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International Journal of Heat and Mass Transfer 144 (2019) 118581

Contents lists available at ScienceDirect

International Journal of Heat and Mass Transfer


journal homepage: www.elsevier.com/locate/ijhmt

A compact and lightweight liquid-cooled thermal management solution


for cylindrical lithium-ion power battery pack
Yongxin Lai a, Weixiong Wu a, Kai Chen a,⇑, Shuangfeng Wang a,⇑, Chuang Xin b
a
Key Laboratory of Enhanced Heat Transfer & Energy Conservation, Ministry of Education, School of Chemistry and Chemical Engineering, South China University of
Technology, Guangzhou 510640, Guangdong, China
b
Dongguan DRN New Energy Co., Ltd, Dongguan 523775, Guangdong, China

a r t i c l e i n f o a b s t r a c t

Article history: Battery thermal management (BTM) is indispensable to the battery pack of electric vehicles (EVs) for
Received 27 December 2018 safety. Among different types of BTM technologies, liquid cooling shows its superiority with high heat
Received in revised form 12 July 2019 transfer coefficient and low power consumption. However, the previous works paid little attention to
Accepted 13 August 2019
the compactness and weight ratio of liquid-cooled BTM system, which is vital to the specific energy of
Available online 27 August 2019
battery pack. In this study, a compact and lightweight liquid-cooled BTM system is presented to control
the maximum temperature (Tmax) and the temperature difference (DT) of lithium-ion power battery pack.
Keywords:
In this liquid-cooled solution, one thermal conductive structure (TCS) with three curved contact surfaces
Battery thermal management
Cylindrical battery
is developed to cool cylindrical battery. The influences of mass flow rate (mf), inner diameter (d), contact
Liquid cooling surface height (h) and contact surface angle (a) of the TCS are investigated through numerical study. It is
Lightweight found that for the 5C discharge rate process of battery, Tmax can be maintained within 313 K when mf is
Structure design larger than 1  104 kg/s. A weight sensitive factor is defined to evaluate the influences of d, h and a on
DT and the weight of TCS. It is found that d is the most important parameter that influences the weight. h
is the secondary parameter, and a is the parameter with the minimal impact on the weight. Then the val-
ues of d, h, and a are designed to reduce the weight of TCS while maintaining its cooling performance. The
designed TCS can control Tmax under 313 K with DT as 4.137 K. Compared to the original TCS, DP, DT and
the weight are respectively reduced by 80%, 14% and 46% for the designed TCS. Furthermore, the perfor-
mance of liquid-cooled system with parallel TCSs is discussed. The flow distribution among parallel TCSs
is improved through designing the positions of the inlet and the outlet, which enables that Tmax and DT of
battery pack is similar to the ones of a single battery. The present study facilitates the guideline for com-
pact and lightweight design of liquid-cooled battery thermal management system.
Ó 2019 Elsevier Ltd. All rights reserved.

1. Introduction temperature rise and large temperature difference of the battery


pack, causing capacity fade [3], thermal runaway [4] and instability
To relieve the pressure of energy consumption and carbon [5]. Besides, severe operating conditions such as extreme fast-
emissions, the majority of nations are promoting the development charging [6], adverse climate [7] and aging of batteries [8] will
of electric vehicles (EVs). Among various types of batteries, result in excessive heat generation to battery pack. According to
lithium-ion (Li-ion) battery is the most promising power source existing studies, the favorable temperature range for Li-ion battery
for EVs for the advantages of high specific energy, long cycle life is between 298 K and 313 K, and the favorable temperature differ-
and non-memory effect. However, the performance of Li-ion bat- ence (DT) is below 5 K [9–11]. Therefore, an efficient battery ther-
tery is highly correlated with the operating temperature [1]. Dur- mal management (BTM) is fundamental for Li-ion battery to
ing the discharge or charge process, considerable amount of heat guarantee the lifespan, safety and stability.
will be generated through internal resistance effect and exother- The existing BTM technologies mainly include air cooling [12–
mic reactions inside the battery [2]. The heat will lead to high 14], liquid cooling [15–17], phase change cooling [18–20] and
hybrid cooling [21–23]. Moreover, in recent years, some novel
methods have been developed by using ammonia [24], nanofluid
⇑ Corresponding authors. [25], sodium alginate film [26] or hydrogel [27] to dissipate the
E-mail addresses: chenkaihb09@126.com (K. Chen), sfwang@scut.edu.cn heat, providing more feasible options to BTM. With the increase
(S. Wang).

https://doi.org/10.1016/j.ijheatmasstransfer.2019.118581
0017-9310/Ó 2019 Elsevier Ltd. All rights reserved.
2 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581

