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Journal of Physics D: Applied Physics

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IOP PUBLISHING JOURNAL OF PHYSICS D: APPLIED PHYSICS
J. Phys. D: Appl. Phys. 46 (2013) 224001 (13pp) doi:10.1088/0022-3727/46/22/224001

Spatial structure of the arc in a pulsed


GMAW process
R Kozakov1 , G Gött1 , H Schöpp1 , D Uhrlandt1 , M Schnick2 , M Häßler2 ,
U Füssel2 and S Rose2
1
Leibniz Institute for Plasma Science and Technology, Felix-Hausdorff-Str. 2, 17489 Greifswald,
Germany
2
Institute of Manufacturing Technology, Technische Universität Dresden, Georg-Bähr-Str 3c, 01062
Dresden, Germany
E-mail: kozakov@inp-greifswald.de

Received 30 November 2012, in final form 6 March 2013


Published 16 May 2013
Online at stacks.iop.org/JPhysD/46/224001

Abstract
A pulsed gas metal arc welding (GMAW) process of steel under argon shielding gas in the
globular mode is investigated by measurements and simulation. The analysis is focussed on
the spatial structure of the arc during the current pulse. Therefore, the radial profiles of the
temperature, the metal vapour species and the electric conductivity are determined at different
heights above the workpiece by optical emission spectroscopy (OES). It is shown that under
the presence of metal vapour the temperature minimum occurs at the centre of the arc. This
minimum is preserved at different axial positions up to 1 mm above the workpiece. In
addition, estimations of the electric field in the arc from the measurements are given. All these
results are compared with magneto-hydrodynamic simulations which include the evaporation
of the wire material and the change of the plasma properties due to the metal vapour admixture
in particular. The experimental method and the simulation model are validated by means of the
satisfactory correspondence between the results. Possible reasons for the remaining deviations
and improvements of the methods which should be aspired are discussed.
(Some figures may appear in colour only in the online journal)

1. Introduction Earlier models of GMAW process were made in analogy


with the models for the tungsten inert gas (TIG) welding and
The gas metal arc welding (GMAW) process is widely used neglected metal vapour. In works [1, 2] the arc properties were
in industry. The welding wire and part of the workpiece calculated using a steady-state model. Transient models of
are melted by the electric arc which is burning in shielding the arc behaviour and droplet transfer were calculated using
gas. The material transfer is performed by the droplets MHD-volume of fluid (VoF) models [3–5]. However, in all
of the welding wire. The pulsed GMAW process is a these publications the temperature distributions of the arc were
modification which enables a one drop per pulse material similar to those for TIG arcs and represented temperatures
transfer. Depending on the current value the process can be at the arc axis between 16 000 and 25 000 K. On the other
operated either in globular or spraying mode. hand, the results of experimental observations [6, 9] show
Magneto-hydrodynamic (MHD) simulations of the certain discrepancy with temperature profiles predicted by
GMAW process are able to build complex models which these models. A temperature minimum at the centre of
describe the process as a whole including wire, arc and spraying arcs in argon as well as in argon with small additions
workpiece. Nevertheless some simplifying assumptions are of CO2 was identified [6]. Influence of the metal vapour on
usually made in the model which allow one to obtain solid the properties of the welding arc was intensively investigated.
results with reasonable efforts. The proof of such assumptions The overview of the current knowledge on this topic can
and their influence on the result can be made by comparison be found in the review [7] and other papers in the journal’s
with experimentally determined plasma parameters. issue. In particular, the GMAW process was investigated in

0022-3727/13/224001+13$33.00 1 © 2013 IOP Publishing Ltd Printed in the UK & the USA
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

