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Article history: Battery thermal management (BTM) is indispensable to the battery pack of electric vehicles (EVs) for
Received 27 December 2018 safety. Among different types of BTM technologies, liquid cooling shows its superiority with high heat
Received in revised form 12 July 2019 transfer coefficient and low power consumption. However, the previous works paid little attention to
Accepted 13 August 2019
the compactness and weight ratio of liquid-cooled BTM system, which is vital to the specific energy of
Available online 27 August 2019
battery pack. In this study, a compact and lightweight liquid-cooled BTM system is presented to control
the maximum temperature (Tmax) and the temperature difference (DT) of lithium-ion power battery pack.
Keywords:
In this liquid-cooled solution, one thermal conductive structure (TCS) with three curved contact surfaces
Battery thermal management
Cylindrical battery
is developed to cool cylindrical battery. The influences of mass flow rate (mf), inner diameter (d), contact
Liquid cooling surface height (h) and contact surface angle (a) of the TCS are investigated through numerical study. It is
Lightweight found that for the 5C discharge rate process of battery, Tmax can be maintained within 313 K when mf is
Structure design larger than 1 104 kg/s. A weight sensitive factor is defined to evaluate the influences of d, h and a on
DT and the weight of TCS. It is found that d is the most important parameter that influences the weight. h
is the secondary parameter, and a is the parameter with the minimal impact on the weight. Then the val-
ues of d, h, and a are designed to reduce the weight of TCS while maintaining its cooling performance. The
designed TCS can control Tmax under 313 K with DT as 4.137 K. Compared to the original TCS, DP, DT and
the weight are respectively reduced by 80%, 14% and 46% for the designed TCS. Furthermore, the perfor-
mance of liquid-cooled system with parallel TCSs is discussed. The flow distribution among parallel TCSs
is improved through designing the positions of the inlet and the outlet, which enables that Tmax and DT of
battery pack is similar to the ones of a single battery. The present study facilitates the guideline for com-
pact and lightweight design of liquid-cooled battery thermal management system.
Ó 2019 Elsevier Ltd. All rights reserved.
https://doi.org/10.1016/j.ijheatmasstransfer.2019.118581
0017-9310/Ó 2019 Elsevier Ltd. All rights reserved.
2 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581
Nomenclature
of specific energy density, the cooling load of the battery pack gets 5 mW power consumption. An aluminum flat tube was introduced
higher correspondingly. Among various BTM technologies, liquid by Zhang et al. [30] for liquid cooling. On both side of each battery
cooling shows excellent thermal management performance with cell, three aluminum flat tubes were arranged in stagger. To
high heat transfer coefficient and low parasitic power consumption improve the temperature difference of the battery, the flexible gra-
[15]. According to the BTM strategies report by National Renew- phite was added between the cell surface and the flat tubes. The
able Energy Laboratory (NREL) of the U.S., liquid-cooled BTM is results showed that the temperature of the battery was under
the optimal choice for current commercial electric vehicle market 313 K and the temperature difference was effectively reduced by
[6]. In recent years, liquid-cooled BTM technology has become flexible graphite.
