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Abstract
An air drawing model of polyethylene terephthalate (PET) polymer and one of the air jet
flow field in the spunbonding process are established. The air jet flow field model is solved
and simulated by means of the finite difference method. Numerical simulation computation
results of the distributions of air velocity match quite well with the experimental data. The
air drawing model of the polymer is solved with the help of distributions of air velocity
measured by Particle Image Velocimetry. The model’s predictions of filament fiber diam-
eters, crystallinities and birefringences coincide well with the experimental data. There-
fore it can be concluded that a higher initial air temperature can yield finer filament fiber
diameter, and a higher initial air velocity can produce a finer fiber diameter as well. The
experimental results show that the agreement between the results and experimental data is
much better, which verifies the reliability of these models. Also they reveal great prospects
for this work in the field of the computer assisted design (CAD) of the spunbonding process.
Key words: spunbonding, polyethylene terephthalate, air drawing model, air jet flow field,
polymer, fiber diameter, crystallinity, birefringence, drawing, numerical computation.
Bo Z. Experimental and Numerical Simulation Study of an Air drawing Model of Polyethylene Terephthalate (PET) Polymer and Model of Air Jet Flow Field 89
in the Spunbonding Nonwoven Process. FIBRES & TEXTILES in Eastern Europe 2014; 22, 1(103): 89-96.
Air drawing theoretical model 0.37 and 0.61, respectively, as far as the C pf= (0.3 + 6 ×10−4 T ) × 4.182 ×107 (10)
of spunbonding polyethylene spunbonding process is concerned).
terephthalate polymer Constitutive equation
The empirical relationship expression of
The air drawing model of spunbonding Reynolds number is as follows: As is commonly known, the polymer
polymer consists of continuity, momen- melt used in the spunbonding process
ρ D (Va − V )
tum, energy, and constitutive equations Red = (5) is a kind of non-Newtonian fluid. How-
[7 - 16]. The surrounding air conditions υa ever, the simplest constitutive equation
(velocity and temperature) are consid- i.e., the Newtonian fluid relationship is
where: r - density of the air, (Va - V ) -
ered as given functions of axial position used in this work because research has
relative velocity between the moving
[17 - 19] and obtained by numerical sim- shown that the temperature dependence
filament fibre and air, and ua - kinematic
ulation. Almost all experimental data are on viscosity is the most dominant effect,
viscosity coefficient of the air.
well fitted by drag force correlation of the while the type of constitutive equation is
following forms: secondary [25, 26]. Therefore for com-
The force on the filament fibre parallel to
the air stream can then be found from the putational simplicity the Newtonian fluid
Continuity equation following relation: constitutive equation was introduced in
π (1) our model:
Q= D 2V ρf 1
4 Fdrag
= ρ (Va -V) 2C f π DL1 (6)
2 π dV
where: Q - polymer mass flow rate, D - Frheo = D 2η (11)
where: Fdrag - air drag force on the fila- 4 dx
filament fibre diameter, V - filament fibre ment fibre, r - air density, D - filament
mean velocity in the spinning direction, Frheo
fibre diameter, L1 - filament fibre length. s= (12)
and rf - specific density of the polymer, (π D 2 / 4 )
(this quantity depends on temperature). Energy equation
= η 48.71exp[2650 /(T + 273)]exp[4( X / X ∞ ) 2
π Dh(T − Ta ) ∆H η (13)
As the polymer density varies with poly- dT f dX 48.71exp[2650 /(T + 273)]exp[4( X / X ) 2 ]
= − = + (7) ∞
mer temperature, the following correla- dx QC pf C pf dx
tion [20 - 22] is also introduced: where: η - shear viscosity of the air.
