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An Introduction to
Radiation Protection
Seventh Edition
An Introduction to
Radiation Protection
Seventh Edition
Alan Martin
Sam Harbison
Karen Beach
Peter Cole
CRC Press
Taylor & Francis Group
6000 Broken Sound Parkway NW, Suite 300
Boca Raton, FL 33487-2742
This book contains information obtained from authentic and highly regarded sources. Reasonable efforts have been made to
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Dedicated to the memory of Marie Cole
Contents
Preface xvii
Authors xix
vii
Contents
xi
Contents
xv
Preface
An Introduction to Radiation Protection is a compre- is also widely used for training at the more advanced
hensive account of radiation hazards and their con- N/SVQ Levels 3 and 4, and in many post-graduate
trol. The book is intended to meet the requirements courses.
of a wide range of readers who are involved, either In Chapter 12 on legislation and regulations relat-
directly or indirectly, with ionizing radiation, includ- ing to radiation protection, while we have concen-
ing nuclear plant designers and operators, medical trated mainly on the requirements of the BSSD and
practitioners and technicians, dentists and research their application in the UK, we have also included
workers. In particular, we believe that the work is brief summaries of the requirements in a number of
suitable for health physics surveyors and technicians other countries. Otherwise, the principles and prac-
who are concerned with the day-to-day control of tice set out in the book are applicable internation-
radiation hazards in nuclear power stations, research ally. Although SI units are used throughout, a table
establishments, hospitals and in industry. of conversion factors is provided for those still using
The book meets most of the requirements of ‘old’ units.
Chapter IV of the European Union’s Basic Safety Every attempt has been made to avoid detailed
Standards Directive (BSSD) ‘Requirements for mathematical treatment, but it has been necessary,
Radiation Protection Education, Training and in some areas, to use some simple mathematics.
Information’ and also covers the general topics on This includes squares, square roots, exponentials,
which Radiation Protection Experts, Medical Physics logarithms and the plotting of graphs on logarith-
Experts and Radiation Protection Officers (as defined mic scales. Where a mathematical treatment is used,
in BSSD Articles 82 to 84) are required to provide we have tried to present it in such a way that, if the
advice. In most practical situations, of course, there mathematics is not fully understood, it does not pre-
are likely to be facility-specific issues that need to be clude an understanding of the chapter in general.
addressed by means of supplementary information As far as possible, each chapter is self-contained
and training. so that the reader can find all the information on a
In the UK, the accepted standards and curricula particular aspect without having to search through
for formal training and qualification in radiation several chapters. The early chapters deal with basic
protection are included at Level 2 in the system of physical principles, the nature of the hazard aris-
National and Scottish Vocational Qualifications ing from the interaction of ionizing radiations with
(N/SVQ) in Radiation Protection, including the biological systems and the levels of radiation which
Level 2 Certificate in Health Physics Monitoring in are regarded as acceptable. Later chapters deal with
the Nuclear Industry (Theory), and the early chapters the methods of measurement and control which are
in the book dealing with the scientific background applied to attain these levels. In the second half of
and the general principles of radiation protection are the book, there are individual chapters on the more
aimed at this level. The later chapters dealing with specialized topics of radiation protection in the
particular aspects of the subject are more detailed nuclear industry, radioactive waste and the decom-
so that, for example, health physics surveyors in a missioning of radioactive facilities, radiation protec-
nuclear power station or technicians in a hospital tion in the non-nuclear industry, radiation protection
can get a deeper understanding of the problems in in medicine and radiological emergencies. There are
their own areas. Experience with previous editions also chapters on legislation, risk assessment and on
has shown that, as a result of this structure, the book the organization of radiation protection services.
xvii
Preface
Each chapter is followed by a summary in note form, of this and earlier editions, the opinions and conclu-
in which the key points are reiterated. In addition, sions expressed in the book are those of the authors.
revision questions, requiring both descriptive and
numerical answers, are provided for the majority of AM SH KB PC
chapters. London
Although we have benefited from many helpful
and constructive suggestions during the preparation
xviii
Authors
Alan Martin formerly ran the consultancy Alan Martin Associates, United Kingdom.
