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quantified using average velocity gradient values (G values) alone. The computational fluid
dynamics (CFD) process was used to investigate the turbulent flow characteristics of a
three-stage hydraulic flocculation facility at the J.D. Kline Water Supply Plant in Halifax,
Nova Scotia. Calculations of the local velocity gradient were achieved using predicted
energy dissipation rates. CFD analysis showed unbalanced mixing conditions in the
hydraulic flocculation tanks resulting from short-circuiting and from recirculation zones.
Inconsistent mixing energy, interrupted with severe spikes in the localized G values at the
weir columns, led to little or no mixing energy in most of the regions in the flocculation
tanks. Practical outcomes of operating at such varying mixing gradients can be detrimental
to the flocculation process and overall organic removal in the treatment plant.
Assessment of hydraulic
flocculation processes
using CFD
C
oagulation and flocculation are key processes in optimizing natu-
ral organic matter removal and subsequent mitigation of disin-
fection by-products (DBPs) formation (Jarvis et al, 2008). Proper
use of coagulant type and dosage, optimal pH and alkalinity con-
ditions, and mixing arrangements are imperative for effective
destabilization of particles through the coagulation process. Subsequent
YAMUNA S. VADASARUKKAI, enhancement of contact between the coagulant, destabilized particles, and
primary particles in water occurs predominantly in the flocculation process
GRAHAM A. GAGNON,
through gentle mixing for 20 to 45 min (Crittenden & MWH, 2005). The
D. REID CAMPBELL, flocculation process promotes the agglomeration of particles—called flocs—to
form irregularly shaped aggregates that can be filtered or settled. These aggre-
AND SARAH C. CLARK
gates are then removed in downstream separation processes (e.g., sedimenta-
tion, filtration, dissolved air flotation).
Floc characteristics (i.e., size and structure) formed during coagulation–floc-
culation processes govern the performance of downstream processes for
improved particle and microbial removal (Jarvis et al, 2008). The flow condi-
tions in flocculation tanks are driven by localized fluid turbulence, and the
resulting flocs are subjected to varying shear rates. The resulting nonuniform
energy distribution (i.e., in the x, y, and z directions) within the tank relates
TABLE 1 Examples of flocculator designs used in conventional and direct-filtration WTPs in Canada
Type of Flocculator
Treatment Capacity
WTP Type ML/d Mechanical Hydraulic Reference
Conventional
Mannheim WTP (Kitchener, Ontario) 72.6 Yes No Arnold, 2008
R.L. Clark WTP (Toronto, Ontario) 415 Yes No City of Toronto, 2010b
R.C. Harris WTP (Toronto, Ontario) 453 No Yes Hargrave et al, 1990
Direct filtration
Island WTP (Toronto, Ontario) 410 No Yes City of Toronto, 2010a
Prescott WTP (East of Brockville, Ontario) 8.2 Yes No Doyle et al, 2002
Point Pleasant WTP (Kingston, Ontario) NA Yes No Kingston Utilities, 2009
Sydenham WTP (Kingston, Ontario) NA No Yes Kingston Utilities, 2009
F.J. Horgan WTP (Toronto, Ontario) 570 Yes Yes Doyle et al, 2002
J.D. Kline WTP (Halifax, Nova Scotia) 95 No Yes
(6a)
2
冕
Nn Nn
冢 冣
exp –
(1 – n)
M M 冢 冣 2
t2m
0
(1 – )2 E( )d (9)
2
These two important parameters, tm and Θ , are used to
in which E( ) is a normalized exit age distribution curve; characterize RTD curves (Teefy & Singer, 1990). Com-
n is a fraction of flow rate effectively used in the treat- parison of the calculated tm with the theoretical mean
–
ment process (with no global bypassing); N is the number (HRT t N) yields an insight into the importance of prefer-
of reactors in the series; M is the fraction of a unit’s ential flow paths and stagnation zones in the tank (Ken-
volume effectively used in the treatment process (with no nedy et al, 2006).
