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Review Article

Composites and Advanced Materials


Volume 32: 1–18
A review of recent developments in © The Author(s) 2023
Article reuse guidelines:
structural applications of natural sagepub.com/journals-permissions
DOI: 10.1177/26349833221147540

fiber-Reinforced composites (NFRCs) journals.sagepub.com/home/acm

Hossein Abdollahiparsa , Ali Shahmirzaloo, Patrick Teuffel and Rijk Blok

Abstract
Natural fiber-reinforced composites (NFRCs) are expected to find growing applications in near future, especially in Europe
where stringent environmental codes are being legislated and public pressure for their enforcement is increasing. Study has
shown that NFRCs are also gaining recognition among civil engineers as a viable alternative to traditional materials for use as
concrete reinforcement in load-bearing structural members as in building frames and bridge decks. The present review
strives to provide a brief overview of NFRCs, state-of-the-art developments in their manufacture, and examples of their
structural applications. Another aspect of the review involves investigation of the challenges facing the use of fiber
composite materials in civil engineering. These include the high manufacturing costs, difficulties associated with appraisal of
its potential benefits, uncertainties about their properties, lack of understanding among civil engineers of the material and
its service life, and the relatively small battery of standards developed for the composite industry. Finally, the study will
conclude with the prospects of bio-composite applications and the emerging trends in novel bio-composites for future
structural applications.

Keywords
Natural fiber composites, biomaterials, structural application, bio-based composites

Introduction each specific application. Therefore, interest in natural fiber-


reinforced composites (NFRCs) composites is growing
The use of natural fibers in composites dates back to three rapidly2–7 in the transportation sector, aerospace, marine,
thousand years ago in ancient Egypt where straw and clay construction, and automotive industry. It is important to
were combined to build walls. Over the last decade, polymer note that natural fibers have some disadvantages, such as
composites reinforced with natural fibers have won an ever- low thermal stability (likely to degrade at 220–250°C).
increasing attention among both academics and industri- Hydrophilic nature of natural fibers results very poor in-
alists. The growing environmental awareness worldwide terface and poor resistance to moisture absorption. The lack
has led to an increasing interest in natural fibers and their of good adhesion between natural fibers and polymeric
applications so that their study is nowadays considered an
important field.1 There exists a wide variety of natural fibers
that can be employed as reinforcement or fillers. Fiber Department of the Built Environment, Eindhoven University of
composites composed of natural fibers offer such advan- Technology, Eindhoven, Netherlands
tages as high strength, lightweight, and high durability as Date received: 21 September 2022; accepted: 3 December 2022
well as resistance to water, chemical attacks, electric cur-
Corresponding author:
rent, fire, and corrosion. Moreover, they have proved cost Hossein Abdollahiparsa, Eindhoven University of Technology, Unit
effective in most applications as the properties of fiber 406 No. 42, De Lismortel street, Eindhoven 5600 MB, Netherlands.
composites can be engineered to match the requirements of Email: parsa.engi@gmail.com

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en-us/nam/open-access-at-sage).
2 Composites and Advanced Materials

matrix materials, as well as the high moisture absorption of


natural fibers, negatively affect the mechanical properties.
To develop composites with better mechanical properties
and environmental performance, it is necessary to enhance
the hydrophobicity of flax fibers by treating them with
appropriate coupling agents or coating them with appro-
priate resins.
Fiber composite materials such as glass fiber, carbon
fiber, and aramid have been widely used in the automotive
and aircraft industries and are now being used for structural
applications. In structural applications, fiber composites
have been used to rehabilitate existing structures such as
bridges and buildings, especially those that are exposed to Figure 1. Production energy for some fibers.11
the marine corrosive environment.8 Their migration from
the customary automotive, marine, aerospace, and military
industries to the construction industry has continued to gain ingredients as primary components of aerospace and marine
momentum over the last decade as new civil engineering structures.12 The difficulty, however, lies in the evaluation
applications develop. The use of fiber composite materials of the quality of natural fibers for use in such applications.
in civil engineering has now evolved from non-structural The real challenge in this regard lies in the development of a
applications, such as handrails and cladding, to primary general relation capable of capturing and predicting the
structural applications such as building frames, bridge structural and mechanical properties of NFRCs since large
decks, and concrete reinforcement.9 The need for more variations are typically observed in their properties and
environmentally friendly materials has nowadays shifted characteristics.
the attention once paid to synthetic products back to The properties of NFRCs are to a large extent influenced
NFRCs. Manufacturing bricks and pottery with straw- by the type of fiber used, the environmental conditions
reinforced clay is the first known use of natural fiber where the fiber producing plants grow, and the type of
composites.10 Much of the early research and development treatment applied to the extracted fibers.8 These issues are,
in fiber composites was devoted to the use of synthetic in fact, critical deterrents to the generalized use of natural
fibers. Although synthetic fiber composite materials such as fibers in different applications. To address this gap, this
glass fibers, carbon fibers, and aramid are high performance article intends to provide a brief review of the literature on
ones, they are not adequately biodegradable as they are bio-composites, major classes of natural fibers, and real-life
made of non-renewable materials. These environmental engineering applications of natural fibers including load-
benefits as well as the associated cost savings are enough bearing structural members such as beams and roofs in
justification for the use of natural fibers. There is a sub- building frames, bridge decks, and concrete reinforcement.
stantial difference between natural fiber composites and Finally, the current limitations on NFRC applications are
glass or carbon composites in terms of environmental im- investigated in order for researchers and engineers to gain an
pact. Taking into consideration that the energy required to understanding of the design requirements of NFRCs for
produce natural fibers is less than half that for synthetic structural applications in future.
fibers, see Figure 1, can justify this.
Application of natural fibers as a construction material is
not new. It has a long history as old as the Persian civili-
Natural fibers
zation in old Iran where many cities and towns still host The new legislation and codes in the US and Europe (and to
ancient monuments and buildings made of adobe. Indeed, a lesser extent in other parts of the world) are now fueling an
parts of Iran are museums of the adobe culture. Long before insatiable hunger for novel recyclable and/or biodegradable
a century ago, people in many small towns and villages in materials to avoid the financial penalties. Moreover, a
China and Korea had already learned to mix straw and mud corresponding interest is growing among materials scien-
to make adobe for building walls. These peoples, however, tists to use natural fibers extracted from wood or such plants
had no idea how they could systematically study the fun- as hemp, flax, jute, kenaf, ramie, and sisal in manufacturing
damental mechanisms and processes involved in the re- new composites. Natural fibers offer such advantages as
inforcing effect of natural fibers and what could be done to biodegradability, appropriate mechanical properties such as
maximize their performance in strengthening structures. high strength and stiffness due to their high cellulose
Currently, however, NFRCs have found wide applications content,13 and sustainability, which make them attractive
in the automotive and building industries and there is still alternatives to synthetic reinforcing fibers commonly used
more room for their development in such structural in composites.14 These have led to a strong resurgence of
Abdollahiparsa et al. 3