Sam Harbison is a health and safety consultant based in Kent and was formerly Her Majesty’s Chief Inspector
of Nuclear Installations, Health and Safety Executive, United Kingdom.
Karen Beach is a Radiation Protection Adviser and a Senior Lecturer in Radiation Protection in the Nuclear
Department of the Defence Academy, United Kingdom.
Peter Cole is a Radiation Protection Adviser and Professor in the Department of Physics, University of
Liverpool and past president of the United Kingdom Society for Radiological Protection.
xix
The structure of matter
1
The structure of matter
K L M N
Nucleus
The proton (p) carries a positive electrical charge up to eight, and the outer shells have progressively
of magnitude 1 unit on the nuclear scale, and a mass greater numbers. The inner shell is known as the
of approximately 1 atomic mass unit (u). K shell, the second is called the L shell, the third
The electron (e−) has a negative electrical charge the M shell, the fourth the N shell and so on. The
of the same magnitude as the proton’s positive maximum numbers of electrons in the K, L, M and N
charge. It has a mass of 1/1840 u, which, for most shells are 2, 8, 18 and 32, respectively. For example,
purposes, is neglected when considering the mass of the atomic system of zinc, illustrated in Figure 1.1,
the atom. has 30 electrons arranged in four shells.
The neutron (n) is electrically neutral and has a Each atom normally has the same number of pro-
mass of approximately 1 u. It can be helpful in under- tons as electrons. This means that the total positive
standing the processes of radioactive decay (see charge on the nucleus is equal to the total negative
Chapter 2) to regard the neutron as a close combina- charge of the atomic electrons, and so the atom is
tion of a proton and an electron, with the positive normally electrically neutral. Two simple atoms,
charge of the proton being cancelled by the negative those of hydrogen and helium, are illustrated in
charge of the electron. Figure 1.2. This particular hydrogen atom is the only
It should be realized that the charges and masses atom that does not contain neutrons. This is because
on the nuclear scale are extremely small. The elec- the repulsive positive charges do not allow more
trical charge associated with a proton or electron is than one proton to form a nucleus without the pres-
about 1.6 × 10−19 coulombs (C). For comparison, the ence of one or more neutrons.
charge stored in a typical AA-type battery is about
5000 C. Similarly, 1 u corresponds to a mass of about
1.7 × 10−27 kg. 1.4 ELEMENTS AND ATOMIC
The neutrons and protons of an atom form a NUMBER
central core or nucleus, around which the elec-
trons occupy various orbits, normally referred to as In the early stages of the evolution of the universe,
shells. The shell closest to the nucleus can contain the two elements hydrogen and helium constituted
a maximum of two electrons, the second can have essentially 100% of matter (apart from a very small
2
1.5 Isotopes and mass number
(a) (b)
e– e–
Ip In
Ip
In Ip
e–
Hydrogen Helium
quantity of lithium). However, processes occurring About 25 elements of a higher atomic number
during the life cycles of early generations of stars have been artificially produced in small quantities
resulted in the production of heavier elements by over the past 75 years or so. They are all unstable and
successive fusion reactions. This process, known as can only be created by processes that do not occur
nucleosynthesis, eventually led to the creation of all naturally on Earth.
the elements that are found on Earth today.