Nomenclature

T temperature (K) g variation percentage (%)


m weight (g) D change in variable
d inner diameter (mm) c the dimensionless uneven coefficient (1)
h contact surface height (mm)
k thermal conductivity (W m1 K1) Subscripts
mf mass flow rate (kg/s) w water
cp specific heat capacity (J kg1 K1) b battery
DP pressure drop (Pa) ir irreversible
p static pressure (Pa) re reversible
Q heat generation rate (W) r radial direction
V volume (m3) a axial direction
U battery voltage (V) X the considered structural parameters
I discharge current of battery (A) max maximum
R equivalent internal resistance (mX)
L thermal conduction length (m2)
! Acronyms
v velocity vector (m s1) TCS thermal conductive structure
A thermal conduction area (m2) BTM battery thermal management
t time (s)
Li-ion lithium-ion
N the number of parallel flow channels (1) SOC state of charge
CFD computational fluid dynamics
Greek symbols OCV open-circuit voltage
a contact surface angle (°) LCP liquid cold plate
q density (kg m3) HPPC hybrid pulse power characterization
l dynamic viscosity (N s m2)
W weight sensitive factor (1)

of specific energy density, the cooling load of the battery pack gets 5 mW power consumption. An aluminum flat tube was introduced
higher correspondingly. Among various BTM technologies, liquid by Zhang et al. [30] for liquid cooling. On both side of each battery
cooling shows excellent thermal management performance with cell, three aluminum flat tubes were arranged in stagger. To
high heat transfer coefficient and low parasitic power consumption improve the temperature difference of the battery, the flexible gra-
[15]. According to the BTM strategies report by National Renew- phite was added between the cell surface and the flat tubes. The
able Energy Laboratory (NREL) of the U.S., liquid-cooled BTM is results showed that the temperature of the battery was under
the optimal choice for current commercial electric vehicle market 313 K and the temperature difference was effectively reduced by
[6]. In recent years, liquid-cooled BTM technology has become flexible graphite.
more and more popular for EVs. Many commercial EVs such as Compared to prismatic and pouch battery, cylindrical battery
Tesla Model 3, Chevrolet Volt, BYD Song DM and BMW i8 have possesses the superiority of better consistency, more mature craft
employed liquid-cooled BTM technology. and longer lifecycle [31,32]. However, due to the shape of cylindri-
Numerous studies have been done to investigate liquid-cooled cal battery cell, surface thermal contact is not available for conven-
BTM systems. The proposed solutions include two ways, direct liq- tional LCPs. To realize liquid cooling, researchers have designed
uid cooling and indirect liquid cooling. Direct cooling has higher some special structures to construct adequate thermal contact
thermal management efficiency by using mineral oil silicone oil, with the cylindrical batteries. Basu et al. [17] proposed and ana-
etc. However, this method needs more power consumption and lyzed a conduction element sheet made by aluminum with
involves more risk of leakage. After comprehensive comparison 1.5 mm in thick and 44 mm in height. Each 18650-type battery
of different cooling methods, Chen et al. [15] suggested that indi- was contacted with two conduction elements. The conduction ele-
rect liquid cooling was more suitable for practical applications. ment could effectively reduce the temperature difference of the
For prismatic and pouch batteries, sandwiching them by liquid battery. Besides, the maximum temperature rise was controlled
cold plate (LCP) is a prevalent solution to tackle the thermal issue. under 7 K. For the Tesla Model S battery pack, Jiang et al [33] dis-
The generated heat of the battery is transferred to LCPs by thermal cussed the BTM performance of a wavy cooling channel wound
conduction and then is dissipated by liquid coolant inside the mini around the batteries. It is found that increasing liquid flow rate
channels of LCPs by thermal convection. Panchal et al. [16] consid- and heat exchange area were beneficial to the performance of cool-
ered one LCP with a serpentine channel inside for prismatic bat- ing channel. Rao et al. [34] employed the aluminum block with arc
tery. The LCP was assessed at different discharge rates and shape surfaces for 26650-type battery. The camber surfaces of the
boundary conditions. The temperature rise of the battery was well blocks matched the battery surfaces to build enough thermal con-
controlled by this type of LCP at 2C discharge rate. Jin et al. [28] tact arc. The effects of the inlet velocity and the block length on the
proposed a LCP with oblique fins inside for BTM. These fins can cooling performance were carried out by simulation. It was found
re-initialize the boundary layers of the coolant to achieve higher that the performance of the blocks can be improved by varying the
heat transfer coefficient. The experimental and numerical results blocks length linearly. Zhao et al. [35] numerically investigated the
showed that this plate had better thermal management perfor- performance of the liquid-cooled cylinder for 42110-type cylindri-
mance than those conventional straight-channel plates. Lan et al. cal battery. The thermal contact surface was established by filling
[29] developed a novel mini-channel based cooling tube, which the battery cell into each cylinder. In the cylinder, there were num-
can maintain the battery temperature in rational range, with only bers of mini-channels to dissipate the heat. The results showed
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 3