Figure 2. Classification of natural fibers.16

interest in natural fibers over the past decade. If used in the highest specific young’s moduli and tensile strengths
combination with a degradable polymer matrix, natural albeit with a great variability.18
fibers also serve as an inexpensive, renewable, and less toxic Mechanical properties of natural fibers composite are
alternative to synthetic fibers. Natural fibers are mainly of affected by some factors, these are listed below:
plant, mineral, or animal origin (Figure 2). The first is
essentially comprised of cellulose, while the last is protein- (1) Selecting fibers (extraction method, type, harvest
based. However, in the composites industry, natural fibers time, treatment and fiber content)
are often referred to as vegetable fibers.15 Plant fibers de- (2) Resin type
rived from bast (stem, soft tissues, or sclerenchyma); plant (3) Stacking sequence of fibers
leaf, seed, fruit, and wood; or cereal and grass straw are (4) Interfacial strength
generally the most popular of natural fibers used as rein- (5) Manufacturing process
forcement in fiber-reinforced composites.6,16
Natural fibers are strong, lightweight, considerably cost- Traditionally, especially in rural areas in developing
effective, abundant, and renewable. An important issue countries, natural fibers have been cultivated and used
concerning natural fibers, however, is the scant literature extensively for such non-structural applications as multi-
reports on their mechanical properties. This is even more purpose ropes, bag, broom, fish net, and filters. These fibers
complicated by the lack of standard methods for their se- have also been used for housing applications as roofing and
lection, collection, treatment, processing, and post- wall insulation. Figure 3 presents pictures of coir (obtained
processing.6,16 The properties of natural fibers depend from the husk of coconut fruit), sisal twine, jute, gomuti, and
mainly on the nature of the plant, the locality where it is short hemp fiber.
grown, plant age, and the extraction method used17 Table 1 These fibers are generally coarse-textured with colors
reports the properties of some natural fibers and the main varying from white to dark brown. Sisal fibers, extracted
types of glass fibers (E-glass). Clearly, flax, hemp, and from the leaves of sisal plant, are stiff and relatively coarse-
ramie fibers amongst the cellulose-based natural fibers have textured, even though less coarse than coir. Gomuti fibers,
4 Composites and Advanced Materials

Table 1. Properties of natural fibers and synthetic fibers.18

Stiffness/young’s Specific tensile


Failure Tensile strength modules strength Specific young’s
Fiber Density (g/cm3) Length (mm) strain (%) (MPa) (GPa) (MPa/cm 3) modules

Ramie 1.5 900–1200 2.0–3.8 400–938 44–128 270–620 29–85


Flax 1.5 5–900 1.2–3.2 345–1830 27–80 230–1220 18–53
Hemp 1.5 5–55 1.6 550–1110 58–70 370–740 39–47
Jute 1.3–1.5 1.5–120 1.5–1.8 393–800 10–55 300–610 7.1–39
Harakeke 1.3 4–5 4.2–5.8 440–990 14–33 388–761 11–25
Sisal 1.3–1.5 900 2.0–2.5 507–855 9.4–28 362–610 6.7–20
Alfa 1.4 350 1.5–2.4 188–308 18–25 134–220 13–18
Cotton 1.5–1.6 10–60 3.0–10 287–800 5.5–13 190–530 3.7–8.4
Coir 1.2 20–150 15–30 131–220 4–6 110–180 3.3–5
Silk 1.3 Continuous 15–60 100–1500 5–25 100–1500 4–20
Feather 0.9 10–30 6.9 100–203 3–10 112–226 3.3–11
Wool 1.3 38–152 13.2–35 50–315 2.3–5 38–242 1.8–3.8
E-glass 2.5 Continuous 2.5 2000–3000 70 800–1400 29

Figure 4. Schematic view of a composite material.21

2017).19 These facts highlight the crucial need for a change


toward more sustainable methods of building in the near
future.