Each element is characterized by the number of
protons in the atomic nucleus and this is called the 1.5 ISOTOPES AND MASS
atomic number, represented by the symbol Z: NUMBER
Atomic number (Z) = Number of protons Although all the atoms of a particular element con-
tain the same number of protons, they may occur
For example, hydrogen has one proton, Z = 1, with different numbers of neutrons. This means
and helium has two protons, Z = 2. It is the number that an element can have several types of atoms. For
of electrons in an atom that determines its chemi- example, hydrogen can occur with zero, one or two
cal properties. In an electrically neutral atom, the neutrons in its nucleus, and the three different types
number of protons equals the number of electrons, of atoms are called isotopes of hydrogen.
and so, indirectly, it is the number of protons in The mass of an atom is determined by the num-
an atom that defines the element. Table 1.1 lists a ber of protons and neutrons if the very small mass
selection of elements with their symbols and atomic of the atomic electrons is neglected. The sum of the
numbers. number of protons plus the number of neutrons is
called the mass number and is represented by the P-33 has 15 protons and 18 neutrons (Z = 15, A = 33)
symbol A: P-34 has 15 protons and 19 neutrons (Z = 15, A = 34)
P-28 has 15 protons and 13 neutrons (Z = 15, A = 28) 1.6 ANCIENT AND MODERN
P-29 has 15 protons and 14 neutrons (Z = 15, A = 29) THEORIES
P-30 has 15 protons and 15 neutrons (Z = 15, A = 30)
P-31 has 15 protons and 16 neutrons (Z = 15, A = 31) It can now be seen that the ancient Greek philoso-
P-32 has 15 protons and 17 neutrons (Z = 15, A = 32) phers were remarkably close to the truth in their
e– e– e–
Ip In Ip In
Ip Ip
In
In In Ip In Ip
e– e– e–
Helium-3 Helium-4 Helium-5
theory that all substances are constituted from the up of even smaller particles called quarks, and there
same basic particles. However, instead of being dif- is some evidence of apparently more fundamental
ferent arrangements of only one type of particle, particles. Thus, the ancient Greeks may yet prove to
different substances appear to result from various have been right in their conjecture that there is just
combinations of protons, neutrons and electrons. It one fundamental particle that provides the basis for
is now known that protons and neutrons are made all others.
REVISION QUESTIONS
1. Following the illustration in Figure 1.1, draw an atom of each of the following nuclides:
a. 42 He
b. 63 Li
c. 73 Li
d. 84 Be
2. For each of the following nuclides of helium, sodium and uranium, how many protons, electrons and
neutrons are there in their atoms: 42 He, 11
23
Na, 238
92 U?
3. What are the masses and charges on the atomic scale of protons, electrons and neutrons?
5
Radioactivity and radiation
2.1 INTRODUCTION
It is found that a few naturally occurring substances
consist of atoms which are unstable, that is they
undergo spontaneous transformation into more
stable product atoms. Such substances are said to
be radioactive, and the transformation process is
known as radioactive decay. Radioactive decay
is usually accompanied by the emission of radia-
tion in the form of charged particles and gamma
(γ) rays.
The fact that some elements are naturally radio-
active was first realized by Becquerel in 1896. He
observed the blackening of photographic emulsions
in the vicinity of a uranium compound. This was sub-
sequently attributed to the effect of radiation being
emitted by the uranium. In the following 10 years,
the experimental work of Rutherford and Soddy,
Pierre and Marie Curie, and others established the
fact that some types of nuclei are unstable and decay
by emitting radiations of three main types, called
alpha, beta and gamma radiation.
During the same period, scientists in several
countries were experimenting with electrical dis-
charge tubes known as Crookes tubes and inves- Figure 2.1 The first medical X-ray.
tigating the fluorescence that occurred in the glass
walls of the tubes. In 1895, the German physicist within weeks investigators in many countries were
Wilhelm Conrad Rontgen discovered that the tubes developing equipment and techniques to exploit
were emitting invisible rays, which he named X-rays, the discovery. The first medical X-ray was taken by
that were capable of penetrating solid objects. The Rontgen himself and was of his wife’s hand (see
potential importance of this discovery, particularly Figure 2.1). When Frau Rontgen saw the photograph,
in the medical field, was quickly appreciated and she exclaimed ‘I have seen my death!’
7
Radioactivity and radiation
2.3 ELECTRONVOLT
α particle Radiation energy is expressed in electronvolts (eV).