from the side by two spectrometers (75 cm and 50 cm Acton


Research) and a high-speed camera. By this arrangement the
horizontal cross-section of the arc at some height above the
workpiece was analysed. Different heights of observations
were chosen by simultaneous vertical shift of workpiece and
torch.
Two spectral regions were examined. One of them was
centred at 533 nm with spectral range of approximately 13 nm.
Iron line radiation could be observed in this region with
approximately 35 spectral lines. Another spectral region
was centred at 700 nm with spectral range of approximately
10 nm. Here the argon line 696.54 nm was examined. The
signal of side-on radiance (W nm−1 m−2 sr −1 ) was spectrally
resolved by a diffraction grating (1200 gr mm−1 ). The absolute
Figure 1. Experimental set-up. M—mirror, SM—spherical mirror. intensities of radiation were obtained by comparison with
radiation of a calibrated tungsten ribbon lamp.
spraying [8] and globular [9] transfer modes. Also a special The welding process was initiated in argon shielding gas
case of the short-arc process was analysed [10, 11]. All with mild steel S235 as a 10 mm thick workpiece and welding
mentioned investigations have shown temperature minimum wire G3Si1 of 1.2 mm diameter. The welding speed was
in the metal vapour dominated region compared with the chosen to be 30 cm min−1 and wire feed rate of 4 m min−1 .
surrounding shielding gas. The welding parameters of the machine were adjusted to
In addition, numerical models respecting metal vapour obtain the arc of approximately 7 mm length. The measuring
were performed in order to investigate the cause of central positions were 1, 2, 3 and 4 mm above the workpiece. The
temperature minimum of GMAW arcs. It seems that the current values were recorded with an oscilloscope and a Hall
radiation emission of metal vapour plasma [12–14] and the current transducer (LEM). The voltage was measured with a
convective cooling from the vaporising wire [15] are dominant differential probe.
effects causing the temperature minimum. Current papers [16,
17] present GMAW models with VoF free surface modelling of 2.2. Evaluation procedure
the droplet and MHD arc models with metal vapour. Therein
the vaporization of metal vapour is calculated using different The total radiation flux emitted within a spectroscopic line can
vaporization models. be obtained by integration over the wavelength for each side-
Plasma parameters in the arc can be measured in sufficient on position y yielding the radiance (W m−2 sr −1 ). This can be
detail with the help of spatially resolved optical emission performed either by a numerical integration of the measured
spectroscopy (OES). This techniques allows one to determine data or by a fit procedure. In the latter case the intensity profile
the temperature along the arc cross-section. Assuming at each side-on position is fitted with the assumed line profile.
rotational symmetry of the arc the radial temperature and In general the line profile is described by a Voigt function,
particle density profiles are usually obtained. For better the convolution of a Gaussian and a Lorentz profile. In the
understanding of physical processes inside the arc a 2D profile case of argon the Doppler width of the atomic line 696.54 nm
of plasma parameters is of major importance. This paper at a temperature of 20000 K is approximately 0.01 nm. The
introduces results of OES measurements on a GMAW process measured line width in argon at atmospheric pressure arcs is
in globular transfer mode at different axial positions along in our case of the order of 0.186 nm. Taking into account
the arc. The experimental results are compared with MHD the apparatus profile of the order of 0.06 nm it can be stated
simulations of the GMAW process. that the measured line width is one order of magnitude larger
The paper is organized as follows. In section 2 the than Doppler width and is mainly due to the Stark broadening
experimental procedure and set-up are described. The results caused by interaction of a free plasma electron with the electric
of the measurements are presented in section 3. The model dipole induced in the argon atom by a previous interaction with
other plasma electrons. The Stark line broadening is described
used for the simulation is presented in section 4. Main results
by a Lorentz profile, and since this effect is more pronounced
of the simulation and experiment are compared and discussed
than the Doppler broadening (described by a Gaussian), the
in section 5. Concluding remarks are summarized in section 6.
combined effect can be still described by a Lorentz profile:

2. Experimental setup and evaluation procedure I 2 1


Iλ = I0 +  2 , (1)
π λ λ−λ0
1+
2.1. Set-up λ/2

The experimental set-up is shown in figure 1. A commercially where I0 is the background radiation, λ0 is the line centre,
available welding machine was used for the investigations as I is the total line intensity and λ is the full-width at half-
already considered in [9]. The arc from the welding torch maximum (FWHM). In the case of a Lorentz profile the fit
fixed above a movable workpiece is simultaneously observed parameter I (see equation (1)) is the ‘area under the curve’