where: T - filament fibre temperature,
ρ=
f 1.356 − (5 ×10−4 T ) (2) Ta - air temperature, h - heat transfer co- Crystallisation kinetics equation:
efficient, which will vary with the axial Variation in the degree of crystallinity
where: T - polymer temperature. position, Cpf - specific heat capacity of along the spinline is given by the follow-
the polymer (it varies with temperature ing equation:
Momentum equation at constant pressure), DHf - heat of fu-
dFrheo π dV sionπ of2 the polymer [17], and Red - de- d X n1k X X
= j ρ C f (Va − V ) D + Q
2
− ρgree D g ( )= (1 − ) ln 1 1 −
dx 2 dx
f
4 of crystallinity. The first right - hand dx X ∞ V X ∞ X ∞
side term of Equation 7 describes the
π dV π n1 −1
j ρ C f (Va − V ) D + Q
2
o
− ρ f D2 g (3) decrease in temperature due to heat loss
2 dx 4 d X n1k X X n1 (14)
by the fibre to the cooling medium and ( )= (1 − ) ln 1 1 −
where: Frheo - rheological force, x - the second term represents the opposite dx X ∞ V X ∞ X ∞
spinning axial direction position, r - air effect that crystallisation has on the tem- where: X - maximum crystallinity [17],
∞
density, j - sign carrier of air drag force, perature due to the release of the latent X/X - relative crystallinity, (ratio of the
∞
when j is -1 for Va > V, and +1 for Va < V, heat of fusion. The value for the heat
absolute crystallinity over the ultimate
ρf - polymer density, V - filament fibre transfer coefficient can be calculated
crystallinity of the material), n1 - the
velocity, Va - x-component of air veloc- from the following relation between Nu
avrami index [17], - k -the crystallisation
ity, drag results from friction between and Red.
rate [17].
the filament fibre and air when the two Nu== γ (Red ) m
Nu (8)
are moving with different velocities be-
Nu.K a Birefringence equation
cause the high air suction in the cham- h= (9)
ber results in high axial air velocities, D ∆nam = Cops (15)
therefore the relative velocity is used in Where the Nusselt number Nu [24], Ka X X
the term instead of the actual velocity of ∆n = (1 − )∆nam + f c ∆ 0c (16)
the air heat conduction coefficient, and γ X∞ X∞
the filament fibre, g is the gravitational and m are empirical constants of the cor-
acceleration, and Cf - air drawing coeffi- ∆nam / ∆ 0a
fa =
relation. (17)
cient of filament fibre as a function of the
Reynolds number, Cf - in Equation 3 was where: Cop - stress optical coefficient
The values of γ and m are 0.42 and 0.334,
given by Matsui [23, 24] with the follow- [17, 27, 28], ∆ 0c - intrinsic amorphous
respectively.
ing correlation: value [17, 27, 28], ∆ 0c - crystalline bire-
Like the polymer density, the specific fringence value [17, 27, 28].
Cf = b . (Red)-n (4)
heat capacity at constant pressure of the
where: Red - Reynolds number based on polymer also changes with the polymer Boundary conditions
the filament fibre diameter, β, n - fitted temperature. The correlation [20 - 22] is V(0) = V0, F(0) = F0, D(0) = D0,
(18)
constants (values of β and n should be given as follows: X(0) = 0, T(0) = T0, Frheo(L) = 0
90 FIBRES & TEXTILES in Eastern Europe 2014, Vol. 22, No. 1(103)
where: L - chamber length, F0 - initial assembly spinning occurs in a very short the air velocity, x - axial position, and y -
rheological force of the polymer melt, time, a two-dimensional, steady, viscous transversal position.