2 protons and 2 neutrons
One electronvolt is the energy gained by an elec-
Mass of 4 units
Charge of +2 units tron in passing through an electrical potential of
1 volt (V). For example, in an X-ray tube, electrons
are accelerated from a heated tungsten filament
through an electrical potential of typically 100,000 V
β particle to the anode. The electrons therefore have an energy
Mass of 1/1840 units
Charge of –1 unit of 100,000 eV when they strike the anode.
The electronvolt is a very small unit, so radia-
tion energies are usually expressed in kilo (1000) or
mega (1,000,000) electronvolts:
γ ray
Electromagnetic One kiloelectronvolt = 1 keV = 1000 eV
radiation of very short
One megaelectronvolt = 1 MeV = 1000 keV
wavelength
Zero mass and charge = 1,000,000 eV
----------JAPAN: Start--------
JAPAN: A. D. 1890-1898.
Rise of Parliamentary parties.
Working of Constitutional Government.
H. N. G. Bushby,
Parliamentary Government in Japan
(Nineteenth Century, July, 1899).
"The history of the Japanese Parliament [see CONSTITUTION OF
JAPAN, in volume 1], briefly told, is as follows: The first
Diet was opened in November, 1890, and the twelfth session in
May, 1898. In this brief space of time there have been four
dissolutions and five Parliaments. From the very first the
collision between the Government and the Diet has been short
and violent. In the case of the first dissolution, in
December, 1891, the question turned on the Budget estimate,
the Diet insisting on the bold curtailment of items of
expenditure. In the second dissolution, in December, 1893, the
question turned on the memorial to be presented to the Throne,
the Opposition insisting in very strong terms on the necessity
of strictly enforcing the terms of treaties with Western
Powers, the Diet regarding the Cabinet as too weak-handed in
foreign politics. The third dissolution, in June, 1894, was
also on the same question. The Cabinet, in these two latter
cases, was under the presidency of Marquis Ito (then Count),
and was vigorously pushing forward negotiations for treaty
revision, through the brilliant diplomacy of Count Mutsu, the
Foreign Minister. This strict-enforcement agitation was looked
upon by the Government as a piece of anti-foreign agitation—a
Jingo movement—and as endangering the success of the
treaty-revision negotiations. In fact, the revised treaty with
Great Britain was on the latter date well-nigh completed, it
being signed in July following by Lord Kimberley and Viscount
Aoki. It was at this stage that the scepticism of foreign
observers as to the final success of representative
institutions in Japan seemed to reach its height. … Marquis
Ito and some of the most tried statesmen of the time were out
of office, forming a sort of reserve force, to be called out
at any grave emergency. But great was the disappointment when
it was seen that after Marquis Ito, with some of the most
trusted statesmen as his colleagues, had been in office but
little over a year, dissolution followed dissolution, and it
seemed that even the Father of the Constitution was unable to
manage its successful working. … There is no question that the
Constitutional situation was at that time exceedingly critical.
"But when the war broke out the situation was "But when the
war broke out the situation was completely changed. In the
August following the whole nation spoke and acted as if they
were one man and had but one mind. In the two sessions of the
Diet held during the war the Government was most ably
supported by the Diet, and everybody hoped that after the war
was over the same good-feeling would continue to rule the
Diet. On the other hand, it was well known that the Opposition
members in the Diet had clearly intimated that their support
of the Government was merely temporary, and that after the
emergency was over they might be expected to continue their
opposition policy. Sure enough, many months before the opening
of the ninth session, mutterings of deep discontent,
especially with reference to the retrocession of the Liaotung
peninsula, began to be widely heard, and it was much feared
that the former scenes of fierce opposition and blind
obstruction would be renewed. However, as the session
approached (December, 1896), rumours were heard of a certain
'entente' between the Government and the Liberal party, at
that time the largest and the best organised in the country.