2
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

light and h is the Planck constant. Under assumption of local


Emission coefficient [10 W m nm sr ]
-1

thermal equilibrium (LTE) the density Ni is connected to the


40
-1

total density of atoms N0 by


30  
-3

gi Ei
20 Ni = N0 (T ) · exp − , (3)
Z(T ) kT
10
6

where gi is the statistical weight of the excited state, Z(T ) is


0 the partition function, calculated according to Planck–Larkin
Fe 526.954

Fe 532.804
Fe 527.036

40

Fe 537.149
approach [20], Ei is the energy level of the excited state and T

Fe 536.993
Fe 534.102
Fe 532.418
Fe 526.331 Fe 526.655

Fe 528.362

is the temperature. Combining both expressions one obtains

Fe 536.746
30
Fe 533.993

Fe 538.337
Fe 528.179

Mn 537.763
the relation
Fe 530.230

Fe 536.540
Fe 527.337

20
 
Fe 533.266

4π εik λik N0 (T ) Ei
10 = exp − . (4)
hcAik gi Z(T ) kT
0
528 530 532 534 536 538 The left-hand side of (4) can be determined experimentally,
Wavelength [nm] the right-hand side depends only on the temperature and the
upper energy level of the transition. Plotting left hand values
Figure 2. Example of the abel inverted spectrum of iron on the axis
of the arc. Top row measurement. Bottom row fit result with
for several lines versus their upper energy levels in semi-
individual line profiles shown. Experimental conditions: Ar; logarithmic scale one should obtain the straight line known as
I ≈ 450 A; U ≈ 32 V; vwire = 4 m min−1 . Time instance T2, Boltzmann–plot where the slope yields the plasma temperature
observation at 4.1 mm above workpiece. and the extrapolated value for Ei = 0 yields the total atom
density N0 . A selection (see table 1) of the fitted lines (typically
or the total intensity of atomic transition. Performing this fit 10) with low optical depth were included in the Boltzmann–
procedure for all side-on positions yields the distribution of the plot analysis. The estimation of optical depth can be found in
radiance I (y) for a given atomic line over the y-coordinate. last column of table 1. For the estimation the Lorentzian line
It should be noted that the Lorentz profile was used during profile with 0.2 nm FWHM was assumed. The optical depth
the fit procedure only for determination of total radiation in the line centre calculated for the effective absorption length
emitted within the line profile, or ‘area under curve’. The of 1 mm is shown for the 50/50 mixture of Fe/Ar under LTE
additional information on lines widths was discarded since the conditions. The values for the typical temperature of 9000 K
accuracy was not sufficient to make statement about real Stark are given. It is obvious that although not all atomic lines can
broadening. The correct procedure should use the Voigt profile be considered as completely optically thin, the optical depth
to be able to extract the real Lorentz component of the overall does not exceed 0.4. The influence of such optical depth has
broadening combined with careful analysis of instrumental minor influence on temperature values, since it was determined
profile influence. If those requirements are fulfilled then by the Boltzmann plot procedure. The influence on the total
information on broadening of the lines can be used as an density of species lies in some underestimation of real values.
additional tool for estimation of electron density or testing the The temperature uncertainty is obtained by the estimation
theories of broadening mechanisms, like for example in [19]. of covariance matrix for the slope and intercept parameters
Under assumption of rotational symmetry of the arc, the of the Boltzmann plot. The relative uncertainty P of each
spectral emission coefficient as a function of the radial position point in Boltzmann plot is determined from the measurement
can be reconstructed from the radiance by Abel transformation. uncertainty of emission coefficient and uncertainty of the
transition probability:

2.2.1. Evaluation by means of Boltzmann plot of Fe lines.    
The radiation from the arc core was analysed in the range from εik 2 Aik 2
P = + .
526 to 540 nm. In that region many partially overlapping lines εik Aik
of atomic iron and some ionic lines are present. The integration These values serve as weights of the individual points in the
of the radiance within the line profiles was performed by Boltzmann plot. The resulting covariance matrix contains
simultaneous fitting of 19 lines with Lorentz profiles as shown variances of slope (temperature) and intercept (density).
in figure 2. The separation of overlapping lines was made
possible by this procedure.
2.2.2. Evaluation by means of single discrete argon line.
The emission coefficient εik of a line at the wavelength λik
Temperature determination by a single line method is based on
is determined by the expression
the same assumptions as already mentioned for the Boltzmann
hc plot method. Expression (4) is also valid for a single argon
εik = Ni · Aik · , (2) line. The only difference consists in additional information of
4πλik
the dependence N0 (T ) which is necessary for the temperature
where Aik is the corresponding transition probability, Ni is determination. This can be taken from the plasma composition
the density of atoms in the radiating state, c is the speed of calculations. In particular, the temperature dependence of the

3
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

Table 1. Characteristic of the iron lines selected for the Boltzmann 600 35
diagnostic method. Data taken from Kurucz spectral database [18].
500 30
Optical
Wavelength Aij Ei Ej depth 25
Nb (nm) (106 s−1 ) (eV) (eV) gi gj 0 l a 400
20