stagnation of space); is the normalized residence time, The dimensionless exit-age distribution function E(Θ)
– –
⬅ t/t N (dimensionless); t N is the total mean residence can be statistically related to the cumulative exit-age
– – –
time in N tanks (s), t N = N t s = Vs/Q; t s is the mean distribution, also known as F(Θ) curve, given in Eq 10.
hydraulic residence time (HRT) of a single tank, calcu-
lated as the ratio of volume of the flocculation tank (Vs)
冕 n
in m3 to the bulk flow rate (Q) in ML/d; and is the F( ) E( )d 冱 E (10)
0 1
Dirac delta function, = 0.0069 (assumed).
The TIS model represents the flow through a series of
equal volume of N continuously mixed flow reactors The function F(Θ) has an S-curve when plotted with
(CMFRs), allowing for dead-spaces (1 – M) and global respect to time t bounded between a minimum of 0 and
bypassing (1 – n) over the whole series of reactors. For a maximum of 1 (Templeton et al, 2006). The F(Θ) curve
n = 1 (no bypassing) and M = 1 (no dead-space), it can therefore represents the cumulative probability of x frac-
be seen that Eq 6a simplifies to a well-known single- tion of fluid element leaving the tank at a residence time
parameter RTD function for a series of completely of Θx, which is less than or equal to the normalized resi-
stirred reactors (Levenspiel, 1999), as given in Eq 6b. dence time (Θ). Certain flow-through curve characteristics
(e.g., tm, Θ
2, Θ , Θ
x max [normalized time at which E(Θ) is
equal to maximum {dimensionless}]) of both the E(Θ) and
N
E( ) (N )N–1 exp (– N ) (6b) F(Θ) are used as “indicators of flow.” These parameters
(N – 1)!
were used in characterizing the flow behavior in the floc-
culation tanks, which is consistent with other studies
The parameter Θ in the E(Θ) curve represents the num- (Stamou, 2008; Kennedy et al, 2006). The F(Θ) curves
ber of reactor volumes of fluid based on entrance condi- generated from the TIS model were used to compare the
tions that have flowed through the reactor in time t results of the CFD particle-tracking simulations.
(Fogler, 2006), given as For each residence time (Θ), the difference (or error)
t between the F(Θ) predicted by the TIS model and the CFD
⬅
–
tN (7) analysis was calculated (Martin-Dominguez et al, 2005),
given as
– –
in which the total reactor volume is t N = Nt s = Vs /Q.
The function E(Θ) in Eqs 6a and 6b is a normalized
RTD. It characterizes the probability distribution function
of the residence time (Θ) of a fluid element in the total tank
冑冱 冤
imax
i=1
冥
F( i)CFDpredicted – F( i)TISpredicted
2
FIGURE 1 Flow distribution arrangements of the three-stage hydraulic flocculation process of JDKWSP’s direct filtration*
4.0 m
4.0 m
Outflow of coagulated water from the
third rapid mix tank through a weir
1.2 m- (48 in.-) diameter conduit of length 19.5 m Rectangular 1.2 m- (48 in.-) diameter conduit
tank of length 12.8 m
0.6 m- (24 in.-)
diameter pipe
5.0 m
10.7 m
5.0 m
Tapered hydraulic
flocculation tank
Tank 2
m
5
1.