Bio-Composites
Figure 3. Pictures of some natural fibers.8
Composite is a combination of two or more materials in
which one serves as the reinforcing phase (fiber, sheet) and
the other as the matrix phase (polymer, ceramics, or metals).
obtained from Arenga Pinnata (sugar-palm) tree, are gen- Figure 4 shows a hybrid material made of a polymer resin
erally stiff and black in color. Hemp and jute fibers have reinforced with fibers; the composite combines the high
finer textures and are smaller in diameter than coir, gomuti, mechanical and physical properties of the fibers used with
and sisal ones but larger than glass fibers (diameter: 2.5– the bonding and physical properties as well as the appealing
10 μm)8. appearance of the polymer.20,21
The construction industry consumes more than 40% of The term ‘bio-composites’ broadly covers those com-
global resources and more than 35% of the global energy to posite materials in which at least one constituent is bio-
produce around 50% of the non-recyclable waste. Until based. Examples include i) non-biodegradable, bio-fiber
now, aggregate materials and concrete have been the pre- reinforced polymers derived from petroleum (e.g., poly-
dominant materials used by the building industry in the EU olefins, polyester, epoxy, vinyl ester, and phenolics); ii) bio-
(UN Environment and International Energy Agency, polymers (e.g., PLA) reinforced with bio-fibers (e.g., jute);
Abdollahiparsa et al. 5

Figure 5. Classification of bio-composites.22,23

Figure 6. Types of natural fiber reinforcement.6

and iii) bio-polymers reinforced with such synthetic fibers While bio-composites with at least one biomass-based
as glass or carbon fibers. Depending on the nature of the component manufactured mostly as wood polymer com-
constituents, bio-based composites may be classified into posites (WPCs) that consist of wood and agricultural res-
partly eco-friendly and green (Figure 5). By green is meant a idues bonded together by thermoplastics found their first
composite whose components are obtained from renewable applications in the building industry back in the 1990s,
sources, potentially reducing carbon dioxide emissions and those containing lignocellulosic fibers were first employed
reliance on petroleum-derived materials. While partly eco- in the automotive industry by Henry Ford in the 1940s.
friendly composites have one constituent, either the fiber or Other than the car industry, the natural fiber-reinforced
the matrix, not obtained from renewable sources.22 polymer composites (NFPCs) have found building and
Natural fiber composites depend for their performance construction, aerospace, and sports applications in such
directly on the fiber counts, length, shape, and arrangement/ products as partition boards, ceilings, boats, office products,
orientation as well as their interfacial adhesion to the ma- and machinery. NFPCs have found their greatest applica-
trix.24 Natural fiber reinforcement may be classified based tions as non-load-bearing indoor components in buildings
on fiber length, dimension, and orientation as shown in because of their vulnerability to outdoor environmental
Figure 6. Reinforcement may come either as fiber or par- attacks.25 In contrast, natural fiber reinforced composites
ticle. When in fiber form, it may be either continuous or also enjoy such advantages as high stiffness to weight ratio,
discontinuous (i.e., chopped) depending on the length-to- lightweight, and biodegradability that make them especially
diameter ratio (l/d). Commonly, fiber-reinforcement may suitable for different applications in the construction
assume a woven or a non-woven arrangement. A woven industry.26
fabric is characterized by continuous interlacing of per- Green buildings are expected to offer ecologically sound
pendicular yarns arranged in a regular pattern, with yarn and healthy places for people to live and work in. Presently,
referring to structures consisting of several interlocked bio-composites are regarded as the major type of material to
fibers.6 make green buildings possible. Based on the type of
6 Composites and Advanced Materials