U [V]
1 526.331 5.157 3.2659 5.6211 5 5 0.038

I [A]
300
2 526.655 8.641 2.9982 5.3519 7 9 0.161 T1 T2 T3 T4 15
3 526.954 1.274 0.859 3.2114 11 9 0.376
4 527.036 2.472 1.6080 3.9600 5 3 0.093 200
10
5 527.337 0.528 2.4844 4.8352 1 3 0.006
6 528.179 3.26 3.0387 5.3856 5 7 0.045 100 5
7 528.362 7.997 3.2412 5.5873 7 7 0.086
8 530.230 6.252 3.2832 5.6211 3 5 0.046 0 0
9 532.418 15.04 3.2114 5.5396 9 9 0.223 -1 0 1 2 3 4 5
10 532.804 1.147 0.9147 3.2412 9 7 0.256 t [ms]
11 533.266 0.635 4.1866 6.5111 5 3 0.0009
12 533.993 6.978 3.2659 5.5873 5 7 0.076 Figure 3. Voltage and current profiles and exposure instances for
13 534.102 0.407 1.6080 3.9289 5 5 0.027 the OES measurements.
14 536.540 0.934 3.5735 5.8838 11 9 0.009 same, the emission coefficient. The sum in parentheses in (5)
15 536.748 57.56 4.4156 6.725 7 9 0.186
changes its value for 696 nm argon line from ≈2 × 10−3 K−1
16 536.996 47.05 4.3716 6.680 9 11 0.197
17 537.149 1.046 0.9582 3.2659 7 5 0.163 at 8000 K up to ≈2 × 10−4 K−1 at 14 000 K. Taking 20%
18 538.337 55.95 4.3128 6.6154 11 13 0.302 uncertainty of emission coefficient we obtain the absolute
a
temperature uncertainty from 100 K at 8000 K up to 1000 K
Optical depth in line centre of Lorentz profile with 0.2 nm FWHM. at 14000 K.
Effective absorption length l = 1 mm. Calculated for LTE density
of Fe atoms at 9000 K in mixture 50% Fe + 50% Ar.
3. Experimental results
neutral atom density can be calculated based on simultaneous
The current pulse profile used in the welding process is shown
solution of Saha and quasi-neutrality equations for the pure
in figure 3. The corresponding voltage profile and time
argon at the pressure of 1 bar. Under the assumption that
instances of spectroscopic measurements (labelled T1, T2 T3
the region where the metal vapour plays a remarkable role
and T4) are also shown there. The radial temperature profiles
is restricted to the spatial extent of iron radiation, the rest of
were measured at four short time instances during the high
the arc can be considered as consisting of pure argon. Then the
current phase of the process whose duration is of approximately
right-hand side of expression (4) can be calculated for different
1.5 ms. The four measurements were performed with the delay
temperatures. By comparing the experimentally determined
incremented by 270 µs and the first one placed (T1) just after
left-hand side with the calculated right-hand side the point at
the beginning of the pulse. The four radial measurements in
which both parts coincide yields the plasma temperature.
time were repeated for four different axial positions along the
The uncertainty of temperature comes from error
arc above the workpiece. The welding torch and workpiece
propagation of the measured noise of the radiance Iλ (y). The
holder were shifted simultaneously in 1 mm steps between
error propagation from radiance to the emission coefficient
measurements. This procedure was aimed at obtaining the
depends on the chosen Abel inversion algorithm which results
measurements at heights 1, 2, 3 and 4 mm above the workpiece.
in emission coefficient uncertainty εik . This can be directly
However, the workpiece deformation due to the thermal
correlated with the uncertainty of the excited atoms density
expansion led to the real measurement height which was
Ni , see equation (2). The measured value of Ni depends non-
different from the set value.
linearly on the temperature (3). The temperature uncertainty
Thus, the set of 16 radial temperature and particle density
T can be written as
profiles was obtained. Each of 16 positions was measured
 
dT dNi −1 repeatedly for 25 times. The welding process was not perfectly
T = Ni = Ni . stable and sometimes the droplet detachment in the pulse
dNi dT
previous to measurement did not occur in the right time so
The derivative dNi /dT can be found from (4): that the arc was disturbed by the droplet. To avoid the
  influence of disturbed measurements a high-speed camera
dNi 1 dN0 Ei 1 dZ
= Ni + − was used for monitoring the welding process. Measurements
dT N0 dT kT 2 Z dT with disturbance were discarded but still at least 10 repeated
and finally measurements were available for each of the 16 profiles. An
example of the arc appearance for the second point in time at
 −1
1 dN0 Ei 1 dZ Ni different heights is shown in the high-speed images in figure 4
T = + 2
− . (5) (top row).
N0 dT kT Z dT Ni
The influence of variable measurement height was
The absolute uncertainty in temperature is proportional to the accounted for by the evaluation of the high-speed images. The
relative uncertainty in the excited atom density or, which is the actual height of the measurement was determined for each

4
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

Figure 4. Examples of high-speed images. Top row—time instance T2 with underlaid measurement position pointed by laser. Bottom row
the real measurement heights for instances T1–T4. Exposure time 5 µs, neutral filter with 5% transmittance.

