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Environmental impacts of takeaway food containers

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DOI: 10.1016/j.jclepro.2018.11.220

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Journal of Cleaner Production 211 (2019) 417e427

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Journal of Cleaner Production


journal homepage: www.elsevier.com/locate/jclepro

Environmental impacts of takeaway food containers


Alejandro Gallego-Schmid a, b, *, Joan Manuel F. Mendoza a, Adisa Azapagic a
a
Sustainable Industrial Systems, School of Chemical Engineering and Analytical Science, The University of Manchester, The Mill, Sackville Street,
Manchester, M13 9PL, UK
b
Tyndall Centre for Climate Change Research, School of Mechanical, Aerospace and Civil Engineering, The University of Manchester, HG1, Pariser Building,
Sackville Street, Manchester, M13 9PL, UK

a r t i c l e i n f o a b s t r a c t

Article history: The consumption of takeaway food is increasing worldwide. Single-use containers used for takeaway
Received 11 September 2018 food represent a significant source of waste and environmental impacts due to their low recyclability.
Received in revised form Consequently, it is important to identify the best available alternatives and improvement opportunities
21 November 2018
to reduce the environmental impacts of fast-food containers. For these purposes, this study estimates
Accepted 23 November 2018
Available online 24 November 2018
and compares for the first time the life cycle impacts of three most widely-used types of takeaway
container: aluminium, polypropylene and extruded polystyrene. These are also compared to reusable
polypropylene containers. The findings suggest that single-use polypropylene containers are the worst
Keywords:
Aluminium
option for seven out of 12 impacts considered, including global warming potential. They are followed by
Global warming the aluminium alternative with five highest impacts, including depletion of ozone layer and human
Fast food toxicity. Overall, extruded polystyrene containers have the lowest impacts due to the lower material and
Packaging electricity requirements in their manufacture. They are also the best option when compared to reused
Polypropylene takeaway polypropylene containers, unless the latter are reused 3e39 times. The number of uses needed
Extruded polystyrene for the reusable “Tupperware” polypropylene food savers is even higher, ranging from 16 to 208 times,
with terrestrial ecotoxicity being always higher than for extruded polystyrene, regardless of the number
of uses. However, extruded polystyrene containers are currently not recycled and cannot be considered a
sustainable option. If they were recycled in accordance with the European Union 2025 policy on waste
packaging, most of their impacts would be reduced by >18%, while also reducing littering and negative
effects on marine organisms. Most of the impacts of the other two types of container would also be
reduced (>20%) through increased recycling. Implementing the European Union 2025 policy on recycling
of waste packaging would reduce all the impacts by 2%e60%, including a 33% reduction in global
warming potential. Based on 2025 million takeaway containers used annually in the European Union, the
latter would save 61,700 t CO2 eq./yr, equivalent to the emissions of 55,000 light-duty vehicles. The
outcomes of this study will be of interest to packaging manufacturers, food outlets, policy makers and
consumers.
© 2018 Elsevier Ltd. All rights reserved.

1. Introduction home and work). If it is consumed away from the food outlet, it is
known as takeaway or take-out food. The takeaway food market
Consumption of fast food is increasing rapidly as a consequence has been growing fast due to the convenience and competitive
of modern lifestyles (Razza et al., 2009). Fast food is defined as the pricing. According to TechNavio (2016), the global delivery and
sale of food and drink for immediate consumption after purchase takeaway food market, which was valued at $89 billion in 2015, is
(Market Line, 2012), either at the food outlets or elsewhere (e.g. expected to grow by 2.7% annually to over $102 billion by 2020.
The increasing importance of the takeaway food sector has
given rise to various sustainability concerns, including food safety
(Meldrum et al., 2009) and labour issues (Schmitt and Jones, 2013).
* Corresponding author. Tyndall Centre for Climate Change Research, School of
Mechanical, Aerospace and Civil Engineering, The University of Manchester, HG1, However, there are also important environmental sustainability
Pariser Building, Sackville Street, Manchester, M13 9PL, UK. issues associated with the takeaway food supply chain. One of these
E-mail addresses: alejandro.gallegoschmid@gmail.com, alejandro. is the use of non-reusable containers with a low recyclability
gallegoschmid@manchester.ac.uk (A. Gallego-Schmid).

https://doi.org/10.1016/j.jclepro.2018.11.220
0959-6526/© 2018 Elsevier Ltd. All rights reserved.
418 A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427