that the cylinder could maintain the maximum temperature under (h) and the contact surface angle (a). These parameters can be
313 K, but it was difficult to make the temperature difference changed to adjust the cooling performance and the weight of the
below 5 K due to the aging effect of the battery. TCS (mTCS).
The above-mentioned works either focus on thermal behaviors For the liquid-cooled BTM system in Fig. 1, the cooling water is
of the battery thermal management system or different cooling distributed by the upper reservoir and then flows into each parallel
methods, while less research has discussed the compactness and TCS. The heat generated by the batteries is transferred to the TCSs
lightweight design for liquid-cooled BTM systems. In practical uti- through heat conduction and dissipated by the cooling water in the
lization, a battery pack with higher specific energy is desirable to channel of TCS, so that the temperature control of battery pack is
achieve longer mile range of EVs. Although liquid cooling shows achieved. The heated cooling water is gathered by the bottom
excellent cooling performance comparing with other BTM tech- reservoir and then leaves the system through the outlet. It can be
nologies, the relatively large weight ratio is an issue needed to observed that the proposed TCS is one of the most important com-
be solved. A compact and lightweight BTM design can improve ponents in the liquid-cooled system, and the parameters of TCS
the specific energy of battery pack and reduce the general weight have significant influence on the thermal performance of the sys-
of finished vehicle. Previous studies have pointed out that energy tem. Therefore, the structure of TCS needs to be designed to
consumption was decreased by 3.3–8% when the weight of vehicle improve the cooling performance and reduce the weight.
got 10% reduction [36,37]. Moreover, the lightweight of the vehicle
enhances the acceleration performance and reduces the braking 2.2. Numerical simulation
length. Department of Energy of America also puts forward a 30%
reduction lightweight plan for EVs [38]. However, the compact To investigate the performance of the TCSs, computational fluid
and lightweight design for liquid-cooled BTM system has been dynamics (CFD) method is introduced. The governing equations are
rarely considered in the existing literature. the continuity equation, the momentum conservation equations
In this study, a liquid-cooled BTM system is designed to realize and the energy equations. For the cooling water, the governing
suitable temperature range and temperature difference for Li-ion equations are expressed as follows.
battery pack. The novelty of the proposed solution concerns a com-
@ qw !
pact and lightweight design for EVs application, improving the þ r  ðqw v Þ ¼ 0 ð1Þ
cooling performance and reducing the weight of battery pack. In @t
the present work, the 18650-type battery cell is introduced and
the 5C high discharge rate process is considered. Experiment is @ ! ! ! !
ðq v Þ þ rðqw v  v Þ ¼ rp þ r  ðlw r v Þ ð2Þ
conducted to obtain the thermal model of the battery cell. A novel @t w
thermal conductive structure (TCS) is proposed to cool the battery
@ !
ðq cpw T w Þ þ r  ðqw cpw v T w Þ ¼ r  ðkw rT w Þ
cell. Based on the numerical method, the influences of mass flow
ð3Þ
rate and structural parameters on the cooling performance and @t w
the weight of the TCS are investigated. Then, the structural param- For the battery cell and the TCS, the governing equations are
eters are designed to reduce the weight of the TCS while maintain- given by
ing its thermal management performance. Finally, the performance
@ Q gen
of liquid-cooled system with parallel TCSs is investigated and is ðq cpb T b Þ ¼ r  ðkb rT b Þ þ ð4Þ
improved through designing the positions of the inlet and the out- @t b Vb
let of the system. The present work is intended to facilitate the
@
guideline for compact and lightweight design of liquid-cooled bat- ðq cpTCS T TCS Þ ¼ r  ðkTCS rT TCS Þ ð5Þ
tery thermal management system, which is beneficial to increasing @t TCS
the mile range of EVs. In Eqs. (1)–(5), q, cp, k and T are density, specific heat, thermal
conductivity and temperature, respectively. The subscripts w, b
and TCS represent the cooling water, the battery and the thermal
!
2. Methodology and simulation conductive structure. v , p and l denote the velocity vector, the
static pressure and the dynamic viscosity, respectively. Qgen and
2.1. A lightweight liquid-cooled BTM system Vb are the heat generation rate and the volume of battery cell.

To realize a long mile range, battery pack comprising dozens of 2.3. Battery model and validation
battery cells is needed for power supply of EVs. In this study, a
liquid-cooled BTM system is proposed to cool battery pack. When discharging, the battery temperature will increase due to
Scheme of the liquid-cooled BTM system is illustrated in Fig. 1. irreversible and reversible heat generation. Generally, the heat
As shown in Fig. 1(a), the battery pack includes 18650-type battery generation can be divided into reaction heat, Joule heat, polling
cells, IC control unit, base plates, and the liquid-cooled BTM sys- heat and side reaction heat. In 1985, Bernardi et al. [39] presented
tem. The liquid-cooled BTM system contains upper reservoir, ther- a lumped model for the heat generation of the battery cell, which
mal conductive structures (TCSs) and bottom reservoir. The upper can be expressed as
reservoir and bottom reservoir are made of engineering plastics to
reduce the weight. The cells are arrayed in staggered structure @U OCV
Q gen ¼ Q ir þ Q re ¼ IðU OCV  UÞ  IT ð6Þ
with constant distance among them. As shown in Fig. 1(b), the TCSs @T
are inserted into the gaps of the cells for a compact size consider- where Qgen is the total heat generation rate of battery cell, Qir and
ation. Each cell is surrounded by three TCSs. In the center of each Qre are the irreversible heat and the reversible heat, respectively. I
TCS, circle liquid channel is set for coolant. To construct effective is the discharge/charge current of battery cell. UOCV is the open-
thermal contact, each TCS is designed with three curved contact circuit voltage. U is the battery voltage. T is the battery temperature
surfaces as shown in Fig. 1(b) and (c). The curvature radius of the and @UOCV/oT is the temperature coefficient of open-circuit voltage.
curved contact surface is identical to the radius of cylindrical bat- During the discharge process, it obtains
tery cell. Fig. 1(c) also shows the main structural parameters of
U ¼ U OCV  IR ð7Þ
TCS, including the inner diameter (d), the contact surface height
4 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581