application in buildings, bio-composites may be classified hydrophilicity of natural fibers results in their high moisture
into two principal groups of products: (1) structural bio- absorption and weak adhesion to hydrophobic matrices. As
composites used as bridge and roofing and (2) nonstructural a remedy, natural fibers can be treated in order to improve
components including windows, exterior building façade, their adhesion to matrix materials. Additionally, most
composite panels, and door frames.27 Furthermore, bamboo natural fibers have low degradation temperatures (∼200°C),
fibers can be used as reinforcement in structural concrete which makes them incompatible with thermosets that have
elements while sisal or coir fiber composites may be used as high decomposition temperature especially when thermoset
roofing components to replace asbestos or asphalt.28 Natural have been hardened with maleic anhydride. This range of
fiber reinforced concrete sheet (both plain and corrugated) degradation temperature also restricts natural fiber com-
and board products in construction applications are light in posites to relatively low temperature applications. Appli-
weight and ideal for use in roofing, ceiling, and walling for cation of natural fibers for industrial purposes has been
affordable housing projects.29 Table 2 reports the various claimed to face such other challenges as large variability in
industrial applications of cellulosic fibers. mechanical properties,32,33 low ultimate strength, low
As already mentioned, bio-composites offer the potential elongation, clogging nozzle flows in injection molding
for “greening” our planet by reducing our dependence on machines, bubbled products, and poor resistance to
petroleum products; unfortunately, however, this potential is weathering.34
yet fully exploited since structural applications of bio- In practice, the major drawbacks of using natural fibers
composites by the industry has been limited by the diffi- are their high degree of moisture absorption (Table 3)19 and
culties associated with taking full advantage of the me- poor dimensional stability. Numerous NFRC is composed
chanical properties of natural fibers.30 of cellulose, a natural polymer with three hydroxyl groups
On the other hand, the main challenge in using these (one oxygen atom covalently bonded to one hydrogen atom)
natural fibers in various polymer matrixes lies in their poor per repeating unit. As long as moisture from the atmosphere
compatibility with the matrix due to their inherently high comes in contact with the fiber, the hydroxyl groups form
moisture absorption that causes dimensional changes in the new hydrogen bonds with water molecules, whereby fiber
lignocellulosic-based fibers. The efficiency of a fiber re- cross section area becomes the main surface exposed to
inforced composite depends on the fiber/matrix interface water penetration. The interaction between hydrophilic fiber
and its ability to transfer stress from the matrix to the fiber. and the hydrophobic matrix causes fibers to swell within the
Stress transfer, indeed, plays a key role in sustaining the matrix that weakens the bonding strength at the interface,
mechanical properties of the resulting composite.31 The leading to dimensional instability, matrix cracking, and poor

Table 2. Natural fiber composite applications in industry.8

Fiber Application in buildings, construction, and others

Hemp fiber Construction products textiles, cordage, geotextiles, paper and packing, furniture, electrical, manufacture bank notes
and manufacture of pipes
Oil palm fiber Building materials such as windows, door frames, structural insulated panel building systems, sidings, fencing, roofing,
decking, other building materials13
Wood fiber Window frame panels, door shutters, decking, railing systems and fencing
Flax fiber Window frame, panels, decking, railing systems, fencing, tennis racket, bicycle frame, fork, seat post, snowboarding, and
laptop cases
Rice husk fiber Building materials such as building panels, bricks, window frame, panels, decking, railing systems, and fencing
Bagasse fiber Window frame, panels, decking, railing systems and fencing
Sisal fiber In construction industry such as panels, doors, shutting plate, and roofing sheets; also, manufacturing of paper and pulp
Stalk fiber Buildings panel, furniture panels, bricks, and constructing drains and pipelines
Kenaf fiber Packing materials, mobile cases, bags, insulations, clothing-grade cloth, soilless potting mixes, animal beddings, and
material that absorbs oil and liquids
Cotton fiber Furniture industry, textile and yarn, goods, and cordage
Coir fibers Building panels, flush door shutters, roofing sheets, storage tank, packing materials helmets and postboxes, mirror casing,
paperweights, projector cover, voltage stabilizer cover, a filling materials for the seat upholstery, brushes and brooms,
ropes, and yarns for nets, bags and mats, as well as padding for mattresses, seat cushions
Ramie fiber Use in products as industrial sewing thread, packing materials, fishing nets, and filter cloths. It is also made into fabrics for
household furnishings (upholstery, canvas) and clothing, paper manufacture
Jute fiber Buildings panels, roofing sheets, door frames, door shutters, transport, packaging, geotextiles, and chip boards
Abdollahiparsa et al. 7

Table 3. Moisture absorption tendency of several natural fibers.17

Type of fiber, %

Moisture absorption tendency, % Jute Banana Coir Flax Mesta PALM Sisal Wood Sun Hemp Ramie

Absorbancy 12.5 10–15 10–12 7 13 10–13 10–12 — 10–11 5–6


Transverse swelling in water 20–22 16–20 5–15 20–25 20–22 18–20 18–20 — 18–20 18–20