potential (MacKerron, 2015). Based on previous studies (AFCMA, results of this study will be of interest to EU policy makers, food
2004; Alupro, 2016; Cassidy and Elyashiv-Barad, 2007), the esti- packaging manufacturers, fast-food outlets and consumers, helping
mates in the current research suggests that over 7.5 billion them to identify environmentally most sustainable food container
extruded polystyrene (EPS) containers are used annually in the USA options and make informed choices.
and more than 1.8 billion aluminium containers in the UK. This
results in the annual consumption of 58,500 t of EPS in USA and 2. Methods
13,680 t of aluminium in the UK. Taking into account their extrac-
tion and processing, this is equivalent to the emissions of 297 Mt The environmental impacts of the containers have been esti-
and 167 Mt of CO2 eq. per year, respectively. mated using LCA, which has been carried out in accordance with
The environmental concerns associated with the use of these the ISO 14040/44 (ISO, 2006a,b) guidelines. The next section de-
containers have been highlighted in several studies (Aarnio and scribes the goal and scope of the study, followed by the inventory
Ha €ma€la
€inen, 2008; Mason et al., 2004; Shokri et al., 2014). How- data and the impact assessment methodology applied in the study.
ever, most focused on waste generation and management rather
than applying a full life cycle perspective. At present, there are no 2.1. Goal and scope of the study
life cycle assessment (LCA) studies of takeaway containers. Related
studies have analysed the environmental impacts associated with The goals of this study are:
the use of biodegradable materials (e.g. Madival et al., 2009; Razza
et al., 2009; Suwanmanee et al., 2013). Other studies considered i) to estimate and compare the environmental impacts of three
reusable cups (e.g. Potting and van der Harst, 2015; Vercalsteren commonly-used takeaway food containers: aluminium, EPS
et al., 2010; Woods and Bakshi, 2014). Furthermore, Rieradevall and PP;
et al. (2000) discussed the implementation of eco-design criteria ii) to assess the environmental implications of reusing PP
to fast-food packaging. takeaway containers and using reusable PP food savers
One of the most critical environmental aspects related to single- (Tupperware) instead of single-use containers; and
use takeaway containers is waste generation. In an attempt to iii) to evaluate the environmental effects of different end-of-life
address this issue, consumers are being encouraged by some management options for the takeaway containers at the EU
groups (e.g. Takeout without, 2016; Tiffin Project Foundation, 2012) level.
to bring their own reusable food container from home and refuse
single-use containers used by fast-food outlets. Some companies The functional unit for the first two goals of the study is defined
have also started to offer discounts to customers for bringing as “production, use and disposal of a container storing a meal for one
reusable cups or selling its side dishes in reusable containers (e.g. person”. The volume of the container considered is 670 ml. This
Mohan, 2010; Starbucks, 2016). In some countries, policy makers represents an average across the takeaway containers, determined
are also considering taxation of single-use food containers. For through own fieldwork and information provided by manufac-
example, the UK government has recently issued a call for evidence turers. For the end-of-life options, the functional unit corresponds
to justify the use of taxation aimed at reducing the demand for to the “total number of takeaway containers used annually in the EU”.
single-use plastics, such as takeaway boxes (HM treasury, 2018). The containers considered in the study are shown in Fig. 1.
However, while it is intuitively plausible that reusable food con- Aluminium and EPS containers have been chosen for study as they
tainers are environmentally better than their single-use counter- are used most commonly (Rieradevall et al., 2000). As shown in
parts, as far as the authors are aware, no study has yet quantified Fig. 1A, in addition to the aluminium body, the aluminium
the actual environmental implications of different takeaway food container also has a paper lid. In the EPS container, the body and the
containers and how they compare with their reusable alternatives. lid are integrated and made of a single material (Fig. 1B). Light-
Therefore, this paper assesses for the first time life cycle environ- weight PP containers are also used widely in the takeaway in-
mental impacts of three types of container typically used by take- dustry and they are more robust and durable than the other two
away food outlets to serve hot food e aluminium, EPS and types (Fig. 1C). Consequently, even if it is usually considered a
polypropylene (PP) e in comparison with reused takeaway PP single-use product, environmentally-conscious customers may opt
containers and “Tupperware” food savers (also made of PP) used by
many consumers worldwide. The number of times the reusable
containers should be reused to balance out the impacts of single-
use containers is also considered.
The geographical area selected for this study is the European
Union (EU) because the number of takeaway outlets has increased
rapidly in recent years and is expected to grow even faster in the
future (Accorsi et al., 2014; Daedal Research, 2014). The UK, Ger-
many, France, Italy and Spain are among the top 13 world con-
sumers of takeaway food, with an expenditure of V9.9 billion in
2014, expected to increase by 17% by 2019 (Lago et al., 2011; Riera,
2015). The focus on the EU is also due to the European Commission
recently adopting an ambitious circular economy package, which
includes revised legislative proposals for packaging waste,
encouraging the recycling of aluminium and plastic packaging that
will also affect takeaway containers (European Commission,
2015a,b). Therefore, there is a need to quantify the impacts asso-
ciated with packaging in the takeaway food sector at EU level, as
Fig. 1. Types of food containers considered in the study. A: Aluminium takeaway
well as the effect of future waste management legislation. Hence, container; B: Extruded polystyrene takeaway container; C: Polypropylene takeaway
this paper also assesses the environmental effects of current and container; D: Polypropylene reusable food saver (Tupperware). [Dimensions (mm):
future end-of-life scenarios for takeaway containers at EU level. The Aluminium: 195x105x48; EPS: 170x133x75); PP (standard size: 160x105x48.].
A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427 419