image corresponding to the recorded spectrum as illustrated of temperature determination from the argon line is based on
in figure 4 (bottom row). The deviation of the real height for the assumption of pure argon atmosphere. This is definitely
one measurement set (25 spectra) did not exceed 0.5 mm. A not the case at the centre of the arc where significant metal
maximum deviation of 1 mm between the real value and the vapour amount is present. Therefore, the temperature values
set value was observed. The distinction in the following text at the centre of the arc determined by this method are omitted
is made between the set value of the measurement height and in the following.
the actual measurement height. The Boltzmann plot evaluation of absolutely calibrated
The images in figure 4 are taken with a high-speed camera spectra allows determining the total density of species from
at 20 000 frames per second and exposure time 5 µs. The the intercept of linear fit with y-axis in semilogarithmic plot.
neutral filter with transmittance of 5% was used and lens The corresponding values of the neutral iron atom densities are
aperture was almost fully closed. The resulting images show shown in figure 6. The knowledge on both temperature and iron
well developed iron dominated core of the arc. The shielding atom density allows the reconstruction of the relative amount
gas radiation is barely seen in these images. The reason of metal vapour in the arc as follows. Plasma LTE composition
for this lies in the relatively small intensity of the argon calculations of Fe–Ar mixture with different amounts of iron
spectrum compared with that of iron. Images in figure 13 give the set of N0Fe (T ) functions, all of which monotonically
were taken with the same parameters but the gamma factor was decrease with temperature. Thus, for given experimental value
increased to 1.45. The argon shielding gas radiation becomes of T we obtain from calculations the possible range of total Fe
more pronounced after such manipulation. Nevertheless the atom density when the mass fraction of iron changes between
absolute instensities of the iron and argon parts of the spectrum 0% and 100%. The measured N0 value which lies in this range
differ by more than one order of magnitude. Due to the limited identifies uniquely the iron mass fraction which was present
dynamic range of the high-speed camera the real extent of the in the moment of measurement. This point indicates that the
argon radiation cannot be judged based on these images. One evaluation procedure relies heavily on the existence of LTE
have two options—either to get the image of iron dominated when plasma can be characterized by a single temperature only.
core and almost nothing from shielding gas region, or get In this case the excitation temperature of iron, determined from
overexposed core region and real extension of the shielding gas Boltzmann plot is equal to the temperature. The possibility to
region. The first option was chosen in our case. An example check the existence of LTE is generally given by the evaluation
for the mutual position of iron dominated core and shielding of lines broadening. The dominating Stark broadening
gas can be found from the comparison of the radial dependence depends on the electron temperature and density. Determining
of Ar and Fe line radiances, e.g., given our previous paper [9] those quantities from line widths information and comparing
in figure 4. The real extension of shielding gas region can be them with the excitation temperature enables one to judge on
rather found in diagrams of radial temperature distribution. the existence of LTE. Such procedure was not possible in our
As an example for reproducibility of the measurements the case. It was shown in [8, 21] that under similar experimental
complete set of the temperature profiles for time T2 at different conditions some results, such as, for example, different courses
heights obtained in the measurements is shown in figure 5. The of electron density and electron temperature profiles, indicate
welding process is not a perfectly repeatable one which causes possible limitations in LTE applicability. Nevertheless the
differences in the plasma properties between two sequential equality of electron and excitation temperatures was shown
current pulses. This fact is illustrated by the spreading in central regions of the arc column, where our Boltzmann
of the measured profiles. The difference in temperature is plot evaluation is also applied.
about 1000 K for measurements based on the Boltzmann plot For each of the four times, the four typical profiles of
evaluation for iron and 500 K for single line measurements of temperature and density were selected from the corresponding
argon except for arc fringes. It should be noted that the method sets similar to those shown in figures 5 and 6. The resulting

5
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

13 13

(a) (b)
12 12

Temperature [kK]
Temperature [kK]

11 11

10 10

9 9

8 8

7 7
0 2 4 6 8 10 12 0 2 4 6 8 10 12
radial position [mm] radial position [mm]

13 13

(c) (d)
12 12
Temperature [kK]

11 Temperature [kK] 11

10 10

9 9

8 8

7 7
0 2 4 6 8 10 12 0 2 4 6 8 10 12
radial position [mm] radial position [mm]

Figure 5. Set of temperature profiles for time instance T2 obtained after evaluation of repeated spectral measurements; (a) set 1 mm (real
average 0.8 mm), (b) 2 mm (1.7 mm), (c) 3 mm (3.4 mm) and (d) 4 mm (4.1 mm) above the workpiece. Results of both Boltzmann plot
evaluation of Iron lines and single line analysis of argon are presented. The results of single line analysis are not valid in the presence of
metal vapour. Temperature values at the arc centre are given by iron line analysis.

16 profiles of temperature and iron mass fraction are shown be used for the estimation of the electric field based on the
in figures 7 and 8. The uncertainty of the temperature following consideration. The total electric current flowing
measurements is shown by the error bars on the selected perpendicular to the horizontal cross-section of the arc is
temperature profiles in figure 7. The uncertainty of the metal defined by
fraction can be roughly estimated to be equal to 50% based on   R
the data in figure 6.
I= j dA = 2π Ez σ (r)r dr, (6)
As can be seen in figure 7, a temperature minimum occurs S 0
in the arc centre where a significant amount of iron can be
found. These results conform to the measurements reported where jz (r) = σ (r)Ez is the current density, R is the arc radius.
earlier [6, 9]. The metal vapour constitutes up to 50% of the Here rotational symmetry and electric field Ez constant over
gas at the centre of the arc. The data in figure 8 show that the arc cross-section is assumed. The integrals on the right-
the metal vapour concentration increases with distance from hand side can be calculated based on data shown in figure 9,
the workpiece. In the beginning of the high current phase the and the electric field is obtained for the given current for the
metal vapour seems to be distributed uniformly along the axis respective axial position.
of the arc (figure 8(a)). Later in the current pulse the vapour The estimations of electric field are summarized
concentration near the workpiece decreases. in figure 10. The increase in the electric field with increasing
The information on mass fraction of iron and temperature distance from the workpiece becomes obvious.
gives the possibility to determine the radial profiles of the
electric conductivity. The results of the calculations are 4. Numerical simulation
shown in figure 9. The data of conductivity dependence
on temperature were taken from [22]. The presence of the For the numerical simulation of the GMAW arc, we use
metal vapour reduces the electric conductivity in the arc centre the commercial simulation software ANSYS CFX. The used
approximately by 30%. The electric conductivity profiles can numerical model focuses on a detailed description of the