more and more popular for EVs. Many commercial EVs such as Compared to prismatic and pouch battery, cylindrical battery
Tesla Model 3, Chevrolet Volt, BYD Song DM and BMW i8 have possesses the superiority of better consistency, more mature craft
employed liquid-cooled BTM technology. and longer lifecycle [31,32]. However, due to the shape of cylindri-
Numerous studies have been done to investigate liquid-cooled cal battery cell, surface thermal contact is not available for conven-
BTM systems. The proposed solutions include two ways, direct liq- tional LCPs. To realize liquid cooling, researchers have designed
uid cooling and indirect liquid cooling. Direct cooling has higher some special structures to construct adequate thermal contact
thermal management efficiency by using mineral oil silicone oil, with the cylindrical batteries. Basu et al. [17] proposed and ana-
etc. However, this method needs more power consumption and lyzed a conduction element sheet made by aluminum with
involves more risk of leakage. After comprehensive comparison 1.5 mm in thick and 44 mm in height. Each 18650-type battery
of different cooling methods, Chen et al. [15] suggested that indi- was contacted with two conduction elements. The conduction ele-
rect liquid cooling was more suitable for practical applications. ment could effectively reduce the temperature difference of the
For prismatic and pouch batteries, sandwiching them by liquid battery. Besides, the maximum temperature rise was controlled
cold plate (LCP) is a prevalent solution to tackle the thermal issue. under 7 K. For the Tesla Model S battery pack, Jiang et al [33] dis-
The generated heat of the battery is transferred to LCPs by thermal cussed the BTM performance of a wavy cooling channel wound
conduction and then is dissipated by liquid coolant inside the mini around the batteries. It is found that increasing liquid flow rate
channels of LCPs by thermal convection. Panchal et al. [16] consid- and heat exchange area were beneficial to the performance of cool-
ered one LCP with a serpentine channel inside for prismatic bat- ing channel. Rao et al. [34] employed the aluminum block with arc
tery. The LCP was assessed at different discharge rates and shape surfaces for 26650-type battery. The camber surfaces of the
boundary conditions. The temperature rise of the battery was well blocks matched the battery surfaces to build enough thermal con-
controlled by this type of LCP at 2C discharge rate. Jin et al. [28] tact arc. The effects of the inlet velocity and the block length on the
proposed a LCP with oblique fins inside for BTM. These fins can cooling performance were carried out by simulation. It was found
re-initialize the boundary layers of the coolant to achieve higher that the performance of the blocks can be improved by varying the
heat transfer coefficient. The experimental and numerical results blocks length linearly. Zhao et al. [35] numerically investigated the
showed that this plate had better thermal management perfor- performance of the liquid-cooled cylinder for 42110-type cylindri-
mance than those conventional straight-channel plates. Lan et al. cal battery. The thermal contact surface was established by filling
[29] developed a novel mini-channel based cooling tube, which the battery cell into each cylinder. In the cylinder, there were num-
can maintain the battery temperature in rational range, with only bers of mini-channels to dissipate the heat. The results showed
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 3
that the cylinder could maintain the maximum temperature under (h) and the contact surface angle (a). These parameters can be
313 K, but it was difficult to make the temperature difference changed to adjust the cooling performance and the weight of the
below 5 K due to the aging effect of the battery. TCS (mTCS).
The above-mentioned works either focus on thermal behaviors For the liquid-cooled BTM system in Fig. 1, the cooling water is
of the battery thermal management system or different cooling distributed by the upper reservoir and then flows into each parallel
methods, while less research has discussed the compactness and TCS. The heat generated by the batteries is transferred to the TCSs
lightweight design for liquid-cooled BTM systems. In practical uti- through heat conduction and dissipated by the cooling water in the
lization, a battery pack with higher specific energy is desirable to channel of TCS, so that the temperature control of battery pack is
achieve longer mile range of EVs. Although liquid cooling shows achieved. The heated cooling water is gathered by the bottom
excellent cooling performance comparing with other BTM tech- reservoir and then leaves the system through the outlet. It can be
nologies, the relatively large weight ratio is an issue needed to observed that the proposed TCS is one of the most important com-
be solved. A compact and lightweight BTM design can improve ponents in the liquid-cooled system, and the parameters of TCS
the specific energy of battery pack and reduce the general weight have significant influence on the thermal performance of the sys-
of finished vehicle. Previous studies have pointed out that energy tem. Therefore, the structure of TCS needs to be designed to
consumption was decreased by 3.3–8% when the weight of vehicle improve the cooling performance and reduce the weight.
got 10% reduction [36,37]. Moreover, the lightweight of the vehicle
enhances the acceleration performance and reduces the braking 2.2. Numerical simulation
length. Department of Energy of America also puts forward a 30%
reduction lightweight plan for EVs [38]. However, the compact To investigate the performance of the TCSs, computational fluid
and lightweight design for liquid-cooled BTM system has been dynamics (CFD) method is introduced. The governing equations are
rarely considered in the existing literature. the continuity equation, the momentum conservation equations
In this study, a liquid-cooled BTM system is designed to realize and the energy equations. For the cooling water, the governing
suitable temperature range and temperature difference for Li-ion equations are expressed as follows.
battery pack. The novelty of the proposed solution concerns a com-
@ qw !
pact and lightweight design for EVs application, improving the þ r ðqw v Þ ¼ 0 ð1Þ
cooling performance and reducing the weight of battery pack. In @t
the present work, the 18650-type battery cell is introduced and
the 5C high discharge rate process is considered. Experiment is @ ! ! ! !