mechanical properties of the final composite.35 Preventing diminished by surface treatment or resurfacing of natural
moisture absorption by the fiber is, therefore, an essential fibers with NaOH or AlCl3, H2SO4, or Ca(OH)2.38–42
step in manufacturing composites. This can be achieved Moreover, additional protection may be provided by ap-
through different chemical treatments to eliminate the hy- plying coating materials on these structures to avoid
drophilic hydroxyl groups from the fiber structure.36 weathering attacks. Overall, natural-fiber composites are
In the absence of chemical agents, physical treatments seen as potentially useful materials for many engineering
have been employed to achieve improved natural fiber applications despite their drawbacks outlined above that
composites. The physical treatments proposed for altering limit their use in near future. In this regard, fracture me-
the structural and surface properties of fibers have been chanics might be exploited to gain insight into the physical
classified into the following four groups: (i) corona, (ii) conditions and processes within these composites that might
plasma, (iii) heat treatments, and (iv) steam pre-treatment.37 help the production of natural-fiber composites with im-
The properties of natural fibers for engineering appli- proved properties.43
cations have not yet been adequately addressed in most
previous research. However, some of the major issues raised
Structural application of natural
include high moisture absorption (5–10%), flammability,
inconsistent raw materials and their properties, and bonding fiber-reinforced composites (NFRC)
between natural fibers and polymeric matrices; these appear Natural fibers as construction materials are not entirely new;
to be the most pressing disadvantages that must be lifted in in fact, they have been used since the early seventies. In
order to adapt natural fiber to real-life applications. Locality, Bangladesh, primary schools were constructed using jute
climate during source plant growing period, plant part fiber reinforced polyester in 1972–1973 as the first natural
harvested for fiber extraction, and plant maturity are also the fiber composite material to be used in a developing
factors that influence the properties of the extracted NF country.39 Natural fiber composites have already been used
since they raise uncertainties regarding the properties of to produce non-structural elements in the automotive in-
natural fibers for product development.12 Cementitious dustry. A study reported in 1986 that coir/polyester com-
materials are recognized as tension-weak materials, in posites were being used to produce mirror casing,
which micro-cracks easily form on the product surface or at paperweights, projector cover, voltage stabilizer covers,
the interface between the cement phase and the aggregates mail-box, helmets, and roofs.40 In the 1980s, Jamaican,
after the hydration reaction is complete. Even though tensile Ghanaian, and Philippine houses were constructed using
loading can be resisted by the embedded steel bar rein- building panels and roofing sheets made from bagasse/
forcement, shrinkage and reduced moisture content cause phenolic. As part of a program to develop wood substi-
micro-cracks during the hydration process. For concrete tutes for packaging and construction, the Government of
structures, cement is the fundamental substance to bond all India supported the development of composite products
the aggregates (i.e., sand, filler, and small and large ag- based on jute. Many attempts have been made to use natural
gregates) together to form structures of high compressive fiber polymer composites to fabricate wall panels, roof
strength. sheets, temporary shelters, and post office boxes, but such
Fiber distribution is also important for in-house or on-site composites fail in wet conditions, either by swelled fibers or
applications. Large amounts of agglomerated fiber would by delamination, due to crack growth between plies.39
cause substantial reductions in concrete strength. Hence, Burgueno et al. have shown that bio-composites are able
many studies in the past have used short natural fibers as a to be used as load-bearing members by arranging their
measure to enhance the tensile strength of the cement phase cellular materials in a way that increases their structural
and, thereby, to minimize the probability of cracking. This is efficiency. To prepare laboratory-scale periodic cellular
why application of natural fiber-cement composites in beams and plates, they impregnated hemp and flax fibers
residential housing projects has been limited to building with unsaturated polyester resin. Tests were conducted on
exterior parts such as siding and roofing. It has been shown, their specimens in order to assess their material and
however, that degradation due to such harsh environmental structural performance. The results were compared to those
conditions as high humidity and temperature may be obtained for short-fiber composite micromechanical models
8 Composites and Advanced Materials