Fig. 1. The scheme of the liquid-cooled battery management module.

where R is the equivalent internal resistance, including the ohmic Ri qi cpi V i


qb cpb ¼ ð10Þ
resistance and the polarization equivalent resistance. By substitut- Ri V i
ing Eq. (7) into Eq. (6), it obtains
The thermal conductivity of the battery is considered as aniso-
2 @U OCV tropic. The radial thermal conductivity kr and the axial thermal
Q gen ¼ Q ir þ Q re ¼ I R  IT ð8Þ
@T conductivity ka are calculated by the following equations.
where Qre can be endothermic or exothermic depending on the dis- Ri Li
charge stage of battery. kr ¼ ð11Þ
Ri ki =Li
In the present study, the NCR 18650-type cylindrical Li-ion bat-
tery is used and its properties are shown in Table 1. For the lumped
model of the battery, the equivalent density (qb) and the heat Ri Ai ki
ka ¼ ð12Þ
capacity (cpb) are calculated as follows. R i Ai
To identify the heat generation rate of the battery during the
mb
qb ¼ ð9Þ discharge process, the equivalent internal resistance (R) and open
Vb circuit voltage coefficient (@UOCV/oT) of one NCR 18650-type cell
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 5

Table 1
Physical properties of materials inside the battery cell [40].

Thickness (lm) Height (mm) Density (kg/m3) Thermal conductivity (W/(mK)) Specific heat capacity (J/(kgK))
Can 300 65 7800 16.8 478
Separator 22 59 1200 1 700
LiCoO2 92 53 2291.6 1.85 1172.8
LiNiCoMnO2 N/A N/A 1500 5 700
LiC6 87 53 5031.7 5 700
Cathode foil 10 55 2700 200 870
Anode foil 10 57 9000 380 381
Electrolyte N/A N/A 1290 0.45 133.9

Table 2
were measured experimentally. Specifically, R is specified by Polynomial fitting of the equivalent internal resistance (R) in various temperatures.
means of Hybrid Pulse Power Characteristic (HPPC) test under Polynomial fitting of equivalent internal resistance (R) Temperature/
the conditions of various values of SOC (from 1.0 to 0.1 with 0.1 K
intervals) and temperatures (from 293 K to 333 K with 10 K inter- 166 – 1334  SOC + 6559  SOC2 – 293
vals). The experimental results are shown in Fig. 2. It can be seen 16,531  SOC3 + 22,391  SOC4 –
that for each SOC, R decreases as the temperature increases, but 15,496  SOC5 + 4301  SOC6
the tendency is weakened when the temperature increases further. 107 – 793  SOC + 4036  SOC2 – 303
10,514  SOC3 + 14,700  SOC4 –
For example, when T changes from 323 K to 333 K, R changes only
10,480  SOC5 + 2989  SOC6
about 5%. Moreover, for each temperature, R has a relatively con- 66 – 382  SOC + 1962  SOC2 – 313
stant value at the early discharge process (SOC > 0.2) and increases 5181  SOC3 + 7378  SOC4 – 5365  SOC5 + 1559  SOC6
notably at the end of discharge process (SOC < 0.2). Based on the 58 – 355  SOC + 1898  SOC2 – 323
experimental data, R can be incorporated as the function of tem- 5121  SOC3 + 7367  SOC4 – 5374  SOC5 + 1559  SOC6
48 – 233  SOC + 1225  SOC2 – 333
perature and SOC by polynomial fitting. The final expressions are 3263  SOC3 + 4667  SOC4 – 3406  SOC5 + 992  SOC6
shown in Table 2. Based on the data in Table 2, R can be obtained
when T is 293 K, 303 K, 313 K, 323 K and 333 K, respectively. When
the temperature is between two testing temperature of R, it can be
calculated by interpolation method. In addition, when the temper-
ature is above 333 K, the value of R can be represented by the inter-
nal resistance when T = 333 K because R changes little at high
temperature.
The values of UOCV were also measured from 293 K to 333 K for
each SOC, and the values of @UOCV/oT for different SOC were
obtained. The curve of @UOCV/oT is depicted in Fig. 3. Generally,
@UOCV/oT increases from SOC = 1.0 to SOC = 0.5 and then decreases
when SOC is below 0.5. @UOCV/oT can also be summarized as the
function of SOC by polynomial fitting. The fitting expression is
shown as
@U OCV
¼  0:355 þ 2:154  SOC  2:869  SOC2 þ 1:028  SOC3
@T
ð13Þ

Fig. 3. Experimental results of open circuit voltage coefficient (@UOCV/@T) with SOC.