ðq v Þ þ rðqw v v Þ ¼ rp þ r ðlw r v Þ ð2Þ
conducted to obtain the thermal model of the battery cell. A novel @t w
thermal conductive structure (TCS) is proposed to cool the battery
@ !
ðq cpw T w Þ þ r ðqw cpw v T w Þ ¼ r ðkw rT w Þ
cell. Based on the numerical method, the influences of mass flow
ð3Þ
rate and structural parameters on the cooling performance and @t w
the weight of the TCS are investigated. Then, the structural param- For the battery cell and the TCS, the governing equations are
eters are designed to reduce the weight of the TCS while maintain- given by
ing its thermal management performance. Finally, the performance
@ Q gen
of liquid-cooled system with parallel TCSs is investigated and is ðq cpb T b Þ ¼ r ðkb rT b Þ þ ð4Þ
improved through designing the positions of the inlet and the out- @t b Vb
let of the system. The present work is intended to facilitate the
@
guideline for compact and lightweight design of liquid-cooled bat- ðq cpTCS T TCS Þ ¼ r ðkTCS rT TCS Þ ð5Þ
tery thermal management system, which is beneficial to increasing @t TCS
the mile range of EVs. In Eqs. (1)–(5), q, cp, k and T are density, specific heat, thermal
conductivity and temperature, respectively. The subscripts w, b
and TCS represent the cooling water, the battery and the thermal
!
2. Methodology and simulation conductive structure. v , p and l denote the velocity vector, the
static pressure and the dynamic viscosity, respectively. Qgen and
2.1. A lightweight liquid-cooled BTM system Vb are the heat generation rate and the volume of battery cell.
To realize a long mile range, battery pack comprising dozens of 2.3. Battery model and validation
battery cells is needed for power supply of EVs. In this study, a
liquid-cooled BTM system is proposed to cool battery pack. When discharging, the battery temperature will increase due to
Scheme of the liquid-cooled BTM system is illustrated in Fig. 1. irreversible and reversible heat generation. Generally, the heat
As shown in Fig. 1(a), the battery pack includes 18650-type battery generation can be divided into reaction heat, Joule heat, polling
cells, IC control unit, base plates, and the liquid-cooled BTM sys- heat and side reaction heat. In 1985, Bernardi et al. [39] presented
tem. The liquid-cooled BTM system contains upper reservoir, ther- a lumped model for the heat generation of the battery cell, which
mal conductive structures (TCSs) and bottom reservoir. The upper can be expressed as
reservoir and bottom reservoir are made of engineering plastics to
reduce the weight. The cells are arrayed in staggered structure @U OCV
Q gen ¼ Q ir þ Q re ¼ IðU OCV UÞ IT ð6Þ
with constant distance among them. As shown in Fig. 1(b), the TCSs @T
are inserted into the gaps of the cells for a compact size consider- where Qgen is the total heat generation rate of battery cell, Qir and
ation. Each cell is surrounded by three TCSs. In the center of each Qre are the irreversible heat and the reversible heat, respectively. I
TCS, circle liquid channel is set for coolant. To construct effective is the discharge/charge current of battery cell. UOCV is the open-
thermal contact, each TCS is designed with three curved contact circuit voltage. U is the battery voltage. T is the battery temperature
surfaces as shown in Fig. 1(b) and (c). The curvature radius of the and @UOCV/oT is the temperature coefficient of open-circuit voltage.
curved contact surface is identical to the radius of cylindrical bat- During the discharge process, it obtains
tery cell. Fig. 1(c) also shows the main structural parameters of
U ¼ U OCV IR ð7Þ
TCS, including the inner diameter (d), the contact surface height
4 Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581
Table 1
Physical properties of materials inside the battery cell [40].