Tank 3
Dual media
filtration unit
*Not to scale
1.2194
1.1585
1.0976
1.0367
0.9758
0.9149
Velocity Magnitude—m/s
0.8540
0.7930
0.6712
0.6103 Inflow (Q total) = 69 ML/d
0.5494
0.4885
Q4 (Qmax) =
0.4276 19.3 ML /d
0.3666
0.3057
Q 3 (Qmin) = 13.6 ML /d
0.2448
0.1839
0.1230 Q 2 = 17.5 ML /d
0.0621
0.0011 Y
Z Q 1 = 18.5 ML/d
X
Qmax—maximum discharge, Qmin—minimum discharge, Qtotal—total inflow into the treatment plant, Qx—discharge in flocculation
tanks, X—depth of tank, Y—width of tank, Z—length of tank
Red circle indicates the inlet location of the third flocculation tank, where minimum discharge occurs.
the wall and the fully turbulent region (Stamou, 2008; initial sets of values and BCs were solved iteratively under
Wang et al, 2008; Baek et al, 2005). steady-state conditions until convergence was attained.
A pressure-based solver using a segregated algorithm Convergence of solution was distinct when the monitor-
was used for all the simulations because of an incompress- ing residuals of the continuity equation were below the
ible flow condition. The numerical algorithm (interpola- tolerance limit of 1 × 10–5 and the momentum equation
tion methods) used to solve the governing equations for along the x, y, and z directions was < 0.001; the total
each individual control volume was “simple” for pres- mass flow rate imbalance between inlet and outlet was
sure-velocity coupling, “standard” for pressure, and less than 0.2%; and the velocity profile of the outlet sur-
“second-order upwind” for momentum, turbulent kinetic face remained constant with the increment in the number
energy, and turbulent dissipation energy. The flow-field of iterations (Vadasarukkai & Gagnon, 2010). All the
problems that were thus generated using appropriate computations were converged within ~ 2,000 iterations.
TABLE 2 Effect of total discharge on flow distribution to flocculation tank inlets (summer simulation at 15oC)
69 18.5 17.5 13.6 19.3 26.9 25.4 19.7 28.0 17.2 2.54
75 20.1 19.0 14.8 21.0 26.9 25.4 19.7 28.0 18.8 2.76
90 24.2 22.8 17.8 25.2 26.9 25.4 19.7 28.0 22.5 3.31
120 32.2 30.5 23.7 33.6 26.9 25.4 19.7 28.0 30 4.41
Qavg—average discharge across the four flocculation tanks, Qx—discharge to flocculation tanks
FIGURE 3 Spatial variation of the G local values for the three-stage tapered hydraulic flocculation tank*
37.5554
35.0665
32.5776
30.0886
27.5997 G floc1 = 9.5 s–1
G floc2 = 3.0 s–1
25.1108 G floc3 = 2.0 s–1
22.6219
20.1329
17.6440
15.1551 G local = 40–50 s–1
12.6662
10.1773
7.6883
5.1994 Y
2.7105 Z
0.2216 X
Glocal — local velocity gradient, Gt—shear work, a dimensionless quality, Gflocx — average velocity gradient
in each flocculation chamber, Qmin1—minimum discharge condition at the third flocculation tank, X—depth of tank,
Y—width of tank, Z—length of tank
*Flocculation design criteria: typical Gt values for flocculation process of 40,000 to 75,000 at 20°C
(AWWA/ASCE, 1997)
TABLE 3 Percentiles of Glocal values for flocculation tanks 1, 2, and 3 at a minimum flow of 13.2 ML/d
Glocal Values—s–1
Flocculation Tank 5th Percentile 50th Percentile (Median) 95th Percentile Average G Value*—s–1
*The average G value was calculated using Eqs 1 and 5 for each flocculation tank.
Path Lines—min.