Based on the expressions of R and @UOCV/oT, the heat generation of


the battery can be determined by Eq. (8).
In order to verify the fitting heat generation model, the thermal
behavior of one 18,650 cylindrical battery was experimentally
investigated. The battery with 5C discharge rate process was tested
by a battery testing system (CT-4008-5V10A-204, Shenzhen New-
are Technology Co. Ltd, China) at ambient temperature of 300 K. K-
type thermocouples were arranged at the surface of the battery cell
to measure the surface temperature by Agilent data acquisition
instrument (Agilent 34970 A). During the test, the battery was
wrapped by heat preservation cotton to minimize the heat loss.
The simulation for the same situation as the experiment was con-
ducted. The comparison of the experimental data and the numeri-
cal results are shown in Fig. 4. It can be observed that the
Fig. 2. Experimental results of the internal equivalent resistance (R) with SOC and
experimental data and numerical results coincide very well. The
temperature. maximum temperature error and the average temperature error
6 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581

4. Effects of the parameters on the performance of TCS

The mass flow rate and the structural parameters significantly


influence the cooling performance and the weight of the TCS
(mTCS). In this section, the effects of the mass flow rate of cooling
water (mf), the inner diameter (d), the contact surface height (h)
and the contact surface angle (a) of the TCS on the performance
of TCS are investigated.

4.1. Effects of mass flow rate of water

In this section, setting h, a and d as 65 mm, 80° and 2 mm,


respectively, the cooling performances of TCS for different values
of mf are investigated. Fig. 5 depicts the values of maximum tem-
perature (Tmax) and temperature difference (DT) of the battery cell
Fig. 4. Comparison of the experimental data and the simulation results. with time for various values of mf. As shown in Fig. 5, three stages
exist during the discharge process. At the first stage (0–100 s), Tmax
and DT increase with time no matter what mf is. At this stage, the
between them are 1.4 K and 0.6 K, respectively. The comparison temperature of battery is relatively low and the temperature dif-
indicates that the fitting heat generation model is feasible to be ference between the water and the battery is small. Thus, the heat
employed in numerical simulation. generation of the battery cell is much larger than the one removed
by the cooling water, resulting in rapid temperature rise for the
battery. In this stage, when larger mf is provided, the heat transfer
3. Calculation parameters coefficient between the battery and the water is larger, so Tmax
increases slower. Moreover, high heat transfer coefficient can make
In order to investigate the performance of the proposed liquid- the surface temperature of the battery rising at slower rate than
cooled BTM system, one 18650-type battery cell with three one- the temperature inside, which makes DT grow faster. From 100 s
third TCSs as shown in Fig. 1(b) is employed for numerical simula- to 600 s, when mf is larger than 1  104 kg/s, the temperature of
tion. 5C high discharge rate process is considered. The spacings the battery is in relatively stable condition, which means that the
among the batteries are set as 2 mm for compact design of the bat- heat generation can be effectively removed by the water. At the
tery pack. The TCS is made of aluminum. The cooling medium in end of the discharge process (600–720 s), the temperature of the
the channel of the TCS is water due to its high heat capacity. battery goes higher, reaching to maximum temperature. This is
The numerical calculation is conducted by commercial CFD because the internal resistance of the battery increases dramati-
software ANSYS FLUENT. Firstly, transient model is considered cally at the end of the discharge process, causing remarkable
due to the unsteady heat generation of battery. As the Reynolds enlargement of the heat generation rate, which can be seen from
number of the flow in the TCS does not exceed 2300, the flow is Fig. 2. For this situation, the temperature rise can be controlled
treated as laminar flow. Mass-flow-inlet and pressure-outlet con- by larger mass flow rate. As for DT, it becomes larger when mf is
ditions are set as the boundary conditions of the cooling water. larger than 4  105 kg/s. This phenomenon is driven by two
The initial temperature of the cooling water, the TCS and the bat- mechanisms. On one hand, the temperature of battery is lower
tery are set as 300 K. In practical applications, when the battery with larger mf. According to the experimental results in Fig. 2,
is in contact with the heat dissipation structure, the contact ther- lower temperature causes larger R. Thus, larger heat generation
mal resistance between the battery surface and the TCSs can be rate is induced for lower temperature of battery cell, which will
reduced using thermal grease or thermal conductive adhesive. deteriorate the temperature homogeneity of battery. On the other
Contact thermal resistance may influence the temperature of the hand, the larger heat transfer coefficient is achieved for larger mf,
battery cell, but it has little influence on the optimal structure of which induces excessively low temperature at the coolant entrance
the TCS. Based on the above considerations, the contact thermal side of battery. Thus, lower minimum temperature for the battery
resistance between the battery surface and the TCSs is ignored in is created.
this study. The interface between the battery cell and the TCS is Table 3 lists the numerical results at the end of the 5C discharge
set as the continuity condition. The outer wall of the TCS and the process for various values of mf. It can be seen that Tmax is reduced
rests of the battery surfaces are chosen as thermal insulation. as mf increases. When mf is larger than 1  104 kg/s, Tmax is con-
The source term of the battery is implemented by coding User trolled below 313 K (40 ), which meets the requirement of battery
Define Function (UDF) in software. Time step of 1 s and 50 itera- temperature. With the additional increase of mf, the improvement
tions per time step are set. The relevant convergence residuals of of cooling effect is weakened. For instance, when mf is risen from
the continuity equation, the velocity equations and the energy 1  103 kg/s to 2  103 kg/s, Tmax is decreased by only 0.80 K.
equation are set as 106, 106 and 109, respectively. Compared to Tmax, DT changes less with mf. At mf as 1  104 kg/
Set the mass flow rate as 1  104 kg/s and take the TCS with s, DT is 4.806 K, satisfying the demand of the temperature differ-
a = 80°, d = 2 mm, h = 65 mm as an example. Grid independent ence of battery. Besides, the pressure drop of the cooling channel
analysis is carried out to confirm the appropriate grid size. The for the TCS is 128 Pa. Table 3 also shows that DP increases rapidly
results show that when the grid number changes from 91,544 to as mf increases. For example, both the situations with mf as
201,995, the temperature difference of the battery cell (DT) 1  103 kg/s and 1  104 kg/s satisfy the temperature demand
changes by 0.3 K. While the grid number further changes from of BTM, but DP of the former is more than 20 times than that of
201,995 to 415,694, DT only changes by 0.04 K. Therefore, the grid the latter. Too large mf is less economical due to large power con-
number of 201,995 is enough for simulation, and the similar grid sumption. Therefore, the moderate mf should be chosen by consid-
size is used for the following studies. ering both the cooling performance and the pressure drop.
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 7