Thickness (lm) Height (mm) Density (kg/m3) Thermal conductivity (W/(mK)) Specific heat capacity (J/(kgK))
Can 300 65 7800 16.8 478
Separator 22 59 1200 1 700
LiCoO2 92 53 2291.6 1.85 1172.8
LiNiCoMnO2 N/A N/A 1500 5 700
LiC6 87 53 5031.7 5 700
Cathode foil 10 55 2700 200 870
Anode foil 10 57 9000 380 381
Electrolyte N/A N/A 1290 0.45 133.9
Table 2
were measured experimentally. Specifically, R is specified by Polynomial fitting of the equivalent internal resistance (R) in various temperatures.
means of Hybrid Pulse Power Characteristic (HPPC) test under Polynomial fitting of equivalent internal resistance (R) Temperature/
the conditions of various values of SOC (from 1.0 to 0.1 with 0.1 K
intervals) and temperatures (from 293 K to 333 K with 10 K inter- 166 – 1334 SOC + 6559 SOC2 – 293
vals). The experimental results are shown in Fig. 2. It can be seen 16,531 SOC3 + 22,391 SOC4 –
that for each SOC, R decreases as the temperature increases, but 15,496 SOC5 + 4301 SOC6
the tendency is weakened when the temperature increases further. 107 – 793 SOC + 4036 SOC2 – 303
10,514 SOC3 + 14,700 SOC4 –
For example, when T changes from 323 K to 333 K, R changes only
10,480 SOC5 + 2989 SOC6
about 5%. Moreover, for each temperature, R has a relatively con- 66 – 382 SOC + 1962 SOC2 – 313
stant value at the early discharge process (SOC > 0.2) and increases 5181 SOC3 + 7378 SOC4 – 5365 SOC5 + 1559 SOC6
notably at the end of discharge process (SOC < 0.2). Based on the 58 – 355 SOC + 1898 SOC2 – 323
experimental data, R can be incorporated as the function of tem- 5121 SOC3 + 7367 SOC4 – 5374 SOC5 + 1559 SOC6
48 – 233 SOC + 1225 SOC2 – 333
perature and SOC by polynomial fitting. The final expressions are 3263 SOC3 + 4667 SOC4 – 3406 SOC5 + 992 SOC6
shown in Table 2. Based on the data in Table 2, R can be obtained
when T is 293 K, 303 K, 313 K, 323 K and 333 K, respectively. When
the temperature is between two testing temperature of R, it can be
calculated by interpolation method. In addition, when the temper-
ature is above 333 K, the value of R can be represented by the inter-
nal resistance when T = 333 K because R changes little at high
temperature.
The values of UOCV were also measured from 293 K to 333 K for
each SOC, and the values of @UOCV/oT for different SOC were
obtained. The curve of @UOCV/oT is depicted in Fig. 3. Generally,
@UOCV/oT increases from SOC = 1.0 to SOC = 0.5 and then decreases
when SOC is below 0.5. @UOCV/oT can also be summarized as the
function of SOC by polynomial fitting. The fitting expression is
shown as
@U OCV
¼ 0:355 þ 2:154 SOC 2:869 SOC2 þ 1:028 SOC3
@T
ð13Þ
Fig. 3. Experimental results of open circuit voltage coefficient (@UOCV/@T) with SOC.
Fig. 5. Tmax (a) and DT (b) with time for 5C discharge rate process for various mass flow rates.
Table 3 Table 4
Temperature and pressure drop for various values of mass flow rates. The performance of the TCSs with various parameters.
ature difference inside the battery cell. Fig. 9 depicts the tempera-
ture distributions of the battery with various values of h. It can be
seen that the slice reduction of the TCS around the inlet can
increase the temperature of battery around the inlet, which can
also reduce the temperature difference of battery. However, when
h is reduced too much, the battery part without contacting the TCS
is difficult to be cooled by the TCS due to small thermal conductiv-
ity of the battery cell, causing obvious increase of Tmax. This can be
seen from the temperature contours in Fig. 9. When h = 65 mm or
h = 55 mm, Tmax exists at the bottom center of the battery. When
h = 53 mm, Tmax exceeds 313 K and exists at the top center of the
battery. As for mTCS, it decreases linearly with h. Therefore, choos-
ing moderate value of h is effective to reduce mTCS while maintain-
ing the cooling performance of the TCS.
Fig. 8. Tmax, DT and mTCS for various contact surface heights of the TCS. Fig. 10. Tmax, DT and the weight for various contact surface angles of the TCS.
Fig. 9. Temperature contours of battery for three values of contact surface height (h) of TCS.
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 9
Table 5
The performance of the TCSs during the design process.