to reuse it. This is not possible for the EPS and aluminium con-  Production: thermoforming and extrusion for PP, silicone, PE
tainers as they are not sturdy enough and cannot be cleaned easily. and PS, aluminium sheet rolling and metal stamping, PE coating
Nevertheless, to make PP containers comparable with the other of paper and packaging
two types, they are assumed in the base case to be used only once  Use: manual and automatic washing (only for reusable
(study goal i)). The environmental implications of their reuse are containers)
explored as part of the study goal ii), together with the use of  End-of-life: wastewater treatment and disposal of post-
reusable Tupperware food savers. The latter have been selected for consumer waste and;
study as they are used widely in Europe (Gallego-Schmid et al.,  Transport:
2018). Tupperware food savers are commonly made of PP because o packaging and raw materials to the production site;
other common plastics have lower resistance to high temperatures o containers to food outlet; and
(Fellows and Axtell, 1993). o production and end-of-life waste to waste management
Although paper and cardboard takeaway containers are also facility.
used, they are much less common as they are less suitable for ‘wet’
food (e.g. served with a sauce). Hence, they are not considered in For the reusable Tupperware food saver, transport of consumer
the study. to and from the retailer to buy the container and to and from the
The scope of the study and the system boundaries are depicted food outlet is excluded. The main reason is the uncertainty related
in Fig. 2. As shown, the following stages have been considered: to consumer behaviour and to the allocation of the impacts to the
food container relative to other items and activities.
 Raw materials:
o polypropylene (PP) and silicone;
o aluminium; 2.2. Inventory data
o polystyrene (PS); and
o cardboard, paper and polyethylene (PE) (for packaging and for The inventory data are detailed in Table 1. These have been
the lid of the aluminium container) calculated through direct measurements (weighing of components)
and primary production data obtained from major producers.

Fig. 2. System boundaries for the different types of container considered in the study. [PP: polypropylene; EPS: extruded polystyrene].
420 A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427

Table 1
Life cycle inventory data for takeaway containers.

Life cycle stage Aluminium Extruded polystyrene Polypropylene Polypropylene food saver (Tupperware)
container container container

Raw materials
Polypropylene (g) e e 31.5 132.8
Aluminium (g) 7.6 e e e
Polystyrene (g) e 7.8 e e
Silicone (g) e e e 8.5
Paper (g) 6.6 e e e
Polyethylene (lid) (g) 0.3 e e e
Packaging
Cardboard (g) 1.5 1.8 2.1 7.7
Polyethylene (g) 0.06 0.07 0.09 0.3
Productiona
Extrusion: electricity (J) e 28.1 57.5 258.4
Thermoforming: electricity (J) e 28.0 112.6 506.1
Sheet rolling: electricity (J) 15.0 e e e
Sheet rolling: heat (J) 14.5 e e e
Metal stamping: electricity (J) 47.4 e e e
Metal stamping: heat (J) 42.9 e e e
Paper lid production: heat (J) 0.01 e e e
Paper lid production: electricity (J) 4.2 e e e
Packaging: heat (J) 0.05 0.06 0.07 0.3
Packaging: electricity (J) 0.7 0.9 1.1 3.8
Transport
Raw materials: transport to factory (kg.km) 2.4 1.5 5.0 22.4
Container: factory to Shanghai port (kg.km) 2.4 e 5.0 22.4
Container: Shanghai to Rotterdam (kg.km) 314.3 e 656.4 2911.2
Container: Rotterdam to Munich (kgt.km) 13.4 e 27.9 123.8
Container: factory to Munich (kg.km) e 4.8 e e
Container: Munich-retailer (kg.km) 2.4 1.5 5.0 22.4
End-of-life: transport waste treatment (kg.km) 0.8 0.5 1.7 7.5
Use (machine dishwashing)
Electricity (J) e e 57.5 57.5
Soap (g) e e 0.2 0.2
Salt (g) e e 0.2 0.2
Rising agent (g) e e 0.03 0.03
Water (L) e e 0.2 0.2
Use (manual washing)
Heat: electricity (J) e e 9.5 9.5
Heat: natural gas (J) e e 23.4 23.4
Heat: oil (J) e e 3.2 3.2
Heat: solar thermal (J) e e 1.0 1.0
Water (L) e e 1.4 1.4
Soap (g) e e 0.5 0.5
End-of-life waste management
Recycling: plastics (g) e e 3.4 14.4
Recycling: aluminium (g) 4.1 e e e
Recycling: cardboard (g) 1.3 1.5 1.8 6.5
Incineration: plastics (g) e 3.9 13.8 58.4
Incineration: cardboard (g) 3.8 0.2 0.2 0.6
Landfilling: plastics (g) 0.06 4.0 14.3 68.5
Landfilling: aluminium (g) 3.5 e e e
Landfilling: cardboard (g) 3.3 0.1 0.2 0.5
a
Electricity mix in 2015: EU28 for EPS and China for the other three types of container. Heat: natural gas.

Ecoinvent v3.3 (Ecoinvent Centre, 2016) has been used as the pri- container vendor (Papstar, 2016a). The containers are assumed to
mary source of background data and any data gaps have been filled be produced in China, the main producer of aluminium foil in the
using the GaBi database (Thinkstep, 2016) and literature. World (Pani, 2015; Xie et al., 2011).
Polystyrene containers used in the takeaway industry are nor-
2.2.1. Raw materials and production of containers mally made of extruded polystyrene (Glenn et al., 2001; Marin
The aluminium container is composed of the aluminium body et al., 2004). The average weight of EPS containers has been esti-
and a paper lid with a thin polyethylene coating on the internal mated based on the data obtained from food outlets and different
side. An average weight has been considered based on the samples producers in Europe (FPA, 2016). The data for the EPS production
obtained from food outlets and different sellers in Europe (EAFA, have been sourced from Ecoinvent while the amount of blowing
2016a). Ecoinvent data for sheet rolling for the production of the agent (butane) is from Ingrao et al. (2015). The packaging data for
aluminium foil and impact extrusion for shaping the container have the containers have been obtained from an EPS container vendor
been used. Data for liquid packaging board have been used to (Papstar, 2016b). The production of EPS is assumed to be in Europe
model the production of the paper lid (Vercalsteren et al., 2010; because the leading producers are located in the Netherlands,
Ligthart and Ansems, 2007; Rieradevall et al., 2000). The packaging Luxemburg, Belgium or Germany (Plastics Europe, 2015; van der
data for the containers have been obtained from an aluminium Harst et al., 2014).
A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427 421