and sandwich analyses. In conclusion, a short-term ana- Beams


lytical assessment of full-scale cellular bio-composite
components concluded that their properties were compa- As the structural members of buildings, bridges, and similar
rable to those of conventional components. structures, beams are traditionally made from wood, re-
Natural fiber-reinforced polymeric structural insulated inforced concrete, steel profiles, or laminated veneer lumber
panels (NSIPs) were developed by Uddin et al. for use in (LVL). Meant to resist bending or flexural stresses, struc-
panelized construction. The sandwich panel is made from tural beams are subjected to three- or four-point bending
skins of laminated polypropylene reinforced with jute, and a tests to determine their load capacity, flexural stress, strain,
core of expanded polystyrene (EPS). The structure was deflection, and modulus of elasticity. It is now possible to
characterized using flexural and low-velocity impact tests. design structural beams and pedestrian bridge girders with
The results of both tests confirmed that NSIPs could serve as loads ranging from low to moderate by using NFRCs. As a
an alternative to OSB SIPs and G/PP SIPs for structural result of their low density and low cost as well as their
applications such as floors and walls.43 environmental benefits, natural fiber composites have been
Despite the many studies conducted so far, no satis- considered for beam development. Recent studies have also
factory results have yet been obtained concerning the shown reduced cost, lower weight, as well as faster and
structural characteristics or economic advantages of easier installation procedures as advantages of fiber com-
NSIPs. A bio-based building component that offers higher posites used as beams.
structural performance is normally associated with sig- The concept of composite sandwich beams due to Dweib
nificantly higher cost, at least due to its larger dimensions. et al.47 is one of the many feasible ones in which several
On the other hand, reducing dimensions to maintain costs layers of materials are combined to form a single structural
within an affordable range will only produce building element. The ultimate goal is to develop monolithic
components of a low structural performance which may structural panels suitable for use as (load-bearing) roofs,
not be able to compete with conventional building ma- flooring, or walls in housing or low-rise commercial
terials. For instance, Singh et al. reported that the single- building projects. The beams thus manufactured have been
layered natural fiber-based panel used as an alternative to subjected to the four-point bending test to determine their
plywood lacked the desired qualities in terms of specific strength, stiffness, and failure mode. First, small unit beams
strength, stiffness, and dimensional stability to be used as a have been designed and fabricated using vacuum-assisted
building material. To deal with this problem, hybrid nat- resin transfer molding (VARTM) technology in which the
ural fibers have been used to develop a composite lami- preform is vacuum-bagged on a one-sided mold, as shown
nate.44 Christian et al. suggested that the shape of in Figure 9, and resin is drawn into the preform from above
structural components could be modified in a way to by sub-zero pressure. Due to the prohibitive costs of high-
prevent the large deflections of natural fiber composites temperature post-curing, room temperature curing of the
due to their low modulus of elasticity.45 Using Natural resin has been found necessary for the manufacture of large-
Fiber Reinforced Plastics (NFRP), Fajrin et al. developed a scale structures.
novel building component they named ‘hybrid structural A sandwich beam is constructed with soybean-oil-based
insulated panels’ (hybrid SIPs). Their test results showed resin, natural fibers (such as flax, recycled paper, and
improved structural properties of the novel hybrid SIPs. chicken feathers), E-glass fiber, and closed cell structural
The authors found that laminates made from the two types foam. Figure 10 shows a schematic illustration of the
of jute and hemp natural fibers and used as an intermediate prototype beam studied in Dweib et al. The beam has a top
layer to form hybrid SIPs would significantly improve the horizontal face sheet, a bottom horizontal face sheet, and
load-carrying capacity of the panels thus made.46 In this two vertical webs.
technique, a natural fiber-reinforced plastic (NFRP) lam- In spite of the fact that the authors reported that recycled
inate is placed as an intermediate layer between the alu- paper produced good composites when they made flat
minum skin and the EPS core to produce a hybrid SIP sheets of composite, they failed to make a three-dimensional
(Figure 7). Figure 8 presents the load-deflection curve structure due to problems with resin flow. In order to
obtained from the full-scale test of structural insulated overcome the problem, other porous fibers, such as recycled
panels. paper, were used along with the main reinforcement
Several load-bearing components have been developed (i.e., recycled paper), to provide flow channels for the resin,
with natural fiber composites, including beams, roofs, particularly through the beam web. An example of how
multipurpose panels, and pedestrian bridges. More interest porous fiber mats were used in combination with recycled
is now being shown in investigations to determine the paper to deliver a better resin flow and properly-infused
suitability of natural fiber composites for structural appli- beams can be seen in Figure 11.
cations that require moderate strength, reduced production The five beam types used in Dweib et al. were subjected
costs, and environmentally friendly features. to four-point bending tests to study their strength, stiffness,
Abdollahiparsa et al. 9

Figure 7. Typical distribution of stress in conventional and hybrid SIPs (above and below).46

Applying this type of composite in building construction


brings various advantages such as desired ductility, high
strength, and stiffness to weight, survivability in severe
weather conditions, fatigue resistance, and design
flexibility.47

Roof
In developing countries, roofing materials are in high
demand due to population growth, the increasing need for
construction materials, and the desire to renovate and
rehab existing homes. In rural tropical Africa, more than
90% of roofs are made with traditional materials such as
grass, coconut leaves, or palm leaves. Tropical environ-
Figure 8. Load-deflection curve of the full-scale structural ments have high rainfall and humidity along with a high
insulated panels.46 incidence of insects and pests that feed on cellulosic
materials, which makes these materials insufficient, which
limits the life of a roof to just a few years.48 The use of
corrugated iron and aluminum roofing materials has in-
and failure mode in a pure bending mode. Table 4 sum- creased in recent years. Peasants, however, are not only
marizes the key results obtained, including failure load, faced with high prices but are also in short supply of these
maximum recorded strain, and global modulus while products. There have been a number of attempts to in-
Table 5 describes the failure modes experienced by the five troduce ceramic tiles, but their higher timber requirements
beams tested. Five different structural beams were suc- and greater skill requirements have made them uneco-
cessfully manufactured and mechanically tested giving nomical to introduce. In Tanzania, natural fiber-reinforced
good results. cement tiles (reinforced with asbestos or sisal fiber) are
10 Composites and Advanced Materials

Figure 9. Schematic view of the VARTM process when a structural part is infused.47

Figure 10. A schematic diagram showing the dimensions of test beams (inches).47

manufactured on a small scale. Materials in this category resources of fibers and resins. The author claimed that even
are heavy and fragile, and therefore they cannot be handled though these materials are not as strong as most conven-
on a rudimentary level in rural Africa and other developing tional materials, their development and subsequent de-
countries. Recently, vegetable fiber-reinforced polymers ployment in developing countries might revolutionize the
have been utilized for roofing and other building purposes. construction industry in these countries, especially for the
A low-cost housing solution has been developed to con- rural peasant population. It makes sense that vegetable fi-
struct houses entirely out of jute and polyester composites bers like sisal growing in these areas would provide strength
using basic hand lay-up methods and filament winding and stiffness comparable to glass fiber. In addition, chemical
molding.49 treatment can be applied to the fiber surface to create an
The work of Bisanda demonstrated the potential for interface that is compatible with most thermosetting resin
developing useful engineering products from natural matrices. The cost of synthetic resins is higher than that of
Abdollahiparsa et al. 11

