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Article history: The quantity of construction and demolition waste is continually increasing throughout the world, and
Received 17 October 2013 recycling this waste is beneficial and necessary for environmental preservation. Because the permeability
Received in revised form of concrete materials is closely related to their durability, this paper predominately discusses the
19 January 2014
permeability of recycled concretes composed of fly ash and clay brick waste. Various proportions of
Accepted 15 February 2014
Available online 24 February 2014
recycled coarse aggregates obtained from clay brick waste were used to replace natural coarse aggre-
gates. The properties of natural aggregates and recycled aggregates were studied, and recycled aggre-
gates exhibited a higher porosity. Additionally, the strength of the recycled concrete decreased because of
Keywords:
Recycled concrete
the incorporation of recycled coarse aggregates. The permeability of water, air and chloride ions was
Clay brick waste evaluated through water absorption, water permeability, air permeability and chloride ion diffusion tests.
Porosity The results indicated that the permeability of water, air and chloride ions increased when recycled coarse
Permeability aggregates were used. Additionally, the recycled concrete containing clay brick waste had increased
porosity and exhibited a loose paste matrix, which may be the reason for the increased permeability.
Ó 2014 Elsevier Ltd. All rights reserved.
http://dx.doi.org/10.1016/j.jclepro.2014.02.040
0959-6526/Ó 2014 Elsevier Ltd. All rights reserved.
176 L. Zong et al. / Journal of Cleaner Production 70 (2014) 175e182
Table 1 durability, reduces the demand for water, consumes less energy
Chemical compositions of cement. and decreases the pressure on natural resources (Mehta and
Sample Chemical composition (wt%) Monteiro, 2006; Bagheri et al., 2013). Moreover, fly ash is
CaO MgO Fe2O3 Al2O3 SiO2 SO3 Loss
economical, and there are numerous fly ash resources. In this
paper, recycled concretes made with fly ash were studied. Clay
Cement 64.43 1.57 3.26 4.76 20.85 1.47 2.65
brick waste was treated and used as a recycled aggregate. The
Fly ash 4.10 1.30 9.60 26.10 51.21 0.40 6.19
permeability of RAC under different permeation medium was also
investigated and compared with the permeability of natural
concrete.
studied the bond between recycled aggregate concrete and steel
rebars and observed a reduced bond strength between the recycle
aggregate concrete and the plain rebar with increasing replacement 2. Materials and methods
percentages of recycled aggregate (RA). Additionally, Marie and
Quiasrawi (2012) discovered that recycled concrete had a lower 2.1. Materials
workability (slump) compared with normal concrete. Various
waste materials have been utilized as recycled aggregates. Medina Samples were prepared using ordinary Portland Cement (OPC)
et al. (2013) explored the durability of concrete made with aggre- and grade I fly ash. The chemical composition of the cement and
gates containing 20e25% ceramic sanitary ware industrial waste, fly ash are provided in table 1. Crushed stones with a maximum
and their findings showed enhanced concrete freeze-thaw resis- size of 25 mm were used as the natural coarse aggregate, and
tance with increasing recycled aggregate content. Zhao et al. (2013) quartz sand with a fineness modulus of 2.48 was used as the fine
prepared concrete using cathode ray tube funnel glass sand as aggregate. It has been proven that concrete admixtures are
recycled fine aggregates and concluded that cathode ray tube beneficial for material performance, therefore a high perfor-
funnel glass can be treated, processed and reutilized for the pro- mance polycarboxylate water-reducing admixture (PCA) was
duction of high-density concrete. used in this study (Barbudo et al., 2013). A recycled coarse
Most existing research compares the mechanical properties of aggregate was prepared from clay bricks, which were collected