216.5
hydraulic flocculation tank. The time required for those 201.1
185.6
170.1
particles to reach the outlet was tracked. Initially, par- 154.7
139.2
ticles were released from the inlet surface. This number 123.7
108.3
was generated automatically in the flow modeling sim- 92.8
77.33
ulation software depending on the two-dimensional 61.86
46.4
facets (i.e., the number of two-dimensional triangular 30.93
15.47
Y
Z Dead (stagnant/nonmixing) zones
0
faces) in the inlet surface. Sensitivity analysis was con- X 77 path lines of particles injected at t = 0
ducted to study the effect of increasing the total number
of particles released (Np = 77, 180, 383, 766, 1,665, and t—detention time, X—depth of tank, Y—width of tank, Z—length
of tank
3,363) on the particle residence time. (Np is the total
0.085
0.080
0.075
number of neutrally buoyant particles released using 0.070
0.065
particle tracking analysis.) 0.060
0.055
Figure 5 shows the trajectories of 77 particles, which 0.050
were injected at the inlet surface of the first flocculation 0.045
0.040
chamber and tracked for 308 min. At a total inflow of 0.035
0.025
6.6 ML/d, the theoretical HRT was calculated to be 154 0.020
min (i.e., HRT = volume/bulk flow rate). At that theo- 0.015 Y Z
0.010
retical HRT, the path lines of less than half the number 0.005
X
of particles (i.e., 41 of 77 total particles) were traced at 0.000
0.085
ever, about 10.4% (i.e., 8 of 77) particles were still 0.080
0.075
residing in the tank. This phenomenon can be correlated 0.070
0.065
to the recirculation flow, which was identified in the 0.060
first flocculation chamber during the flow-field analysis. 0.055
0.050
Most of the particles were entrained in the recirculation 0.045
region, whereas the short-circuiting path carried the 0.040
0.035
remaining particles to the second flocculation chamber. 0.025
0.020
As shown in Figures 5 and 6, the path lines of particles 0.015 Z
Y
never visited some portions of the second and third floc- 0.010
0.005
culation chambers. 0.000 X
FIGURE 7 Probability distribution function of the residence time of particles in the hydraulic flocculation tank
1.4
1.2
1.0
0.8
Ni/NP
0.6
0.4
0.2
0.0
0.00 0.45 0.90 1.35 1.80 2.25 2.70
t
Normalized Residence Time — = –
tN
Ni—number of particles that exited the flocculation tank in a discrete time increment of d , NP—number of neutrally buoyant
–
particles initially released, t—detention time, tN—total mean residence time in N tanks, —normalized residence time
The bar represents the density of observations falling within each bin (i.e., residence time); the height of each bar represents
the proportion of particles (ratio) having that range of . The area under the curve gives the probability distribution function of
the particle residence time.
FIGURE 8 E( ) and F( ) curves predicted using the results of particle tracking CFD analysis for the hydraulic
flocculation tank
0.9
1.2
0.8 Particles Leaving Tank at
Cumulative Fraction of
1.0 0.7
0.6
0.8
E( )
0.5
0.6
0.4
0.4 0.3
0.2
0.2
0.1
0.0 0.0
0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 2.2
–
= t/ tN
Normalized Time—
–
CFD—computational fluid dynamics, E( )—exit age distribution, F( )—cumulative exit age distribution, t—detention time, tN—total mean
residence time in N tanks, —normalized residence time
The hatched area indicates the fraction of those particles exiting the outlet—because of dead space and recirculation zones—that are
older than the theoretical hydraulic retention time.
0.8 capacity when the shear rate was reduced. Although the
0.7 JDKWSP has a relatively flat HGL during the plant’s
Leaving Tank at t
TABLE 4 G, t, and Gavgt values of hydraulic flocculators and the recommended design criteria for the flocculation process
G—average velocity gradient value, Gavgt—shear work, a dimensionless quality, t—detention time
*Detention time for the design is the overall mean residence time in N number of flocculation tank-in-series (AWWA/ASCE, 1997).
†Gavgt is approximately calculated as the product of average of velocity gradients in the compartment, assuming equal size tanks, i.e., Gavg = (Gfloc1 + Gfloc2 +
–
Gfloc3)/N and t N (Hargrave et al, 1990).
‡Flocculation design criteria: typical G values and detention time for flocculation process at 20oC (AWWA/ASCE, 1997).
§Average G value in each flocculation tank, calculated corresponding to the inflow condition (i.e., 69–120 ML/d).