Figure 11. A schematic view of the porous fiber in the preform.47

Table 4. An overview of the failure load, maximum strain, and modulus.47

Beam global modulus, MPa (ksi)


Reinforcement fiber Failure load kN (klb) Maximun strain, με from deflection-load data

Flax mat 10.2 (2.3) 9842 300 (43.5)


Woven E-glass fiber 39.3 (8.83) 4273 1580 (229.2)
Recycled paper/chicken feathers 24.2 (5.44) 15045 950 (137.8)
Recycled paper/corrugated form 25.8 (5.8) 11158 1214 (176.1)
Recycled paper/woven E-glass fiber 25.6 (5.76) 5667 1670 (242.2)

Table 5. Descriptions of the beams’ failure modes.47

Failure description

Flax beam A brittle failure mode was observed. The beam was broken down into two parts.
The location of fracture was between the two loading points, and about 1.5 from
one of the loading point
Recycled paper/chicken feathers beam and recycled A brittle failure mode was observed. The beam was broken down into two parts.
paper/corrugated paper beam The location of fracture was between the two loading points, and about 2.0 from
the center of the beam
Woven E-glass beam and recycled paper with E-glass A non-brittle failure mode was observed. After the maximum loading was reached,
beam the beam began to unload. Finally the beam could hold as a whole, but a
permanent crack close to one of the loading point separated the top face into
two parts

sisal fiber, making these composites less suitable for low- other construction purposes in tropical developing coun-
technology applications. CNSL (cashew nut shell liquid) tries. It has been shown that bio-based composite materials
has been identified as a cheap, naturally occurring resin with can be used not only for roof structures, but also to fabricate
a phenol base. Using sisal fiber in the form of plain-woven structural beams with good results. A large-scale composite
mats, a CNSL-formaldehyde resin matrix has been blended structural panel has been manufactured successfully based
with sisal fiber in compression to form corrugated com- on beam test results. Additionally, natural materials such as
posites. Composite materials and related manufacturing plant oil-based resins and natural fibers have been suc-
processes have been examined in order to determine cessfully utilized as composite components for making
whether corrugated composites are suitable for roofing and roofs for homes at low material and operational costs.50 The
12 Composites and Advanced Materials

Figure 12. Schematic view of the three different foam-core structural composites.50

Figure 13. Schematic view of the hypothetical house.50

Figure 12 illustrates the different possible designs for a successfully used to produce structural panels of this size,
panel made of a composite skin and a foam core. allowing visual inspection of the resin flow and an op-
The bio-based composite roof was designed for a hy- portunity to use additional vacuum and injection lines on the
pothetical ranch-style house with an area of 7.32 m by normally hidden bottom side.50
15.24 m. Eaves height was 4.75 m (15 ft) and roof rise was
3.05 m (10 ft). Instead of a conventional roof made up of
rafter/truss and plywood, the roof was designed as a
Tiny house
monolithic composite sandwich panel with one-way webs Over the past few years, researchers have been focused on
running from the eaves to the ridge. An illustration of the developing completely novel building materials in response
house is shown in Figure 13. to the need by the growing world population and the tre-
There was a pitched roof consisting of two structural mendous pressure on the climate due to high CO2 emissions
panels of 1.52 m by 2.59 m and a depth of 0.089 m that were by the construction industry, which have resulted in de-
attached at the ridge (Figure 14). A modified vacuum as- forestation, climate change, and the rapidly declining bio-
sisted resin transfer molding process (VARTM) has been diversity. On account of this, the Tiny House prototype
Abdollahiparsa et al. 13

Figure 14. Bagged on a table and under vacuum part ready to be infused with resin.50

Figure 15. Picture of tiny house.52

shown in Figure 15 was presented in Emmen (NL). The functions. For this purpose, use was made of a new tech-
prototype is completely built with bio-composites produced nology known as vacuum injection in which all the ma-
from agricultural products, residual flows, and recycled terials are placed on a foam plate and wrapped in a film
materials so as to confirm it is possible to construct a modern before the air is sucked out to create a vacuum and the resin
home without wood, concrete, or steel structures.51 This is allowed to flow inside. Thus, a sandwich panel is created
prototypical house made out of such natural fibers as burlap, that comprises the roof structure, heat insulation, and eaves
hemp, and flax serves as a strategic step towards full-scale gutter profiles.51
industrial application of bio-composites in construction.52
In the Tiny House project, use was made of insulating
sandwich panels with bio-PUR, paper-based extrusion Bridges
profiles, structural pultrusion profiles with natural fibers, Very few examples have been so far developed of bio-
and 100% bio-resins. In addition, this is a typical example of composites used as infrastructure components. One ex-
what can be done with composites to integrate multiple ample is the pedestrian bridge made by the Eindhoven
14 Composites and Advanced Materials

Figure 16. The bio-composite footbridge, 18 months after the installation across the river Dommel.53