recycled concrete with conventional concrete (Akhtaruzzaman from a construction site. The strength of the waste bricks was
and Hasnat, 1988). According to research achievements, the me- measured according to the National Standard of Fired Common
chanical performance of RAC nearly satisfies the requirements Brick GB5101-2003, and the strength was determined to be MU10
that are imposed for conventional concrete. However, there are (the compressive strength exceeded 10 MPa). The clay bricks
fewer studies on the permeability of RAC. The service life of were crushed and washed before use. The basic performance of
concrete structures depends on the durability of the concrete the RA was evaluated, and the grade, density and crush index
materials. Furthermore, permeability is the most important factor were determined. The physical properties of natural aggregates
that affects concrete durability. The economic impact of concrete (NAs) and recycled aggregates (RAs) made from clay bricks are
durability has motivated over two decades of extensive research. given in Table 2. Fig. 1 illustrates the RA preparation process,
The mechanism that controls permeability depends on the fluid which includes crushing, sieving and grading. Fig. 2 shows the
or chemical species of interest. For example, in concrete, the grading curve of the RAs and NAs. The standard error calculated
permeation of air affects carbonation action, whereas the from the experimental data was less than 1. According to GB/T
permeation of chloride ions affects steel corrosion. Many dura- 14685-2001, the national standard on the use of pebble and
bility test methods consider the penetration of deleterious sub- crushed stone for buildings, and based on grading, the crushed
stances into concrete as a rate-controlling step in the degradation RAs collected from the demolition plant were qualified for use in
process. Highly permeable concrete facilitates the penetration of concrete.
water and harmful substances, which results in the deterioration
of either the concrete or the steel reinforcements embedded in 2.2. Methods
the concrete (Chia and Zhang, 2002). The transport of gases,
liquids and ions through concrete is important because their in- 2.2.1. Preparation of concrete samples
teractions with concrete constituents or pore water can directly All concrete mixtures were prepared in the laboratory. Concrete
or indirectly alter the integrity of the concrete and deteriorate the samples with sizes of 100 mm 100 mm 100 mm,
structure, as mentioned above (Basheer et al., 2001). Experi- 100 mm 100 mm 400 mm, 200 mm 200 mm 200 mm and
mental evidence exists that illustrates a correlation between F100 mm 200 mm were prepared. The proportions of the con-
relevant transport properties and either the penetration of crete mixtures are presented in detail in Table 3. The following RA
different aggressive substances or mechanisms of deterioration levels were used to replace coarse aggregates: 0%, 30%, 40% and 50%
(Dhir et al., 1994). by volume fraction. Additionally, 15% by weight fly ash was used as
Fly ash, a type of industrial waste, has been widely applied in a replacement for cement. Because the RAs have a high saturated
concrete materials. The use of fly ash as a partial replacement for surface dry absorption, similar to recycled aggregates made with
cement in concrete has numerous benefits; it reduces greenhouse old concrete (Mefteh et al., 2013), additional water was used to
gas emissions, demonstrates good long term strength and prepare the recycled concrete. Therefore, the water content in the
Table 2
Physical properties of NAs and RAs.
Sample Apparent density Bulk density (Kg/m3) Grading (mm) Elongated particle Saturated surface dry Moisture Crush index (%)
(kg/m3) content (%) absorption (%) content (%)
Table 3
Mix proportions of concrete.
on the mechanical results, the use of RAC produced with 100% RAs
made from clay bricks is not practical.
Fig. 7. Concrete produced with varying RA content: (a) RA30%, (b) RA40% and (c)
RA50%.
Fig. 10. Water permeability coefficients for concrete. Fig. 12. Carbonation depths of the samples.