V0 - initial velocity of the polymer melt, turbulent flow of a perfect gas in the
D0 - initial diameter of the polymer melt, absence of body forces is considered. Momentum equation in x direction
T0 - initial temperature of the polymer Equation 20, the governing equation, is
melt. expressed as follows: ∂ ( ρ uu ) ∂ ( ρ uv) ∂ ∂u ∂
+ = 2 ( µ + µt ) + ( µ
∂x ∂y ∂x ∂x ∂y
div( ρ uφ − Γφ gradφ ) = Sφ (20)
The “freezing-point” is defined as the ∂ ( ρ uu ) ∂ ( ρ uv) ∂ ∂u ∂ ∂u ∂v
boundary condition. The method used where + = 2 ( µ + µt ) + ( µ(23)
+ µt ) + −
∂x ∂y ∂x ∂x ∂y ∂y ∂x
for determining the initial rheological 1 0 0
∂ ( ρuu ) ∂ ( ρ uv) ∂ ∂u ∂ ∂u ∂v ∂P
force F0 is the searching “freezing-point” φ = u Γφ = ∂x
µ + S∂φ y= = 2 ( µ + µt ) + ( µ + µt ) + −
−∇p∂+x S ∂x ∂y
+ Su
method, which requires checking wheth- ∂y ∂x ∂x
T k / c ST
er the fibre diameters before and beyond k2
some “point” along the filament are equal where: r - air density, u - velocity vector, with, µt = ρ Cu
f - the conserved property, Γf - diffusion ε
to each other when F0 is considered to be
the sum of the cumulative gravitational coefficient, Sf - source term for the vari- where: P - air pressure, m - kinematic vis-
and air drawing force acting upon the fro- able f, T - temperature, m - dynamic vis- cosity of the air, m - turbulent viscosity of
t
zen part of the filament fibre. If the fibre cosity, k - heat conductivity, c - specific the air, C - constant of k-ε model, ε - tur-
u
diameters are found to be the same, the heat of the fluid, p - pressure, S - source bulent dissipation rate of air, k - dissipa-
“point” is the so-called “freezing-point” term, and ST - represents the viscosity tion rate of turbulent kinetic energy of air.
and is used in this iteration as the appro- disssipation rate.
priate initial rheological force. Momentum equation in y direction
Considering the compressibility of the
By means of numerical simulations of the air, the ideal gas equation is used to close ∂ ( ρ vu ) ∂ ( ρ vv) ∂ ∂u ∂v
the equation system: + = ( µ + µt ) + +
air jet flow field, we can determine the ∂x ∂y ∂x ∂y ∂x
distributions of the x-component of air p = raRT (21)
velocity Va and air temperature Ta along ∂ ( ρ vu ) ∂ ( ρ vv) ∂ ∂u ∂v ∂ ∂v ∂P
where: R - gas constant. + = ( µ + µt ) + + 2 (24)
( µ + µt ) −
the axial position x. It allows to solve the ∂x ∂y ∂x ∂y ∂x ∂y ∂y ∂y
air drawing model of the polymer using Theoretical∂ ( ρmodel
vu ) ∂of( ρthe
vv) air ∂jet flow ∂u ∂v ∂ ∂v ∂P
the fourth-order Runge-Kutta method. +
field in the spunbonding =process ( µ + µt ) + + 2 ( µ + µt ) − + Sv
∂x ∂y ∂x ∂y ∂x ∂y ∂y ∂y
The air jet flow field of the spunbonding Here, m = uar, mt = utr
Dynamics balance equation
process is considered as a steady and vis- where: P - pressure of the air, r density
F = Fasp + Fgrav - Fdrag - Finter (19) cous flow. The flow field is assumed to of the air, ua kinematic viscosity coeffi-
where: F - force on the filament fibre, be two-dimensional. A k-ε model is the cient of the air, ut turbulent viscosity co-
Fasp - tension exerted by the aerodynam- most widely used turbulence model in efficient of the air, m kinematic viscosity
ic drawing device, Fgrav - gravitational engineering computations and it yields of the air, and mt the turbulent viscosity
force, Fdrag - air drag on the filament fi- very accurate results in the case of high of the air.
bre, Finter - inertial force. Reynolds numbers; it is defined as the
preferred turbulence model. The air flow Energy equation
field of model consists of the following
∂ ( ρ uT ) ∂ ( ρ vT ) ∂ µ ∂T ∂
Numerical simulation equations: continuity, momentum, en- + = (25) µ+ t +
of the mathematical model ergy, turbulent kinetic energy and tur- ∂ x ∂y ∂ x s t ∂x ∂y
of the air jet flow field bulent dissipation rate [29 ∂ ( ρ- uT
31].
