
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
1·0
0·9
Grade of membership
0·8
0·7
0·6 Low
0·5 Medium
0·4 High
0·3
0·2
0·1
0
0 5 10 15 20 25 30 35 40
Concreting temperature: °C
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
1·0
0·9
Grade of membership
0·8
0·7
Low
0·6
Medium
0·5
High
0·4
0·3
0·2
0·1
0
1 × 10–14 3 × 10–14 1 × 10–13 3 × 10–13 5 × 10–13 7 × 10–13 1 × 10–12 3 × 10–12 5 × 10–12 7 × 10–12 1 × 10–11 3 × 10–11
Apparent diffusion coefficient: m2/s
which are defined in Equation 8. Experimental Da values from The criteria for deciding the boundaries in Equations 5–8 and
several studies (Aït-Mokhtar et al., 2013; Kuosa et al., 2013; the shape of the membership functions (triangular and trapezoi-
Peterson et al., 2013) were used to create Figure 4. Those dal forms) were defined based on the Brazilian standard (ABNT,
values were determined in different studies and by different 2014) and recommendations from other fuzzy logic research
methods, and consequently with different precision. It was (Jantzen, 1998). Especially in engineering, triangular and trape-
thus considered imprudent to represent a class by a single zoidal fuzzy set membership functions are sufficiently accurate
maximum value, so an attempt was made to create a transition and have the advantage of simple implementation (Wolkenhauer,
between the classes. Usually, membership functions are defined 2001). Kute and Kale (2013) note that, in Sugeno’s method
from user experience and triangular or trapezoidal functions (Takagi and Sugeno, 1985), the output membership function is a
are usually chosen due to their simplicity; therefore, trapezoi- constant or linear function. Liu et al. (2014) made a consistent
dal functions were adopted in Figure 4. analysis of triangular fuzzy membership functions and many
authors use triangular functions (Chen et al., 2013; Nazari and
For Da = low Milani, 2011; Nieto-Morote and Ruz-Vila, 2011).
If Da 1 1013 ! μ ¼ 1 Initially, the fuzzy vectors for the input variables Fw/c, fck and
Da 1 1013 T (A, B and C) were determined in order to perform the defuz-
8a: If 1 1013 Da 1 1012 ! μ ¼
1 1012 1 1013 zification. The rules possible to be applied were identified in
If 1 1012 Da ! μ ¼ 0 accordance with the fuzzy rules base, considering that the
fuzzy operators used the conjunction ‘and’ the max–min infer-
ence was used to obtain the composition of the output variable
of the fuzzy system. Therefore, combination of the vectors A,
For Da = normal
B and C formed the matrix D and application of the max–min
If Da 3 1013 ! μ ¼ 0
inference generated the vector E. This procedure is presented
in Section 3.5.
Da 3 1013
If 3 1013 Da 1 1012 ! μ ¼
1 1012 3 1013
Finally, the value of the chloride diffusion coefficient was
8b: If 1 1012 Da 3 1012 ! μ ¼ 1
determined by the centre of maximum defuzzification method,
Da 3 1012
If 3 1012 Da 1 1011 ! μ ¼ 1 which consists of a weighted average of the maximum values
1 1011 3 1012
of the output variable membership functions part of the fuzzy
If Da . 1 1011 ! μ ¼ 0
system.
7
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
showed that most of these parameters have non-linear time- max–min inference, there is a pertinence of 0·2 for the two
dependent characteristics. Thus, to produce more realistic pre- membership functions (output variable) are the non-zero values
dictions, the development of time-dependent diffusion coeffi- from Equation 9, defined by the inference rules, so that the esti-
cient models is encouraged. mated chloride diffusion coefficient is given by Equation 10
using the centre of maximum defuzzification method.
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Structures and Buildings Fuzzy logic for estimating chloride
diffusion in concrete
Mazer, Lima and Medeiros-Junior
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