Fig. 5. Tmax (a) and DT (b) with time for 5C discharge rate process for various mass flow rates.

Table 3 Table 4
Temperature and pressure drop for various values of mass flow rates. The performance of the TCSs with various parameters.

mf Tmax DT DP D h a Tmax DT mTCS DP W


(kg/s) (K) (K) (Pa) (mm) (mm) (°) (K) (K) (g) (Pa)
1  105 323.49 4.756 11 1 65 80 312.30 4.6242 9.77 1992 –
2  105 318.11 4.591 22 1.5 65 80 312.28 4.6764 9.60 403 6.60
4  105 314.83 4.533 45 2 65 80 312.22 4.8059 9.36 128 3.72
1  104 312.22 4.806 128 2.5 65 80 312.24 4.7989 9.05 53 87.97
2  104 310.74 5.057 302 3 65 80 312.23 4.8410 8.67 26 18.00
1  103 308.19 5.338 2681
2 65 80 312.22 4.8059 9.36 128 –
2  103 307.39 5.338 7224
2 64 80 312.25 4.5741 9.21 128 0.62
2 62 80 312.30 4.2860 8.93 128 0.50
2 60 80 312.36 4.0585 8.64 128 0.63
2 58 80 312.42 3.8670 8.35 128 0.75
2 56 80 312.49 3.7004 8.06 128 0.86
2 55 80 312.62 3.6991 7.92 128 108.24
2 54 80 312.83 3.8180 7.77 128 1.21
2 53 80 313.06 3.9419 7.63 128 1.16
2 65 40 312.68 5.5771 5.68 128 0.20
2 65 60 312.40 5.1233 7.52 128 0.29
2 65 80 312.22 4.8059 9.36 128 0.47
2 65 100 312.08 4.5459 11.79 128 0.94
2 65 120 311.97 4.3447 15.58 128 –

result in smaller frictional resistance. Moreover, mTCS is decreased


significantly as d increases. However, considering the structural
strength, d cannot be too large due to the demand of the structural
strength. Therefore, moderate d should be chosen under the con-
sideration of DP and mTCS.
Fig. 6. Tmax, DT and pressure drop for various inner diameters of TCS.

4.3. Effects of the contact surface height of TCS


4.2. Effects of the inner diameter of TCS
In this section, mf, d and a are set as 1  104 kg/s, 2 mm and
In this section, mf, a and h are set as 1  104 kg/s, 80°, 65 mm, 80°, respectively, and the influence of h is investigated. As the tem-
respectively, and the effects of d on the performance of TCS is perature of the battery cell around the TCS inlet is lower than the
investigated. The values of Tmax, DT and DP at the end of the dis- one around the outlet, the contact surface height of the TCS is
charge process for various values of d are shown in Fig. 6. The rel- reduced from the inlet part, the schematic of which is shown in
ative results are also summarized in Table 4. It can be seen that Fig. 7. Tmax, DT and mTCS for various values of h are shown in
Tmax and DT change little with d. As mf is fixed, smaller d leads to Fig. 8. The relative results are summarized in Table 4. It can be
larger velocity, resulting in a larger convective heat transfer coeffi- observed that Tmax increases gently as h decreases. DT decreases
cient. Meanwhile, the heat transfer area is reduced as d is first and then increases with h, finally achieving the minimum
decreased. Thus, the total convective heat transfer changes little value when h = 55 mm. It can be concluded that the TCS achieves
with d. That is, the value of d does not influence the cooling perfor- the best cooling performance when h = 55 mm. Note that the cool-
mance of the TCS much. As for the pressure drop of the channel in ing water around the inlet has lower temperature than the one
the TCS, DP decreases as d increases. This is because larger d will around the outlet, which is one of the reasons causing the temper-
8 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581

ature difference inside the battery cell. Fig. 9 depicts the tempera-
ture distributions of the battery with various values of h. It can be
seen that the slice reduction of the TCS around the inlet can
increase the temperature of battery around the inlet, which can
also reduce the temperature difference of battery. However, when
h is reduced too much, the battery part without contacting the TCS
is difficult to be cooled by the TCS due to small thermal conductiv-
ity of the battery cell, causing obvious increase of Tmax. This can be
seen from the temperature contours in Fig. 9. When h = 65 mm or
h = 55 mm, Tmax exists at the bottom center of the battery. When
h = 53 mm, Tmax exceeds 313 K and exists at the top center of the
battery. As for mTCS, it decreases linearly with h. Therefore, choos-
ing moderate value of h is effective to reduce mTCS while maintain-
ing the cooling performance of the TCS.