) In∂ (this
ρ vT ) ∂ µt ∂T ∂ µt ∂T
in the spunbonding process paper, we adopted the k-ε standard+model =
∂x details are
∂y
µ + + µ +
∂x s t ∂x ∂y s t ∂y
for computation. Below some
The fibre diameter of spunbonding non- given.
woven is intensely affected by the air jet where s - Prandtl number of turbulence.
t
flow field of the spunbonding drafting as- Values of the constants of the standard Turbulent kinetic energy equation
sembly (attenuator), shown in Figure 1. k-ε model are C1e = 1.44, C2e = 1.92 and
In this paper, we established a model of Cu = 0.09 [32]. The turbulent Prandtl ∂ ( ρ ku ) ∂ ( ρ kv) ∂ µ ∂k ∂
the air jet flow field to simulate the flow numbers are as follows: sk = 1.0, se = 1.3, + = µ + t +
field and we solved it numerically via the ∂x ∂y ∂x s k ∂x ∂y
Prt = 1.0 and st = 0.9 [32], where σt, σk
finite difference method. Distributions of and σε are Prandtl numbers of turbulence,
∂ ( ρ ku ) ∂ ( ρ kv) ∂ µ ∂k ∂ µ ∂k
the centreline x-component of air veloc- turbulent kinetic energy and turbulent + = µ + t + µ + t + Gk
ity along the x-axis are demonstrated. ∂x ∂y ∂x s k ∂x ∂y s k ∂y
dissipation rate, respectively.
∂ ( ρ ku ) ∂ ( ρ kv) ∂ µ ∂k ∂ µ ∂k
Governing equations + = µ + t + µ + t + Gk − ρε
Continuity equation
∂x ∂y ∂x s k ∂x ∂y s k ∂y
By ignoring the influence of polymer fi-
∂ ( ρ u ) ∂ ( ρ v)
bres or strands, air jet flow in the drafting + 0
= (22) with,
assembly (attenuator) will be a classical ∂x ∂y
µ ∂v
2 2 2
∂u ∂v ∂u
fluid flow problem. Since the spunbond- where: r - air density, u - x-component =
Gk t
2 + 2 + + (26)
ρ ∂x ∂y ∂y ∂x
ing air drawing process in the drafting of the air velocity, v - y-component of
FIBRES & TEXTILES in Eastern Europe 2014, Vol. 22, No. 1(103) 91
b) the staggered grid is presented to
avoid tooth-like distributions of ve-
Polymer locity and pressure;
h1 h2 f c) the preferred difference scheme for
melt
Air space independent variables is the sec-
y
ond-order upwind difference scheme;
a d e
d) the TDMA method is used to solve the
b c
difference equations.
x
92 FIBRES & TEXTILES in Eastern Europe 2014, Vol. 22, No. 1(103)
Numerical simulation of the air Figure 3. Distribu-
tions of centreline 32
drawing model of polymer in x-component of the
the spunbonding process air velocity along 30
Experimental
the x-axis. 28 Numerical
Experiments were performed on the
spunbonding process at our university. 26
The melt flow index (MFI) experiments 4 85.0 25.8 24.40 5.42
15.6
5 75.0 22.08 21.11 4.39
of polyethylene terephthalate (PET) were
FIBRES & TEXTILES in Eastern Europe 2014, Vol. 22, No. 1(103) 93
30 30
Initial air temperature, °C Initial air speed, m/s
from top to botton from top to botton
28 28
Fibre diameter, mm
Fibre diameter, mm
12.8 75
15.6 85
26 26
18.4 95
24 24
22 22
20 20
18 18
10 20 30 40 50 60 70 10 20 30 40 50 60 70
a) b)
Distance from spinneret, cm Distance from spinneret, cm
Figure 4. Showing relationship between fibre diameter and distance from spinneret with initial air: a) temperature, °C and b) speed, m/s.
perature, the finer the fibre diameter ob- with an increase in the polymer through- distance from the spinneret, which is in
tained, which is primarily due to the fact put rate. Higher polymer throughput rates agreement with the diameter profiles.
that the initial air temperature increased, also lead to higher fibre diameters, which
and both the air drawing force and degree is primarily due to each polymer through-
of drawing increased, which yield a finer put rate having its own air speed, with the n Conclusion
fibre diameter. Secondly when the initial axial air flow controlling the drag over An air drawing model of polyethylene
air temperature increased, the filament fi- the entire spinline, which also affects heat terephthalate (PET) polymer and a model
bre cooled more slowly along the spinline, loss from the fibre. of the air jet flow field in the spunbonding
with the drawing (tensile) time of poly-
process were developed. We numerically
mer being extended (lengthened), which Figure 5.b shows the polymer melt
resulted in a finer fibre diameter. Thirdly simulated the air jet flow field model by
temperature profiles for different poly- means of the finite difference method.