For the PP containers (takeaway and reusable Tupperware food 2.2.3.2. Waste management at the EU level. The European
savers), primary production data have been obtained from a major Commission (2015b) has proposed that 75% of aluminium and
producer, including the amount and type of raw and packaging 55% of plastic packaging waste should be recycled by 2025. This is
materials and a detailed description of production (Table 1). A sil- in line with the EU's approach to waste management based on the
icone rubber is also used in food-savers as part of the lid to ensure waste hierarchy (European Parliament, 2008), which sets the
tight closure. Both PP and silicone are extruded and thermoformed following priority order for waste: prevention, reuse, recycling,
to obtain the desired shape. According to Suwanmanee et al. (2013), recovery and, as the least preferred option, disposal (which in-
most of the manufacturing of plastic containers is located in South cludes landfilling and incineration without energy recovery). Based
East Asia. Therefore, the production of PP containers is considered on these, the following scenarios have been considered for the end-
to be located in China and its electricity grid mix has been used in of-life waste management of the takeaway containers:
LCA modelling.
 current situation;
 best case: implementation at the EU28 level of the best current
2.2.2. Use end-of-life waste management in an EU country according to
No impacts have been considered for the single-use takeaway the EU waste hierarchy;
containers. For the reused PP takeaway containers and Tupperware  EU 2025 proposal: the implementation in EU28 of waste man-
food savers, the impacts of their cleaning, either in a dishwasher or agement proposed by the European Commission for 2025
by hand, have been considered. The inventory data for this are (European Commission, 2015b); and
based on Gallego-Schmid et al. (2018), recalculated for the size of  worst case: for comparison, the implementation at the EU28
the container considered here (from 1100 to 670 ml). level of the worst current end-of-life management in an EU
country according to the EU waste hierarchy.
2.2.3. End-of-life waste management
The specific data for each container are described below and are
2.2.3.1. Single containers. The assumptions for end-of-life man- summarised in Table 2:
agement of each type of the container can be found in Table 1. The
‘net scrap’ approach has been applied for recycling (Bergsma and  Aluminium containers: Two scenarios has been analysed with
Sevenster, 2013). This means that the system has been credited the increase in the recycling rate from the current 54%e75% and
only for the percentage of recycled material that exceeds the 89%. The first increase is the EU's proposed goal for 2025
recycled content in the original raw materials. For example, (European Commission, 2015b) and the second is the current
aluminium is initially made up of 32% recycled and 68% virgin recycling rate of aluminium packaging in Germany, the highest
metal, but 54% is recycled at the end-of-life of the container. among all 10 EU countries with available data (Eurostat, 2016).
Therefore the system has been credited for recycling 22% of Finally, as the worst scenario, the current 22% recycling ratio of
aluminium (54% minus 32%) at the end of its life. The impact from the Czech Republic has been considered (Eurostat, 2016).
the recycling process are also included. The system has also been  EPS containers: Two scenarios of 100% incineration with energy
credited for the electricity generated by incineration of waste ma- recovery (currently in Austria and Sweden) and 100% landfilling
terials. The EU electricity mix in year 2014 (ENTSO-E, 2016) has (Greece, Croatia, Cyprus, Lithuania and Malta) have been
been used for these purposes. Data for all waste and wastewater assessed (Eurostat, 2016). A third scenario of 55% recycling and
treatments have been sourced from Ecoinvent, except for PP recy- 45% incineration with energy recovery has been considered
cling, which are from Schmidt (2012). based on the EU proposal for plastic packaging in 2025
The following assumptions have been made for end-of-life of (European Commission, 2015b).
different materials:  PP containers: Similar to the aluminium containers, the best and
worst current performance at country level and the proposal for
 for PP, data for non-bottle rigid PP packaging treatment in the the EU by 2025 have been considered as alternative scenarios.
EU28 have been considered: 44% incineration with energy re- According to the priority order of the EU waste hierarchy, Ger-
covery, 11% recycling and 45% for landfilling (Lho ^te, 2011); many has the best treatment ratios for non-bottle rigid PP
 for aluminium, 54% of the aluminium has been considered be packaging (30% recycling, 69% incineration with energy recovery
recycled and 46% landfilled (Eurostat, 2016; EAFA, 2016b); and 1% landfilling) and the UK has the worst (2% recycling, 8%
 EPS containers are generally not recycled and are either land- incineration with energy recovery and 90% landfilling) out of the
filled or incinerated (Belley et al., 2011; Davis and Song, 2006; five countries (France, Germany, Poland, Spain and UK) with
Ingrao et al., 2015). Considering the data for plastic packaging ^te, 2011). The third scenario is the same as for
available data (Lho
waste treatment in Europe that is not recycled, it has been EPS: 55% recycling and 45% incineration by 2025, based on the
assumed that 50% goes to landfilling and 50% to incineration European Commission's (2015b) proposal.
with energy recovery (Eurostat, 2016);
 the strong bond between cellulose fibre board and the poly- Estimating the number of different types of container used in
ethylene coating make the paper lids in the aluminium the EU is a challenge as no specific data are available. Nevertheless,
container difficult to recycle (Mitchell et al., 2014). According to based on data from previous studies (Lago et al., 2011; Riera, 2015),
Eurostat (2016), 54% of the paper packaging that is not recycled estimates in this study1 suggest that the total number of takeaway
is incinerated and 46% landfilled; these values have been food servings in the top five EU consumer countries (UK, Germany,
assumed here for the paper lid; France, Italy and Spain) will reach 1916 million by 2025. For the rest
 for the cardboard packaging of the containers, end-of-life
packaging data for the EU28 have been assumed: 85% recy-
cling, 8% incineration with energy recovery and 7% landfilling 1
The total number of servings reported in the quoted studies is 1638 million for
(Eurostat, 2016); and the year 2014. They forecast an increase to 1760 million by 2019, a growth of 1.5%
 for the silicone (in Tupperware) and polyethylene (in pack- per annum. The same annual increase rate has been applied in the current study for
aging), 100% landfilling has been assumed. the period 2019e2025, to obtain the total value of 1916 million in 2025.
422 A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427