And in the coming session the Government secured a majority,
through the support of the Liberals, for most of its important
Bills.
"Now this 'entente' between Marquis Ito and the Liberals was a
great step in advance in the constitutional history of the
country, and a very bold departure in a new direction on the
part of the Marquis. He was known to be an admirer of the
German system, and a chief upholder of the policy of Chozen
Naikaku, or the Transcendental Cabinet policy, which meant a
Ministry responsible to the Emperor alone. Marquis Ito saw
evidently at this stage the impossibility of carrying on the
Government without a secure parliamentary support, and Count
Itagaki, the Liberal leader, saw in the Marquis a faithful
ally, whose character as a great constructive statesman, and
whose history as the author of the Constitution, both forbade
his ever proving disloyal to the Constitution. The 'entente'
was cemented in May following by the entrance of Count Itagaki
into the Cabinet as the Home Minister. On the other hand, this
entente' led to the formation of the Progressist party by the
union of the six Opposition parties, as well as to the union
of Count Okuma, the Progressist leader, and Count Matsugata,
leader of the Kagoshima statesmen. Their united opposition was
now quite effective in harassing the administration. At this
stage certain neutral men, particularly Count Inouye,
suggested compromise, offering a scheme of a Coalition
Cabinet. … But Count Itagaki was firm in opposing such a
compromise, saying it was tantamount to the ignoring of party
distinction, and as such was a retrogression instead of being
a forward step in the constitutional history of the country.
He finally tendered his resignation. When Marquis Ito saw that
the Count was firm in his determination, he, too, resigned,
saying that he felt so deeply obliged to the Liberals for
their late parliamentary support that he would not let the
Count go out of office alone. Thus fell the Ito Ministry after
five years' brilliant service.
{279}
Tokiwo Yokoi,
New Japan and her Constitutional Outlook
(Contemporary Review, September, 1898).
JAPAN: A. D. 1895.
The war with China.
Treaty of Shimonoseki.
Korean independence secured.
Part of Feng-tien, Formosa and the Pescadores ceded by China.
Relinquishment of Feng-tien by Japan.
JAPAN: A. D. 1896.
Affairs in Formosa.
Retirement of Marquis Ito.
Progressists in power.
Destructive sea-wave.
JAPAN: A. D. 1897.
New tariff.
JAPAN: A. D. 1897-1898.
Contentions with Russia in Korea.
JAPAN: A. D. 1898-1899.
The struggle between clan government and party government.
{280}
"It now seemed to many that the death-blow had been given to
clan government, and that at last the era of government by
party had commenced. … The elements of which the Kensei-to was
composed were the two great ones of the Progressives, led by
Count Okuma, and the Liberals, led by Count Itagaki. These two
parties acted together in a condition of veiled hostility.
There was coalition without any approach to amalgamation. A
common hunger for office, a common dislike for clan
government, obscured for a little while a mutual jealousy and
distrust. Meanwhile the Kensei-to as a whole, and both wings
of it, were divided into endless clubs, cliques, and
associations. Our own Temperance, Colonial, Church, and China
parties are affable and self-effacing in comparison. Thus, to
name only a few of the political divisions of the Kensei-to,
there were the territorial associations of the Kwanto-kai (led
by Mr. Hoshi), the Hokuriku-kai (led by Mr. Sugita), the
Kyushu Kurabu (led by Mr. Matsuda), the Tohoku-dantai, the
Chugoku-kai, and the Shigoku-kai; there were the Satsuma
section, the Tosa section, the Kakushinto, the Young
Constitutionalists, the Senior Politicians (such as Baron
Kusumoto, Mr. Hiraoka, the chief organiser of the coalition,
and others), the Central Constitutionalist Club, and so forth.
Each clique had its private organisation and animosities; each
aspired to dictate to the Cabinet and secure portfolios for
its members in the House. They combined and recombined among
themselves. … Clearly, however loyally the two leaders wished
to work together, each must find it impossible in such
circumstances to preserve discipline among his own followers.