6
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

8 8

7 (a) 7 (b)
6 6

NFe [10 m ]
NFe [10 m ]

5 5

-3
-3

4 4

22
22

3 3

2 2

1 1

0 0
0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0
radial position [mm] radial position [mm]
8 8

7 (c) 7 (d)
6 6
NFe [10 m ]

5 NFe [10 m ] 5
-3

-3

4 4
22

22

3 3

2 2

1 1

0 0
0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0
radial position [mm] radial position [mm]

Figure 6. Set of neutral iron density profiles for time instance T2 obtained after evaluation of repeated spectral measurements; (a) set 1 mm
(real average 0.8 mm), (b) 2 mm (1.7 mm), (c) 3 mm (3.4 mm) and (d) 4 mm (4.1 mm) above the workpiece.

physical processes in the arc and neglects the influence of At the fluid–solid interface of the wire, we define an
metal transfer. In the rotationally periodic steady-state model, additional mass flux which includes the formation of metal
we treat the wire electrode and contact tube, the shielding gas vapour. The formulation of the mass flux term is based on an
nozzle and the workpiece as solid bodies separated from the assumed vaporization profile, shown in figure 11. The integral
fluid region by fluid–solid interfaces with a fixed geometry, value of the mass flux is related to the feeding rate of the wire.
see figure 11. At the ambient regions (GHIJ), we assume a perfect shielding
In the solid domains for the wire (see the range ABPQN gas cover. A detailed description of the MHD-equation system
in figure 11) and contact tube (BCQR), the shielding gas could be found in [14, 24].
nozzle (DGFE) and the workpiece (MJKL), we solve only In our calculations, we consider a pulsed GMAW process
for the conjugated heat transfer, the electric potential and the using argon as the shielding gas. The wire and the workpiece
magnetic vector potential. In the fluid domain (remaining part are assumed to be iron. Due to vaporization effects, the
in figure 11), we solve an MHD equation system. The heat shielding gas is loaded by iron vapour. The plasma is assumed
loss due to radiation processes is treated by a net emission to be in LTE. Density, specific heat, thermal and electric
coefficient model. conductivity, and viscosity as well as the combined diffusion
The equations for energy, electric potential and magnetic coefficients are taken from the datasets of Murphy for argon–
vector potential are solved in a unified matrix and need no iron mixtures [22]. The net emission coefficients for argon–
boundary conditions at the fluid–solid interfaces. The mass iron mixtures are taken from the datasets of Menart and
and momentum equations are solved only in the fluid domain, Malik [25].
assuming no slip walls at the fluid–solid interfaces. A specific approach is used for the numerical simulation
The content of metal vapour in the shielding gas is of the arc at different times in the pulse phase of the
calculated, using the demixing model of Murphy [22]. In pulsed GMAW in correspondence with the OES measurements
addition to the convective and diffusive mixing, turbulent (compare figure 3). At the time points of measurements, the
effects are taken into account using the SST turbulence arc is assumed to be nearly in steady state and the droplet
model [23]. has not been detached already. The properties of the arc are

7
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

14 14

(a) (b)
Temperature [10 K]

Temperature [10 K]
13 13
3

3
12 12

11 3.79 mm 0.86 mm 11 0.8 mm


1.31 mm
10 10
3.4 mm 1.72 mm
9 3.35 mm 9
4.1 mm
8 8
0 1 2 3 4 5 6 7 8 9 10 11 12 0 1 2 3 4 5 6 7 8 9 10 11 12
radial position [mm] radial position [mm]

14 14

(c) (d)
Temperature [10 K]

Temperature [10 K]
13 13
3.4 mm
3

12 3 12

11 11
0.64 mm
10 10 0.7 mm
3.2 mm
9 9 4.4 mm
4.2 mm 2 mm
1.7 mm
8 8
0 1 2 3 4 5 6 7 8 9 10 11 12 0 1 2 3 4 5 6 7 8 9 10 11 12
radial position [mm] radial position [mm]

Figure 7. Resulting temperature profiles for four time instances and different heights; (a) T1, (b) T2, (c) T3 and (d) T4. The real
measurement heights above the work piece are marked.