Table 2
End-of-life scenarios for the takeaway containers in the European Union (EU28)a.

Current situation Best case Worst case EU 2025 proposal

Aluminium R: 54%, L: 46%b R: 89%, L: 11%b R: 22%, L: 78%b R: 75%, L: 15%d


PP R: 11%, I: 44%, L: 45%c R: 30%, I: 69%, L: 1%c R: 2%, I: 8%, L: 90%c R: 55%, I: 45%d
EPS I: 50%, L: 50%b I: 100%b L: 100%b R: 55%, I: 45%d
a
R: recycling, I: incineration with energy recovery, L: landfilling.
b
Eurostat (2016).
c
Lho^ te (2011).
d
European Commission (2015b).

of the EU countries, no data are available and hence some as- ozone depletion potential (ODP), photochemical oxidants creation
sumptions have to be made to obtain the total number of con- potential (POCP), terrestrial ecotoxicity potential (TETP) and the
tainers in use. Taking a conservative approach, it has been supposed primary energy demand (PED).
that the remaining EU countries consume in total a third of the
takeaway meals consumed in the top five countries, i.e. a total of
3. Results and discussion
639 million. Therefore, the total for the whole EU in 2025 has been
estimated at 2556 million takeaway food servings. Assuming an
3.1. Non-reusable takeaway containers
equal share of the three types of container, the total number of each
type used annually in the EU is estimated at around 850 million.
As can be seen in Fig. 3, the aluminium container has the highest
However, this would imply that no other types of container are
impacts for five categories: ADPe, HTP, MAETP, ODP and TETP. These
used. Therefore, the analysis considers an exploratory range of
are, respectively, between 2e23 and 4e28 times higher than for the
500e850 million units/yr, with an average of 675 million for each of
PP and EPS. The PP container is the most impactful for the other
the three types of container. It should be noted that these figures
seven impacts, largely due to the production of PP and its eventual
are estimates rather than necessarily the actual figures. Neverthe-
landfilling. These impacts are 2e3 times greater than for the
less, they represent best approximations available currently and are
aluminium and 3e6 higher than for the EPS containers.
aimed at understanding the magnitude of the impacts related to
The results in Fig. 3 also show that the EPS is the best option
the use of takeaway containers in the EU.
across the impact categories. Against the aluminium container, its
impacts are 7%e28 times lower and against the PP, 25% to six times
2.2.4. Transport better. This is due to a lower amount of EPS needed to manufacture
The following distances and transport means have been the container compared to PP (four times) and less energy required
considered: for the production of EPS in comparison with aluminium. These
findings go against the ongoing debate on the negative impacts of
 For the raw materials and packaging, distances in Ecoinvent EPS containers and their ban in India, China, Taiwan and in several
have been assumed. If not specified in the database, a distance of cities in the USA and UK, based on concerns about food health and
150 km to the factory in 16e32 t Euro 3 trucks has been safety, inefficient recycling, low degradability and contribution to
considered. marine pollution (Barnes et al., 2011). However, these bans remain
 The aluminium and PP containers are shipped from China to controversial and some of them have been revoked through law
Europe by a transoceanic tanker, assuming a distance of suits by packaging manufacturers (Bapasola, 2015; Mueller, 2015).
19,500 km from Shanghai to Rotterdam (World Ship Council, Regarding health and safety, Cohen et al. (2002) found that the risk
2016). Afterwards, the containers are transported by 16e32 t of migration of styrene from EPS to packaged food are quite low and
Euro 6 truck to a distribution centre located in Munich, the of no concern. These findings are in agreement with the European
central geographical location of Europe (829 km). Common Food Safety Authority (EFSA) which stated that EPS is safe for use
distances of 150 km have been assumed for transport of the for contact with food (European Commission, 2011). In relation to
containers from the production site to the port in Shanghai recyclability, manufacturers argue that EPS is technically recy-
(truck 16e32 t Euro 3) and from a distribution centre to retailer clable; however, in practice, due to low cost-effectiveness, the
(16e32 t Euro 6 truck). recycling rate is negligible (Razza et al., 2015). Because of its
 An average transport distance of 500 km has been assumed for lightness e EPS is 95% air by weight e vast amounts need to be
the EPS containers in Europe, from the factory to the distribution collected and compressed, or “densified,” before being shipped to a
centre in Munich (16e32 t Euro 6 truck). recycler (MacKerron, 2015). Therefore, large investments in com-
 For waste treatment, a distance of 50 km in a 16e32 t Euro 6 pactors and logistical systems are necessary to achieve significant
truck has been assumed for all the containers. percentages of recycling. Nevertheless, the potential benefits of
(theoretically) increasing the recycling rate of EPS at the EU level
2.3. Impact assessment are considered in section 0 to gauge the magnitude of environ-
mental savings that could be achieved. Finally, the low degrad-
GaBi v6.5 software (Thinkstep, 2016) has been used to model the ability and contribution to marine debris are clearly related. The
system. The environmental impacts have been calculated following EPS containers, due to their lightness, can easily be blown away,
the CML 2001 (January 2016 version) mid-point impact assessment contributing to urban and riverine litter (Rubio, 2014). Owing to
method (Guine e et al., 2001). The following impacts are considered: their low degradability, EPS waste remains in the environment and
abiotic depletion potential of elements (ADPe.), abiotic depletion can end up in marine environments. For example, Fok and Cheung
potential of fossil resources (ADPf.), acidification potential (AP), (2015) found that 92% of the microplastics collected on 25 beaches
eutrophication potential (EP), global warming potential (GWP), along the Hong Kong coastline was EPS. Aquatic organisms can
human toxicity potential (HTP), marine aquatic ecotoxicity poten- ingest these microplastics or become entangled in larger parts of
tial (MAETP), freshwater aquatic ecotoxicity potential (FAETP), plastic (Stefatos et al., 1999; Sutherland et al., 2010) with
A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427 423