Indeed, the leaders scarcely tried to lead. … It was
impossible to carry on the Government under such conditions.
The Okuma-Itagaki Cabinet fell, and Field Marshal the Marquis
Yamagata, Premier of the first Japanese Ministry, was summoned
by the Emperor. Once more a clan Ministry, independent of
party, was formed; once more it seemed as though party
government was to be indefinitely postponed. … Marquis
Yamagata formed his Ministry in November 1898, on strictly
clan lines. … Being an old soldier, he wisely determined to
profit by experience and seek an ally. No one knew better than
himself the need of passing the Land Tax Bill, on which the
efficiency of the national defence and the future of Japan
depended. … It was natural, therefore, for him to approach the
Liberals, who had shown themselves favourable to an increase
of the Land Tax. … On the 27th of November the support of the
Liberals was assured, an event which prompted the 'Jiji' to
express its joy that Marquis Yamagata had become a party man,
leaving 'the mouldy, effete cause of the non-partisan
Ministry.' The Government party consisted now of the National
Unionists (in favour of clan government' and loyal followers
of Marquis Yamagata), the Liberals, and a few so-called
Independents (who, of course, speedily formed themselves into
a club), giving the Government a majority of about fifteen or
twenty votes in the House. …
H. N. G. Bushby,
Parliamentary Government in Japan
(Nineteenth Century, July, 1899).
"Japan has been promoted. The great sign that Europe regards a
Power as only semi-civilised is the demand that all who visit
it, or trade in it, should be exempted from the jurisdiction
of the local Courts, the Consuls acting when necessary as
Judges. This rule is maintained even when the Powers thus
stigmatised send Ambassadors, and is, no doubt, very keenly
resented. It seems specially offensive to the Japanese, who
have a high opinion of their own merits, and they have for
seventeen years demanded the treatment accorded to fully
civilised States. As the alliance of Japan is now earnestly
sought by all Europe this has been conceded, and on Monday,
July 17th, the Consular jurisdiction ceased. (Owing to some
blunder, the powers of the French and Austrian Consuls last a
fortnight longer, but the difference is only formal.) The
Japanese are highly delighted, and the European traders are
not displeased, as with the Consular jurisdictions all
restrictions on trading with the interior disappear."
The Spectator
(London), July 22, 1899.
{281}
With still finer care for the honor and good name of Japan,
the following instruction to schools was published on the same
day by Count Kabayma, the Minister of State for Education:
"The schools under the direct control of the Government serve
as models to all the public and private educational
institutions throughout the country. It is therefore my
earnest desire that the behavior of the students at such
schools should be regulated with notably strict regard to the
canons of propriety, so that they may show themselves worthy
of the station they occupy. The date of the operation of the
revised treaties is now imminent, and His Imperial Majesty has
issued a gracious rescript. It may be expected that the coming
and going of foreigners in the interior of the country will
henceforth grow more frequent, and if at such a time students
be left without proper control, and suffered to neglect the
dictates of propriety by cherishing sentiments of petty
arrogance and behaving in a violent, outrageous, or vulgar
manner, not only will the educational systems be brought into
discredit, but also the prestige of the country will be
impaired and its reputation may even be destroyed. For that
reason I have addressed an instruction to the local governors
urging them to guard against any defects in educational
methods, and I am now constrained to appeal to the Government
schools which serve for models. I trust that those upon whom
the functions of direction and teaching devolve, paying
respectful attention to the august intention, will discharge
their duties carefully towards the students, and, by securing
the latter's strict adherence to rules, will contrive that
they shall serve as a worthy example to the schools throughout
the country."
{282}
JAPAN: A. D. 1900.
Naval strength.
JAPAN: A. D. 1900-1901.
Strategic importance of Korea.
Interest in the designs of Russia.
JAPAN: A. D. 1901.
Movement to erect a monument to commemorate the
visit of Commodore Perry.
----------JAPAN: End--------