when the initial air temperature increased,
the viscosity and stress decreased, which mer throughput rates. This figure shows Computation results of the distributions
produced a finer fibre diameter. that the cooling rate is lower for higher of x-components of the air velocity along
polymer throughput rates, which is also the spinline during the spunbonding pro-
Relationship between the initial air observed in conventional melt spinning. cess are in accordance with experimental
velocity and fibre diameter This is attributed to the fact that the in- data as well. The newly developed formu-
crease in stress is at least partly due to las are introduced into the spunbonding
Figure 4.b gives the effect of the initial
the variations in air flow conditions with air drawing model to predict the fibre di-
air velocity on fibre diameter, which
a changing polymer throughput rate. ameter. The distributions of air speed are
changes with variations in the distance
also introduced into the air drawing mod-
from the spinneret. Initial air veloci-
Figure 5.c shows the relationship be- el of polyethylene terephthalate (PET)
ties of 75.0 m/s, 85.0 m/s, and 95.0 m/s
tween fibre crystallinity and the distance polymer. We can predict the drawing ef-
were considered. As Figure 4.b shows,
from the spinneret with the polymer fects by means of the air drawing model,
the higher the initial air velocities, the
throughput. and model predictions of fibre diameters,
finer the fibre diameters obtained, which
crystallinities and birefringences are in
is mainly attributed to the fact that with
Figure 5.d shows the relationship be- conformity with experiment data. It was
an increase in the initial air velocity, air
found that a higher initial air speed and a
drawing force and degree of drawing, a tween fibre birefringence and the dis-
higher initial air temperature can all yield
finer fibre diameter was produced. tance from the spinneret with the poly-
finer fibres. The results predicted coincide
mer throughput rate. Predictions of fibre
well with the actual data measured, which
Effects of spunbonding nonwoven birefringence are shown in Figure 5.d,
reveal that these models are accurate. It
processing parameters on fibre where it is clear that the birefringence is also shows that this area of research has
performance decreasing with an increasing polymer great potential in the field of computer as-
The subfigures of Figure 5 show the rela- throughput rate. However, at high poly- sisted design in the spunbonding nonwo-
tionship between fibre diameter, polymer mer throughput rates, the curves tend to ven process and technology.
melt temperature, fibre crystallinity, fibre approach each other down the spinline.
birefringence, polymer melt velocity and
distance from the spinneret with the pol- Figure 5.e shows the relationship be- Acknowledgements
ymer throughput rate, as presented by the tween the polymer melt velocity and dis- The authors would like to thank Professors
air drawing model, shown in Figure 5. tance from the spinneret with the polymer Zhen-hua Lu and Ying-zheng Liu of the Tur-
throughput rate. The polymer melt veloc- bo machinery Institute at Shanghai Jiaotong
Figure 5.a shows the relationship be- University for assistance in the design and
tween the fibre diameter and distance ity profiles in Figure 5.e indicate that the
construction of the experimental apparatus.
from the spinneret with the polymer final velocity increases with an increase The permission by Phoenics Inc. to use their
throughput rate. This figure shows that in the polymer throughput rate, with the software with an educational license is gra-
the fibre diameter decreases more slowly velocity tending to stabilise at a higher tefully acknowledged.
94 FIBRES & TEXTILES in Eastern Europe 2014, Vol. 22, No. 1(103)
28 300
Polymer throughput rate, Polymer throughput rate,
20 100
18 50
0 60 120 180 240 300 360 0 60 120 180 240 300 360
a) b)
Distance from spinneret, cm Distance from spinneret, cm
60 0.022
50 0.020
Fibre birefringgence
Fibre crystallity, %
40 0.018
0 60 120 180 240 300 360 0 60 120 180 240 300 360
c) d)
Distance from spinneret, cm Distance from spinneret, cm
30
Polymer melt velocity, m/min
25
20
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