The concrete permeability coefficients are given in Fig. 10, and concrete. The greatest increase in the air permeability coefficient
the data indicate a significant increase in the permeability coeffi- was approximately three-fold. Concrete mixes were designed
cient of RAC that is cured for 28 days. Concrete mixtures with 50% with varying proportions of RA content (0%, 30%, 40% and 50%) by
RA exhibited the highest water permeability and showed an mass, and the mix with 30% RA exhibited the smallest increase in
approximately two-fold increase compared with the water air permeability. However, the air permeability of RAC is still
permeability of NAC. Additionally, increased water penetration was within the accepted range for conventional concrete that is not
observed when a higher replacement rate of RA was used. This is exposed to aggressive environments (1018e1017 m2) (Perraton
attributed to the more porous characteristic of RAs made from clay et al., 1988). The carbonation depth of the concrete samples
brick waste. As previously mentioned, water plays an extremely was determined to evaluate the permeation of air. The carbon-
important role in the durability of concrete structures and is ation behavior of RAC is not only determined by the quality of
essential for many damaging actions that reduce the performance new mortar but also by the quality and quantity of RA. The results
of concrete materials. Therefore, the application of RAC made with of the carbonation test for different concrete mixes are shown in
clay brick waste should be limited in coastal or subsurface Fig. 12. The RAC also exhibited a greater carbonation depth.
structures. Furthermore, the carbonation depth increased with increasing RA
replacement percentages. After being cured in a CO2 environment
for 28 days, the carbonation depth of NC was approximately
3.3. Air permeability 8.9 mm. Moreover, the carbonation depths of the RCs were
10.5 mm, 13.7 mm and 14.5 mm, respectively. Therefore, it can be
The air permeability coefficients for the four different mix- concluded that RAC produced with crushed clay bricks has a
tures are given in Fig. 11. The replacement of natural aggregates lower carbonation resistance than conventional concrete.
with recycled aggregates increased the air permeability of Because carbonation can accelerate the corrosion of steel bars in
Fig. 11. Air permeability coefficients for concrete. Fig. 13. Chloride ion permeability of concrete.
L. Zong et al. / Journal of Cleaner Production 70 (2014) 175e182 181
3.5. Microstructure
4. Conclusions clay brick waste and fly ash. The results indicated that the water
absorption of recycled concrete was higher than that of normal
Aggregates are a major component of concrete and signifi- concrete. The permeability of water, air and chloride ions was
cantly affect the engineering properties of concrete mixtures. On enhanced when recycled coarse aggregates were used, and
one hand, the supply of natural resources is diminishing; how- higher RA contents further increased concrete permeability.
ever, on the other hand, construction waste is increasing, which Recycled concrete containing crushed clay bricks demonstrated
is producing significant environmental pollution. Reusing waste poor impermeability. The addition of RAs formed a loose paste
bricks as recycled aggregates not only solves the problem matrix that contained pores and voids, which can increase
regarding the shortage of natural stones but also effectively permeability. Based on the combined results in this study, it was
utilizes construction waste. According to results of this study, the possible to blend crushed clay bricks to produce RAC, and the
density of concrete samples decreased as the content of RA concrete mix containing 30% RA was more economical and per-
increased. Both the compressive and flexural strength also formed the best. However, further research is required to
decreased when RAs were used. Furthermore, the durability of determine the practical applications of using recycled concrete
concrete materials depends on their permeability. Therefore, this containing RAs from crushed clay bricks, especially in severe
study also determined the permeability of RAC produced with environmental conditions.
182 L. Zong et al. / Journal of Cleaner Production 70 (2014) 175e182
Acknowledgments Limbachiya, M., Meddah, M.S., Ouchagour, Y., 2012. Use of recycled concrete
aggregate in fly-ash concrete. Constr. Build. Mater. 27, 439e449.
Marie, I., Quiasrawi, H., 2012. Closed-loop recycling of recycled concrete aggregates.
This research was supported by the National Natural Science J. Clean. Prod. 37, 243e248.
Foundation of China (No. 51108231) and is a Science and Technol- Martínez-Lage, I., Martínez-Abella, F., Vázquez-Herrero, C., Juan, L.P.O., 2012.
ogy Planned Project for the Ministry of Housing and Urban-rural Properties of plain concrete made with mixed recycled coarse aggregate. Constr.
Build. Mater. 37, 171e176.
Development of China (No. 2013-K4-20). Medina, C., et al., 2013. Freeze-thaw durability of recycled concrete containing
ceramic aggregate. J. Clean. Prod. 40, 151e160.
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