Fig. 3. Life cycle environmental impacts of single-use containers. [All impacts expressed per 670 ml container. The values on top of each bar represent the total impact after the
recycling credits and for relevant impacts should be multiplied by the factor shown in brackets to obtain the original values. EPS: extruded polystyrene. PP: polypropylene. ADPe:
abiotic depletion potential of elements, ADPf: abiotic depletion potential of fossil resources, AP: acidification potential, EP: eutrophication potential, GWP: global warming potential,
HTP: human toxicity potential, MAETP: marine aquatic ecotoxicity potential, FAETP: freshwater aquatic ecotoxicity potential, ODP: ozone layer depletion potential, POCP:
photochemical ozone creation potential, TETP: terrestrial ecotoxicity potential, PED: primary energy demand and DCB: dichlorobenzene.].

detrimental consequences for marine life. Thus, despite its lower carbon in the leachates associated with EPS landfilling is what leads
life cycle environmental impacts relative to the other containers, to the high EP and the emissions of CO2 while heavy metals due to
EPS cannot be considered a sustainable packaging option unless its incineration contribute to GWP, FAETP, HTP and MAETP.
end-of-life management can be improved significantly. The raw materials stage is also the main contributor (>43%) to
ADPf, PED, POCP and GWP of PP containers, mainly due to the
consumption of fuel oil and the emissions of VOCs and CO2 in the PP
3.1.1. Contribution analysis and improvement opportunities production process. The manufacture of the container is the main
As indicated in Fig. 3, the extraction and refining of aluminium contributor (>42%) to ADPe, AP and TETP. All these impacts are
are the main contributors (>48%) to 11 of the 12 impacts of the mainly related to the generation of the electricity consumed in the
aluminium container. These are mainly associated with the gen- extrusion and thermoforming processes. Transport only contrib-
eration of electricity used in the refining process (ADPe, ADPf, AP, utes significantly (>35%) to ADPe. due to the metals used in the
EP, GWP, PED) and the emissions of carbon monoxide (POCP), battery of the trucks and ODP, related to halogenated gases used as
hydrogen fluoride (MAETP), polycyclic aromatic hydrocarbons fire suppressants in pipelines. In the end-of-life stage, only land-
(HTP) and heavy metals (FETP) from the aluminium extraction and filling contributes significantly to EP (69%), FAETP (56%), HTP (39%)
refining process. The production process of the PE-coated paper lid and MAETP (37%). However, this stage also has a positive effect on
is the main contributor to ODP (86%) due to the emissions of halon seven categories (5%e21%) due to the systems credits for PP
1301 in the coating process. The stamping of the aluminium foil to incineration and recycling.
obtain the desired shape contributes 24% to both aquatic toxicities, In summary, the findings suggest that the raw materials,
mainly due to the electricity consumed in the process. Finally, end- container production and end-of-life contribute significantly to
of-life treatment has a positive impact on all impact categories most impacts. To address these, different improvement opportu-
(between 2 and 23% reduction), mainly due to the system credits nities could implemented. In the raw materials stage, these include
associated with aluminium recycling. For further details on the life product light-weighting and increasing the recycled content in the
cycle stages that contribute most to the impacts of the aluminium containers. However, manufacturers claim that the container
container, see Table S1 the Supporting Information (SI). thickness has already been reduced significantly and further light-
The production of EPS in the raw materials stage contributes weighting can compromise the function of the containers (EAA,
more than half of ADPf, AP, GWP, POCP and PED of the EPS 2016; Ingrao et al., 2015; Tupperware, 2016). Regarding the
container. It also has a significant contribution (>20%) to HTP, increased recycled content, recycled plastics are not commonly
MAETP, ODP and TETP. The consumption of fuel oil and electricity used in food packaging because of concerns about food safety and
and the emissions of CO2, SO2 and non-methane volatile organic hygiene standards (Mudgal et al., 2011). This restriction does not
compounds (VOCs) are the main cause of these impacts. The apply to aluminium, but there have not been significant changes in
extrusion and thermoforming processes in the production stage are the amount of recycled aluminium (30%) in recent years (EAA,
the main contributors to six of the impact categories (>33%), mainly 2013; EAA, 2008).
due to electricity consumption. Transport has no significant influ- There are fewer improvement opportunities in the manufacture
ence in any category (<9%). Finally, the end-of-life stage contributes of containers. Production processes, such as plastics extrusion and
significantly to EP (62%) and FAETP (46%) and, to a lesser extent, to thermoforming or aluminium sheet rolling and stamping, are
HTP (28%), GWP (20%) and MAETP (16%). The increase of organic
424 A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427