Fig. 12. Schematic diagram of the 4 types inlet and outlet directions of the reservoir plate.
listed in Table 5. It can be observed that when h = 56 mm, the min- decreases. In order to make sure that Tmax is controlled below
imum DT as 3.692 K is obtained. When h changes from 56 mm to 313 K, a is chosen as 50° and the relevant TCS is denoted as TCS-
55 mm, mTCS is reduced further with DT almost unchanged. Thus, 3. DT of TCS-3 is only 4.1 K. Compared to TCS-0, DT is reduced by
h is chosen as 55 mm and the relevant TCS is denoted as TCS-2. 14% and mTCS is reduced by 46% for TCS-3. In general, considering
Compared to TCS-0, DT is reduced by 23% and mTCS is reduced by the improvement of DT and mTCS, the structural parameters are
22% for TCS-2. Based on the structural parameters with chosen as d = 3 mm, h = 55 mm and a = 50°. With the designed
h = 55 mm and d = 3 mm, a is designed. The results for various val- parameters, the TCS can meet the temperature control require-
ues of a are summarized in Table 5. The results show that Tmax and ments of battery cell.
DT increase gradually as a decreases, and mTCS decreases as a To test the effectiveness of the present lightweight design, the
solutions in previous studies [17,34] are introduced to compare
Table 6 with TCS-0 and TCS-3. For various solutions, the weight ratios of
Effect of different inlet and outlet directions on flow distribution uniformity of flow the cooling structure to the whole battery system are calculated,
channel structure. and the results are shown in Fig. 11. It can be seen from Fig. 11 that
System c DP (Pa) before the lightweight design, the weight ratio of TCS-0 is similar
AA1-00 0.090 146.5
to the ones of the cooling structures in previous studies. After
AA1-10 0.023 150.1 the present lightweight design, the weight ratio of TCS-3 is reduced
AA1-01 0.091 182.0 by at least 36% compared to other solutions, which verifies the
AA1-11 0.022 186.1 effectiveness of the present design.
Fig. 13. The flow rate distribution among the parallel TCSs for AA1-00 and AA1-01.
Y. Lai et al. / International Journal of Heat and Mass Transfer 144 (2019) 118581 11
6. Performance of liquid-cooled BTMS parameter that influences mTCS, h is the secondary parameter,
and a is the parameter with the minimal impact on mTCS.
In this section, the performance of parallel liquid-cooled BTMS 3. The three structural parameters of TCS are designed according
shown in Fig. 1 is discussed. In the system, the designed TCS com- to the order as d, h and a. Compared to the original TCS, DP,
poses the parallel channels. Note that the uniformity of the flow DT and mTCS are respectively reduced by 80%, 14% and 46% for
rates among parallel TCSs significantly influences the temperature the designed TCS while Tmax is controlled below 313 K.
uniformity of battery pack. The mass flow rate in different parallel 4. For the liquid-cooled system with parallel TCSs, the flow rates
channels in the system is calculated by numerical method. In order among the parallel channels can be homogenized through
to evaluate the uniformity of the flow rates among parallel chan- designing the directions of the inlet and the outlet of the sys-
nels, the dimensionless uneven coefficient c is defined by tem. For the improved system, the temperature difference of
battery pack is similar to the one of a single battery cell.
rffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
PN 2
i¼1 ðmf mf Þ
i
It is worth noting that the design process in this study is avail-
c¼ pffiffiffiffi ð17Þ able for various types of cylindrical batteries. The present study
mf N
facilitates the guideline for compact and lightweight design of
the liquid-cooled BTM system.
where mif and mf are the mass flow rate of the ith channels and the
average flow rate among the parallel flow channels, respectively. N Declaration of Competing Interest
is the number of parallel flow channels. The smaller the c value is,
the better the uniformity of the flow rates is. When c is equal to 0, The authors declared that there is no conflict of interest.
the flow rates among parallel channels are the same. Four systems
with different positions of inlets and outlets are considered, which
Acknowledgements
are denoted as AA1-00, AA1-10, AA1-01 and AA1-11, respectively.
The schematics of the systems are shown in Fig. 12.
This study was supported by National Natural Science Founda-
The comparison of the performances for various systems are
tion of China (Grant No. 51536003) and Dongguan Innovative
shown in Table 6. It can be seen from Table 6 that AA1-10 performs
Research Team Program (No. 2014607119).
better than other systems. The dimensionless uneven coefficient
and the pressure drop of AA1-10 are both small. It means that
AA1-10 can achieve uniform flow rates among the parallel channels References
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