University of Technology (Figure 16), in which the girder is susceptible to moisture and damage while a special coating
a bio-composite of hemp and flax fibers attached to a had been applied on the composite in this case to prevent
polylactic acid (PLA)-based foam core.53 moisture penetration. After years of service, the fibers are
Three alternatives are traditionally in use for bridge still enclosed in the epoxy matrix, making it difficult for
building in the Netherlands, namely concrete, steel, and moisture to reach them. The epoxy, a very durable resin that
composites. Even if environmental concerns are not the keeps out almost anything, accounts for more than fifty
most important factor, composites often come in as the percent of the material used. A coating applied as an extra
winning solution. A composite bridge requires hardly any protective layer can guarantee even higher levels of wa-
maintenance, while a steel bridge has to be painted every terproofing and protection against moisture penetration.
5 years. From a building cost viewpoint, concrete is usually Currently, 100% bio-based resins are being developed but
the cheapest alternative albeit a concrete bridge is impos- more research is warranted before they can be used in
sible in some locations because of its high weight while it building bridges. Once this technology becomes possible,
also occupies more space and takes more time to construct. the composites could in theory be shredded, ground, and
In such cases, a steel bridge might be preferred but only at a scattered all over the land. There will then be no need for
higher cost. It follows that a composite bridge stands as the using different resins to make biodegradable bio-
really most economical solution. Moreover, a bio-composite composites.54 It is a misconception that it is always an
bridge will reasonably be the winner if environmental advantage if a product is biodegradable; this is only true for
concerns are the main factor to consider. In most focus short-lived products like packaging.
points, flax fibers score considerably higher than glass, The Florida footbridge (Figure 18) is part of a 4-year
except for one: land use.54 The Ritsumasyl bridge is made of Interreg NWE research project called Smart Circular Bridge
flax reinforced epoxy, which is more flexible than steel but (SCB) led by Eindhoven University of Technology (our
less stiff than a glass fiber composite (Figure 17). In order to group) and involves 14 partners. 90 FBG sensors were used
ensure the required stiffness would be achieved, the bridge to collect strain and temperature data in real-time. An ex-
design had to be modified solely by increasing bridge perimental application of natural fiber-composites for load-
thickness. bearing purposes is the goal of the SCB project. The design,
Although most materials exhibit a tendency to creep, the production, and construction of two other pedestrian and
creeping in this bridge completely vanished after a while. cycling bridges (one in Germany and one in the Nether-
There were even more surprising results; when tested for lands) will take place in the next 3 years. The SCB project
fatigue in Delft, a lifespan of a hundred years, rather than the proposes a new approach to overcome uncertainties through
required 50 years, was determined for the bridge; this came the use of a structural health monitoring system, which can
as a surprise because natural fibers were thought to be monitor mechanical behavior and assess structural safety.
Abdollahiparsa et al. 15

Figure 17. The bio-composite bicycle bridge “Ritsumasyl.”54

Figure 18. The floriade bio-composite bicycle bridge.

Discussion as outlined above still await remedies while no substantial


progress is yet reported in this regard. This is mainly
Application of natural fibers is on the rise and will because not much research has been devoted to the as-
continue to dominate the market for the years to come. In sessment of the life cycle of natural textile reinforced
real life situations, natural fibers will carry on to be new composites. Moreover, composite processing methods
materials used to make reinforced composites for dif- need further investigation in order to enhance their po-
ferent structural applications. However, their mechanical tential performance.
and chemical properties will remain not fully known for Bio-composites or biodegradable materials (like wood)
some time since they are not synthesized and no specific are characterized by shorter life-spans and require more
methodology is yet known for their manufacturing. The safety provisions to account for rotting and aging. A long-
drawbacks with natural fiber bio-composite application lasting, load-bearing product is highly unlikely to be
16 Composites and Advanced Materials

biodegradable because any biodegradable material might Acknowledgements


encounter problems of moisture penetration in the long run. The authors would like to express his deepest gratitude to Rijk
Water absorption deforms the surface of composites as a Blok for always giving encouragement and providing invaluable
result of swelling that creates voids, leading to reduced suggestions. His enthusiasm, knowledge and exacting attention to
strength and increased mass. The presently available detail have been an inspiration and kept this work on track al-
mathematical and numerical models for predicting the though he recently passed away. We lost a brilliant scientist and an
properties of natural fiber-reinforced composites are not excellent professor in our department. Truly, your spirit is forever
always accurate enough due to the nonavailability of reli- with us.
able input data. In another vein, it is no easy to model natural
fibers as a result of varying diameters along fiber length.
Finally, composite materials reinforced with natural fibers Declaration of conflicting interests
are, in most cases, basically limited to the low to medium The author(s) declared no potential conflicts of interest with re-
load bearing applications. spect to the research, authorship, and/or publication of this article.
These considerations require an enormous amount of
research in future as many of the issues raised in previous Funding
works still await reasonable and convincing answers in
The author(s) received no financial support for the research, au-
order to guarantee the reliability of natural fiber composites
thorship, and/or publication of this article.
for different applications. Thus, those research efforts may
be recommended as prioritized whose goal it is to improve
the properties of fiber-reinforced composites for different ORCID iD
applications. Hossein Abdollahiparsa  https://orcid.org/0000-0002-3291-0311

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