4.4. Effects of contact surface angle of TCS

In this section, mf, d and h are set as 1  104 kg/s, 2 mm,


65 mm, respectively. The effect of the contact surface angle (a) of
TCS is studied. The values of 40°, 60°, 80°, 100° and 120° are con-
sidered for a. Fig. 10 depicts the comparison of Tmax and DT at
Fig. 7. Schematic of the contact surface height of the TCS.
the end of the 5C discharge process and the weights of the TCSs.

Fig. 8. Tmax, DT and mTCS for various contact surface heights of the TCS. Fig. 10. Tmax, DT and the weight for various contact surface angles of the TCS.

Fig. 9. Temperature contours of battery for three values of contact surface height (h) of TCS.
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 9

The relative results are also summarized in Table 4. The numerical


results show that Tmax and DT are reduced as a increases. Larger a
increases the heat transfer area between the battery cell and the
TCS, which enhances the heat conduction. When a changes from
40° to 120°, Tmax and DT are reduced by 0.7 K and 1.2 K, respec-
tively. However, larger a will remarkably increase mTCS. Changing
a from 40° to 120°, mTCS is increased by about three times. There-
fore, the appropriate contact surface angle should be chosen after
considering the cooling performance and mTCS.

5. Design of the structure of TCS

In this section, the structural parameters of the TCS are


designed to improve the cooling performance and reduce mTCS.
From the analysis above, DT is more sensitive to the structural
parameters than Tmax, so DT is mainly considered. To evaluate
the influences of three structural parameters (h, a and d) on DT
Fig. 11. Comparisons of weight ratios of different schemes.
and mTCS, a weight sensitive factor is defined as
 
 mTCS;1  mTCS;2 
wX ¼   ð14Þ percentage of mTCS compared to the one of TCS-0. Similarly, a neg-
ðDT 1  DT 2 Þ  ðX 1  X 2 Þ ative value of gmTCS means mTCS is reduced. The subscripts n repre-
sents the values of TCS-n and 0 represents the value of TCS-0.
where WX is the weight sensitive factor. X represents the considered
structural parameters, such as h, a and d. The subscripts x and y rep- DT n  DT 0
resent two parameter values. W represents the variability of mTCS to gDT n ¼ ð15Þ
DT 0
the change of DT for the unit change of one certain parameter.
When the value of W is larger, the influence of the parameter on mTCS;n  mTCS;0
mTCS is more obvious. Note that X1 and X2 are the adjacent values gmTCS;n ¼ ð16Þ
mTCS;n
of X. For example, for the parameter point as h = 55 mm, d = 2 mm
and a = 80°,Wh is defined as (8.061379  7.917426)/ When designing TCS, d is designed first with other parameters
((3.70043  3.69910)  (56–55)) = 108.24. The values of W for var- fixed. According to the results in Table 5, the cooling performance
ious situations are also listed in Table 4. It can be seen that d is the changes little, and mTCS and DP are reduced remarkably as d
most important parameter that influences on mTCS. h is the sec- increases. Thus, from the view of mTCS and DP, d is desirable to
ondary parameter, and a is the parameter with the minimal impact be large. However, considering the structural strength of the TCS,
on mTCS. Based on this characteristic, the structural parameters of d cannot be too large. Considering the cooling performance, pres-
the TCS are designed. Table 5 lists the performances of the TCSs sure drop and the structural strength, d is chosen as 3 mm, and
with various parameters during the design process. The TCS with the TCS with h = 65 mm, a = 80° and d = 3 mm is denoted as TCS-
h, a and d as 65 mm, 80°, 2 mm is defined as the original TCS, which 1. The results in Table 5 show that TCS-1 has similar cooling perfor-
is denoted as TCS-0. In Table 5, gDT represents the variation percent- mance as TCS-0, but mTCS is reduced by 7%, and DP is reduced by
age of DT compared to the one of TCS-0. A negative value of gDT 80%. Based on TCS-1, the value of h is designed. Various values of
means DT is decreased after design. gmTCS represents the variation h are considered and the performance of the relevant TCSs are

Table 5
The performance of the TCSs during the design process.

d h a Tmax DT gDT mTCS gmTCS DP


(mm) (mm) (°) (K) (K) (%) (g) (%) (Pa)
TCS-0 2 65 80 312.22 4.806 0.0% 9.36 0.00% 128.11
1 65 80 312.30 4.624 4% 9.77 4% 1992.06
1.5 65 80 312.28 4.676 3% 9.60 3% 403.35
2 65 80 312.22 4.806 0.0% 9.36 0.00% 128.11
2.5 65 80 312.24 4.799 0.2% 9.05 3% 53.21
TCS-1 3 65 80 312.23 4.841 0.7% 8.67 7% 26.13
3 65 80 312.23 4.841 0.7% 8.67 7% 26.13
3 64 80 312.25 4.596 4% 8.53 9% 26.13
3 62 80 312.30 4.296 11% 8.27 12% 26.13
3 60 80 312.36 4.060 16% 8.00 14% 26.13
3 58 80 312.42 3.865 20% 7.73 17% 26.13
3 56 80 312.49 3.692 23% 7.47 20% 26.13
TCS-2 3 55 80 312.60 3.696 23% 7.33 22% 26.13
3 54 80 312.82 3.807 21% 7.20 23% 26.13
3 53 80 313.05 3.930 18% 7.07 24% 26.13
3 55 40 313.07 4.369 9% 4.22 54% 26.13
TCS-3 3 55 50 312.90 4.137 14% 5.03 46% 26.13
3 55 60 312.77 3.953 18% 5.78 38% 26.13
3 55 70 312.67 3.805 21% 6.53 30% 26.13
3 55 80 312.60 3.696 23% 7.33 22% 26.13
3 55 90 312.55 3.604 25% 8.27 12% 26.13
10 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581