mainly influenced by the vaporization rate at the wire, since the mass fraction of iron and electric conductivity for two spatial
transport of metal vapour with the arc flow and the radiation positions are plotted in each diagram. The arc length of 7 mm
are high and therefore cause much smaller time scales as the was considered in the simulations corresponding to the average
vaporization rate changes. length in the experiment. The comparison is made for the
However, the amount of metal vaporized at the wire middle of the arc—approximately 4 mm and for the position
electrode can only be estimated in the model used, since the approximately 1 mm above the workpiece.
flow and the heat convection are not solved in droplet and Experimental and calculated temperature profiles in
no self-consisted formulation of vaporization is implemented. figure 12 show a similar structure—minimum at the centre
The vaporization rate is the most sensitive unknown in the and broader wings at the periphery. Differences in the absolute
model. Based on the finding of earlier papers [26], that values reach from 1000 in the arc core (iron vapour dominated)
the amount of evaporation affects mainly the diameter and and 3000 K in the adjacent region (argon dominated) in the
the shape of the metal vapour arc core, we varied gradually the instance T1 and 4000 K in the arc core and 2000 K in the
metal vaporization rate between 1% and 8% related to the adjacent region for time instance T4. The experimental
wire feed rate of 4 m min−1 or 6–48 mg s−1 , respectively. uncertainty in temperature determination (see figure 7) is much
The resulting arc shapes were compared with high-speed smaller than these discrepancies. The discrepancy in the
images and OES measurements. The best match was found arc core can be explained by the different amounts of metal
for T1 with 2%, for T2 with 3%, for T3 with 4%, and for T4 vapour in experiment and model. The discrepancy in the
with 5% evaporation related to the wire feed rate. Thus the adjacent region can be explained by the systematic error in the
model indicates that the vaporization rate is increasing during measurements which is due to the limited spacial resolution of
the pulse. the optical system. The temperature profiles determined with
the argon line method cannot resolve the region adjacent to the
5. Comparison of experiment and simulation arc core and give smeared temperatures with lower amplitude.
Also, the experimental temperature profiles are broader in the
The comparison of the simulation results and experimental fringes of the arc than the calculated ones, in particular near to
values are shown in figure 12. The data for temperature, the workpiece. A possible explanation can lie in the deviation

8
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

60 60

(a) (b)
Mass fraction of Iron [%]

Mass fraction of Iron [%]


50 50
4.1 mm
40 40
3.35 mm
30 30

20 20
3.4 mm
1.72 mm 0.8 mm
10
3.79 mm 0.86 mm 10

1.31 mm
0 0
0.0 0.5 1.0 1.5 2.0 0.0 0.5 1.0 1.5 2.0
radial position [mm] radial position [mm]

60 60

(c) (d)
Mass fraction of Iron [%]

Mass fraction of Iron [%]


4.4 mm
50 50
4.2 mm
40 40
3.4 mm 3.2 mm
30 30
2 mm
20 20 0.7 mm
0.64 mm

10 10 1.7 mm

0 0
0.0 0.5 1.0 1.5 2.0 0.0 0.5 1.0 1.5 2.0
radial position [mm] radial position [mm]

Figure 8. Resulting Iron mass fraction profiles for four time instances and different heights; (a) T1, (b) T2, (c) T3 and (d) T4. The real
measurement heights above the work piece are marked.

from the LTE assumption. On the one hand the description of field values on the arc axis from the MHD simulations (also
the plasma with single temperature is then inconsistent. On given in figure 10). A sufficient agreement is obtained. The
the other hand the temperature profiles in the fringes were values of the conductivity in fringes of the arc are probably
obtained with the evaluation of single argon line with the help overestimated in the measurements and underestimated in the
of equation (4). This evaluation procedure is underlined with simulation which lead to the larger values of axial electric field
the LTE calculation of the plasma composition and is known to in the simulation.
lead to overestimations of the temperature [27, 28]. Possible In addition to the spectroscopic measurements, the high
reasons for deviations in the simulation are discussed later in speed images of the arc can also be used to evaluate the
this section. accuracy of the simulation. The simulation model considers
The experimentally defined iron mass fraction is by a the local net radiation emission within the arc. Hence, the
factor of about two lower than the simulation results. The side-on view of the arc, e.g. the side-on radiance, can be
discrepancy is likely to be caused by the non-self-consistent calculated by integrating the radiation emission in a certain
description of the metal vapour in the simulation. In addition, direction. Assigning colours to the radiation according to
the limited accuracy and reproducibility in the experimental the wavelength—blueish for iron radiation whose visible part
determination of the iron atom densities (compare values lies presumably in the range 400–550 nm and reddish for
in figure 6) must be considered. However, a sufficient the argon radiation whose visible part lies mostly in the
qualitative coincidence is obtained—broader profiles with range 600–800 nm—one obtains images shown in the right
lower amplitude near the workpiece and narrower profiles with column of figure 13. These images can be compared with
higher amplitude in the arc centre. experimental images taken by the high-speed camera (left
The electric conductivity profiles show similar qualitative column of figure 13). A quite good agreement of the arc
structure. The remaining discrepancies are mostly associated structure is obtained expect for an underestimation of the width
with the similar deviations in the temperature profiles. of the argon range in the simulation.
The electric field given in figure 10 determined from In addition to the non-self-consistent description of the
the measurements can be compared with the axial electric metal evaporation another incompletion of the simulation

9
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

8 8

electric conductivity [10 Ω m ]

electric conductivity [10 Ω m ]


-1

-1
-1
(a) (b)