mature and no significant advancement is expected in the future. widespread use of reusable containers. One of these is the incon-
However, the end-of-life stage is where the most feasible oppor- venience requiring consumers to carry the container to the food
tunities for improvements are expected in the short to medium outlet and to clean it afterwards. Only committed or incentivised
terms for the three types of containers. These are considered for (e.g. food discounts) consumers could achieve the number of reuses
each container at EU level in section 0. Prior to that, the impacts of necessary to balance out the impacts of single-use containers,
the three non-reusable containers are compared to the reusable PP especially those made of EPS. Another problem is the portion sizes
containers (takeaway and Tupperware). e this can be dealt with more easily if the reused containers are
provided by the food outlet but less so if consumers bring their own
reusable containers which would invariably be of different sizes.
3.2. Reusable vs non-reusable containers Another issue is related to possible legal challenges, for example,
due to food poisoning. This could be either due to food contami-
In order to compare reusable and non-reusable containers, the nation at the outlet or due to the inadequate cleaning of the con-
concept of “transition point” has been applied. The transition point tainers by the consumer, but it would be difficult to prove who is
is defined as the point where a system starts to perform better than responsible. Thus, these and other related barriers should be
the system with which it is being compared (Ligthart and Ansems, considered as part of future research to identify the best way
2007). This can be determined by varying certain variables of in- forward.
terest. In this study, the variable of interest is the number of times In addition, other improvement opportunities should also be
both types of PP container (takeaway and Tupperware) have to be considered. One of these includes better end-of-life management of
reused to balance out the impacts of the single-use aluminium and single-use waste containers. This is discussed further in the next
EPS containers. section, with the focus on the EU level to determine the magnitude
Table 3 shows the transition points. It can be seen that the of potential environmental improvements.
Tupperware container has to be reused eight times to equal the
impacts of the aluminium containers for half of the impacts cate-
gories considered, 11 times for GWP and up to 16 to balance out all 3.3. End-of-life scenarios at the EU level
the impacts. The number of reuses needed increases even more
with respect to the EPS containers. The Tupperware should be As indicated in Fig. 4 and Table S5 in the SI, implementing the EU
reused 18 times to equal the GWP of EPS and 24 times to balance proposal for recycling 75% of aluminium and 55% of plastic pack-
out half of the impacts categories. As Tupperware containers can be aging waste by 2025 (Table 2) would reduce all the impacts by 2%
reused on average 43 times before they need to be discarded (ODP) to 60% (EP and FAETP). For GWP, the reduction would amount
(Gallego-Schmid et al., 2018; Harnoto, 2013), they could balance out to 33%, saving 61,700 t CO2 eq./yr if a total of 2025 million/yr of
all the impacts of the aluminium container and most of the EPS containers are assumed with an equal share of each type (45,700
container. The only exception for the latter are ADPe, for which 208 and 77,300 t CO2 eq. for 1500 and 2550 million/yr, respectively).
reuses would be required and TETP, which can never be better than These savings are equivalent to the greenhouse gas emissions
for the EPS container. The reason for these two exceptions is the generated annually by around 55,000 (40,500-69,000) light-duty
high impacts from the use of electricity to heat the water for vehicles (Winkler et al., 2014).
washing the reusable containers. The implementation of the “Best” scenario (highest recycling
The results are more favourable for the reused PP takeaway rates practiced currently in some EU countries; see Table 2) would
containers which match all the impacts of the aluminium option improve seven impact categories on the EU 2025 proposal, but the
only after four reuses, with GWP requiring only three reuses. They differences between the two scenarios are relatively small (3e18
also balance out most of the impacts of the EPS containers after percentage points). However the EU 2025 scenario would lead to
nine reuses; for GWP, this reduces to four times. This level of reuse higher reductions in APDf, AP, GWP, POCP and PED. Finally, the
is more realistic for consumers than the number of uses required implementation of the worst scenario (lowest recycling in some EU
for the Tupperware. Furthermore, this type of plastic container is countries) would increase all impacts by 2% (GWP) to 62% (EP)
already in use by food outlets, making it easier for businesses to compared to the current situation.
encourage their reuse, while reducing the total cost of containers Fig. 4 also shows the contribution of different waste manage-
they need to purchase, improving their environmental credentials ment options to the total impacts for each scenario. It can be seen
at no extra cost and securing customer loyalty. that EPS containers generally contribute the least to the total im-
However, there are various practical and legal obstacles to a pacts. Aluminium containers are the main cause of ADPe, HTP, ODP,

Table 3
Number of uses of polypropylene (PP) reusable containers needed to equal the impacts of single-use containers (aluminium and extruded polystyrene (EPS)).