Fig. 12. Schematic diagram of the 4 types inlet and outlet directions of the reservoir plate.

listed in Table 5. It can be observed that when h = 56 mm, the min- decreases. In order to make sure that Tmax is controlled below
imum DT as 3.692 K is obtained. When h changes from 56 mm to 313 K, a is chosen as 50° and the relevant TCS is denoted as TCS-
55 mm, mTCS is reduced further with DT almost unchanged. Thus, 3. DT of TCS-3 is only 4.1 K. Compared to TCS-0, DT is reduced by
h is chosen as 55 mm and the relevant TCS is denoted as TCS-2. 14% and mTCS is reduced by 46% for TCS-3. In general, considering
Compared to TCS-0, DT is reduced by 23% and mTCS is reduced by the improvement of DT and mTCS, the structural parameters are
22% for TCS-2. Based on the structural parameters with chosen as d = 3 mm, h = 55 mm and a = 50°. With the designed
h = 55 mm and d = 3 mm, a is designed. The results for various val- parameters, the TCS can meet the temperature control require-
ues of a are summarized in Table 5. The results show that Tmax and ments of battery cell.
DT increase gradually as a decreases, and mTCS decreases as a To test the effectiveness of the present lightweight design, the
solutions in previous studies [17,34] are introduced to compare
Table 6 with TCS-0 and TCS-3. For various solutions, the weight ratios of
Effect of different inlet and outlet directions on flow distribution uniformity of flow the cooling structure to the whole battery system are calculated,
channel structure. and the results are shown in Fig. 11. It can be seen from Fig. 11 that
System c DP (Pa) before the lightweight design, the weight ratio of TCS-0 is similar
AA1-00 0.090 146.5
to the ones of the cooling structures in previous studies. After
AA1-10 0.023 150.1 the present lightweight design, the weight ratio of TCS-3 is reduced
AA1-01 0.091 182.0 by at least 36% compared to other solutions, which verifies the
AA1-11 0.022 186.1 effectiveness of the present design.

Fig. 13. The flow rate distribution among the parallel TCSs for AA1-00 and AA1-01.
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 11

6. Performance of liquid-cooled BTMS parameter that influences mTCS, h is the secondary parameter,
and a is the parameter with the minimal impact on mTCS.
In this section, the performance of parallel liquid-cooled BTMS 3. The three structural parameters of TCS are designed according
shown in Fig. 1 is discussed. In the system, the designed TCS com- to the order as d, h and a. Compared to the original TCS, DP,
poses the parallel channels. Note that the uniformity of the flow DT and mTCS are respectively reduced by 80%, 14% and 46% for
rates among parallel TCSs significantly influences the temperature the designed TCS while Tmax is controlled below 313 K.
uniformity of battery pack. The mass flow rate in different parallel 4. For the liquid-cooled system with parallel TCSs, the flow rates
channels in the system is calculated by numerical method. In order among the parallel channels can be homogenized through
to evaluate the uniformity of the flow rates among parallel chan- designing the directions of the inlet and the outlet of the sys-
nels, the dimensionless uneven coefficient c is defined by tem. For the improved system, the temperature difference of
battery pack is similar to the one of a single battery cell.
rffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
PN  2
i¼1 ðmf  mf Þ
i
It is worth noting that the design process in this study is avail-
c¼  pffiffiffiffi ð17Þ able for various types of cylindrical batteries. The present study
mf N
facilitates the guideline for compact and lightweight design of
 the liquid-cooled BTM system.
where mif and mf are the mass flow rate of the ith channels and the
average flow rate among the parallel flow channels, respectively. N Declaration of Competing Interest
is the number of parallel flow channels. The smaller the c value is,
the better the uniformity of the flow rates is. When c is equal to 0, The authors declared that there is no conflict of interest.
the flow rates among parallel channels are the same. Four systems
with different positions of inlets and outlets are considered, which
Acknowledgements
are denoted as AA1-00, AA1-10, AA1-01 and AA1-11, respectively.
The schematics of the systems are shown in Fig. 12.
This study was supported by National Natural Science Founda-
The comparison of the performances for various systems are
tion of China (Grant No. 51536003) and Dongguan Innovative
shown in Table 6. It can be seen from Table 6 that AA1-10 performs
Research Team Program (No. 2014607119).
better than other systems. The dimensionless uneven coefficient
and the pressure drop of AA1-10 are both small. It means that
AA1-10 can achieve uniform flow rates among the parallel channels References
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