-1
3.35 mm
6 6
3

3
4 0.86 mm 4
0.8 mm
1.31 mm
4.1 mm 1.72 mm
2
3.79 mm 2 3.4 mm

0 0
0 2 4 6 8 10 12 0 2 4 6 8 10 12
radial position [mm] radial position [mm]
8 8
electric conductivity [10 Ω m ]

electric conductivity [10 Ω m ]


-1

-1
(c) (d)
-1

-1
6 6
3

3
4 4
0.64 mm 0.7 mm

2
4.2 mm 2 mm 2 3.2 mm
3.4 mm
4.4 mm 1.7 mm

0 0
0 2 4 6 8 10 12 0 2 4 6 8 10 12
radial position [mm] radial position [mm]

Figure 9. Resulting electric conductivity profiles for four time instances and different heights; (a) T1, (b) T2, (c) T3 and (d) T4. The real
measurement heights above the work piece are marked.

18

16

14
electric field [V/cm]

12

10

6 ( ) T1
4 ( ) T2
( ) T3
2
( ) T4
0 Figure 11. Computational domain of the GMAW arc model [14].
0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 4.5 5.0 5.5
axial position [mm]
and its re-absorption in other spatial regions is not included
Figure 10. Comparison of axial electric field determined according in this approach. It is expected by the authors that the
to (6) (open symbols) and simulation result (full symbols). inclusion of an appropriate radiation transport model in the
MHD simulation will lead to broader temperature profiles and
model may be a main reason for remaining deviations between reduce the deviations. This inclusion is planned for future
experimental and simulation results. This concerns the modelling work.
approach of the net emission coefficient to describe the
radiation loss in the arc. The net emission approach considers 6. Conclusion
to some extent not only the local radiation emission but also
the local radiation absorption and enables an overall sufficient The high current phase of a pulsed GMAW process in argon
description of the arc energy balance. However, the transport in globular mode has been investigated. Radial profiles of
effect by radiation emission in one spatial region of the arc temperature, mass fraction of iron and electric conductivity

10
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

1.0 10

electric conductivity [10 Ω m ]


-1
16

-1
mass fraction of Iron [%]
0.8 8
14

3
Temperature [kK]

0.6 6
12

10 0.4 4

8 0.2 2

6 0.0 0
0 2 4 6 8 10 12 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0 2 4 6 8 10 12
radial position [mm] radial position [mm] radial position [mm]

1.0 10

electric conductivity [10 Ω m ]


-1
16

-1
mass fraction of Iron [%] 0.8 8

3
14
Temperature [kK]

0.6 6
12

0.4 4
10

8 0.2 2

6 0.0 0
0 2 4 6 8 10 12 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0 2 4 6 8 10 12
radial position [mm] radial position [mm] radial position [mm]

1.0 10

electric conductivity [10 Ω m ]


-1
16

-1
mass fraction of Iron [%]

0.8 8

3
14
Temperature [kK]

0.6 6
12

0.4 4
10

8 0.2 2

6 0.0 0
0 2 4 6 8 10 12 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0 2 4 6 8 10 12
radial position [mm] radial position [mm] radial position [mm]

1.0 10
electric conductivity [10 Ω m ]
-1

16
-1
mass fraction of Iron [%]

0.8 8
3

14
Temperature [kK]

0.6 6
12

0.4 4
10

8 0.2 2

6 0.0 0
0 2 4 6 8 10 12 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 0 2 4 6 8 10 12
radial position [mm] radial position [mm] radial position [mm]

Figure 12. Comparison of simulation results (solid curves) and experimental values (symbols). Left column—temperatures, middle
column—mass fraction of iron and right column—electric conductivity. Time instances from T1 (top) to T4 (bottom). Black curves
represent approximately 1 mm above the workpiece, blue curves represent approximately middle of the arc.

at different heights above the workpiece were determined by to describe the arc at the points in time which has been
optical emission spectroscopy and the analysis of iron and investigated in the measurements.
argon atom lines under the assumption of LTE. Experimental Very similar structures and a sufficiently good quantitative
errors are estimated which are quite low at least in the case agreement in the plasma properties have been obtained in
of the temperature, except for the outer arc fringes. The axial the simulation and in the measurements which is assessed
electric field was also estimated based on the measurement as a general validation of both the simulation model and the
results. A magneto-hydrodynamic model of the arc assuming experimental method. Therefore, the model is well suited to
rotational symmetry, steady-state and LTE and considering study the basic physical mechanisms which lead to the arc
the admixture of iron vapour in argon, the resulting change structure with peculiarities like the strong radiation and the low
of the thermodynamic and transport properties and the net temperature and conductivity in the metal dominated arc core.
emission as well as demixing and turbulence has been adapted The detailed discussion of the arc structure and the underlying

11
J. Phys. D: Appl. Phys. 46 (2013) 224001 R Kozakov et al

Effort should also be spent to improve the description of the


metal evaporation at the melted wire tip which probably will
decrease the present overestimation by the model.

Acknowledgments

This work was supported by the DFG (grant no. UH 106/3-1,


WE 4416/1-1, FU 307/5-110).

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