Impacta PP food saver (Tupperware) vs aluminium PP food saver (Tupperware) vs EPS Reusable takeaway PP vs aluminium Reusable takeaway PP vs EPS

ADPe. 3 208 1 32
ADPf. 16 18 4 4
AP 8 29 2 7
EP 14 18 3 4
FAETP 12 39 3 9
GWP 11 18 3 4
HTP 2 37 1 9
MAETP 4 24 1 6
ODP 1 27 1 3
POCP 9 16 2 4
TETP 8 eb 2 eb
PED 10 19 3 5
a
For the impacts nomenclature, see Fig. 3.
b
EPS container performs always better than the reusable containers for TETP.
A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427 425

Fig. 4. Annual environmental impacts of aluminium (Al), extruded polystyrene (EPS) and polypropylene (PP) containers in the EU28 considering different end-of-life scenarios.
[Basis: 675 million/yr of each type of container (total of 2025 million), with the error bars showing the range from 500 to 850 million/yr (total 1500e2550 million). R: recycling; L:
landfilling; I: Incineration with energy recovery. For the description of the scenarios, see Table 2 and for the impacts nomenclature, see Fig. 3.].

MAETP and TETP for all scenarios while PP containers contribute virgin material. GWP would be reduced by 9600 t CO2 eq./yr.
most to ADPf, AP, GWP, POCP and PED; for EP and FAETP, the highest However, as discussed in section 3.1, achieving these recycling rates
contributor depends on the scenario. will require large investment in compactors and logistical systems
With reference to the specific types of container, increasing the as well as consumer engagement.
recycling rate of aluminium would result in significant environ- Finally, if in the worst case 90% of PP containers are landfilled, as
mental improvements (Table S6 in the SI). For every 10% increase in opposed to 45% at present, all the impacts but GWP are increased
the amount of aluminium recycled, the impacts would be reduced (Table S8), with EP, FAETP and ODP being most affected (>31%).
by 6%e19%, with the highest reductions found for TETP (14%) and GWP is reduced by 9% (8800 t CO2 eq.) because of the reduced
HTP (19%). These savings are due to the credits for avoiding the use emissions of CO2 from incineration. The best case and the EU 2025
of virgin aluminium and the reduced amount of waste landfilled. scenarios each lead to significant reductions (>52%) in EP, FAETP,
For the GWP, increasing the current EU aluminium recycling rate HTP, MAETP, related to the avoidance of landfilling and leachates of
from 54% to 75%, as per the EU 2025 proposal, would save 11,600 t heavy metals and organic carbon. The best case, with a higher
CO2 eq. per 675 million of aluminium containers annually, repre- percentage of incineration (69%), has the lowest ADPe., ODP and
senting a reduction of 23% on the current situation. Increasing the TETP, mainly due to the credits for energy recovery. However, the
recycling to 89%, the best current recycling rate in the EU, would reductions in GWP are minimal (<1%) because of the CO2 emissions
reduce the impact by 38%, saving 19,400 t CO2 eq./yr. On the other from incineration of plastics. The EU 2025 scenario, with a signifi-
hand, if aluminium is recycled in all EU countries at the same rate as cant percentage of recycling (55%), would lead to the highest re-
in the country with the lowest recycling rate (22%), the impacts ductions (>38%) in ADPf., EP, GWP, POCP and PED, mainly due to the
would increase by 19%e60% compared to the current situation, credits for the avoidance of virgin PP. For the GWP, the total
with an increase in GWP of 35%. reduction of 40,500 t CO2 eq. per 675 million containers is equiv-
In the case of EPS, landfilling all containers in the worst case or alent to avoiding the annual emissions of 36,500 light-duty
incinerating them in the best scenario shows no significant effect vehicles.
on the impacts compared to the current situation (Table S7 in the
SI). The only exceptions are EP, ODP and GWP. For the EP, 100% 4. Conclusions
incineration reduces the impact by 69%, mainly because of the
avoidance of the organic carbon in landfill leachates. Incineration This study has presented for the first time life cycle environ-
also reduces ODP (by 15%) due to the credits for the avoided natural mental impacts of most-commonly used takeaway containers:
gas displaced by the heat recovered from the incinerator. This is in aluminium, EPS and PP. The results suggest that the use of
turn associated with the reduced use of halogens as fire suppres- aluminium containers leads to the highest depletion of elements
sants in gas pipelines. For the rest of the impacts, 100% incineration and ozone layer as well as human, marine and terrestrial toxicities.
improves the current situation by 3%e7%, except for FAETP, HTP and The PP container is the worst alternative for the other seven impact
TETP which are not affected by the changes in the rate of inciner- categories considered.
ation (or landfilling). Finally, in the 100% landfilling scenario, GWP The best option among the three is the EPS container with the
is reduced by 18%, principally due to the reduction in CO2 emissions lowest impacts across the 12 categories. Against the aluminium
from EPS incineration. container, its impacts are 7%e28 times lower and against the PP,
Implementing the EU 2025 proposal of 55% EPS recycling and 25% to six times better. The EPS is also the best option when
45% incineration would improve the impacts by more than 18% for compared to reusable takeaway PP containers, unless these are
ten of the categories considered. The highest reductions are found reused 3e39 times, depending on the impact. The number of uses
for ADPf., GWP, POCP and PED, the categories most influenced by for the reusable PP Tupperware food savers is even higher, ranging
the production of EPS, benefiting from the credits for the avoided from 16 to 208 times, with terrestrial ecotoxicity being always
426 A. Gallego-Schmid et al. / Journal of Cleaner Production 211 (2019) 417e427

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